rino 0.1.0
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- data/README +44 -0
- data/Rakefile +123 -0
- data/ext/extconf.rb +26 -0
- data/ext/ruby_inchi_main.so +0 -0
- data/ext/src/aux2atom.h +2786 -0
- data/ext/src/comdef.h +148 -0
- data/ext/src/e_0dstereo.c +3014 -0
- data/ext/src/e_0dstereo.h +31 -0
- data/ext/src/e_comdef.h +57 -0
- data/ext/src/e_ctl_data.h +147 -0
- data/ext/src/e_ichi_io.c +498 -0
- data/ext/src/e_ichi_io.h +40 -0
- data/ext/src/e_ichi_parms.c +37 -0
- data/ext/src/e_ichi_parms.h +41 -0
- data/ext/src/e_ichicomp.h +50 -0
- data/ext/src/e_ichierr.h +40 -0
- data/ext/src/e_ichimain.c +593 -0
- data/ext/src/e_ichisize.h +43 -0
- data/ext/src/e_inchi_atom.c +75 -0
- data/ext/src/e_inchi_atom.h +33 -0
- data/ext/src/e_inpdef.h +41 -0
- data/ext/src/e_mode.h +706 -0
- data/ext/src/e_mol2atom.c +649 -0
- data/ext/src/e_readinch.c +58 -0
- data/ext/src/e_readmol.c +54 -0
- data/ext/src/e_readmol.h +180 -0
- data/ext/src/e_readstru.c +251 -0
- data/ext/src/e_readstru.h +33 -0
- data/ext/src/e_util.c +284 -0
- data/ext/src/e_util.h +61 -0
- data/ext/src/extr_ct.h +251 -0
- data/ext/src/ichi.h +206 -0
- data/ext/src/ichi_bns.c +7999 -0
- data/ext/src/ichi_bns.h +231 -0
- data/ext/src/ichican2.c +5000 -0
- data/ext/src/ichicano.c +2195 -0
- data/ext/src/ichicano.h +49 -0
- data/ext/src/ichicans.c +1625 -0
- data/ext/src/ichicant.h +379 -0
- data/ext/src/ichicomn.h +260 -0
- data/ext/src/ichicomp.h +50 -0
- data/ext/src/ichidrp.h +119 -0
- data/ext/src/ichierr.h +124 -0
- data/ext/src/ichiisot.c +101 -0
- data/ext/src/ichilnct.c +286 -0
- data/ext/src/ichimain.h +132 -0
- data/ext/src/ichimak2.c +1189 -0
- data/ext/src/ichimake.c +3812 -0
- data/ext/src/ichimake.h +205 -0
- data/ext/src/ichimap1.c +851 -0
- data/ext/src/ichimap2.c +2856 -0
- data/ext/src/ichimap4.c +1609 -0
- data/ext/src/ichinorm.c +741 -0
- data/ext/src/ichinorm.h +67 -0
- data/ext/src/ichiparm.c +45 -0
- data/ext/src/ichiparm.h +1441 -0
- data/ext/src/ichiprt1.c +3612 -0
- data/ext/src/ichiprt2.c +1511 -0
- data/ext/src/ichiprt3.c +3011 -0
- data/ext/src/ichiqueu.c +1003 -0
- data/ext/src/ichiring.c +326 -0
- data/ext/src/ichiring.h +49 -0
- data/ext/src/ichisize.h +35 -0
- data/ext/src/ichisort.c +539 -0
- data/ext/src/ichister.c +3538 -0
- data/ext/src/ichister.h +35 -0
- data/ext/src/ichitaut.c +3843 -0
- data/ext/src/ichitaut.h +387 -0
- data/ext/src/ichitime.h +74 -0
- data/ext/src/inchi_api.h +670 -0
- data/ext/src/inchi_dll.c +1480 -0
- data/ext/src/inchi_dll.h +34 -0
- data/ext/src/inchi_dll_main.c +23 -0
- data/ext/src/inchi_dll_main.h +31 -0
- data/ext/src/inpdef.h +328 -0
- data/ext/src/lreadmol.h +1246 -0
- data/ext/src/mode.h +706 -0
- data/ext/src/ruby_inchi_main.c +558 -0
- data/ext/src/runichi.c +4179 -0
- data/ext/src/strutil.c +3861 -0
- data/ext/src/strutil.h +182 -0
- data/ext/src/util.c +1130 -0
- data/ext/src/util.h +85 -0
- data/lib/clean_tempfile.rb +220 -0
- data/lib/rino.rb +111 -0
- data/test/test.rb +386 -0
- metadata +130 -0
data/ext/src/strutil.c
ADDED
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/*
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* International Union of Pure and Applied Chemistry (IUPAC)
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* International Chemical Identifier (InChI)
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* Version 1
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* Software version 1.00
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* April 13, 2005
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* Developed at NIST
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*/
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#include <stdio.h>
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#include <stdlib.h>
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#include <string.h>
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#include <ctype.h>
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#include <math.h>
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#include "mode.h"
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#include "inpdef.h"
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#include "util.h"
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#include "ichi.h"
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#include "strutil.h"
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#include "ichierr.h"
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#include "ichicomp.h"
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#include "extr_ct.h"
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#include "ichister.h"
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/* local prototypes */
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int cmp_components( const void *a1, const void *a2 );
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int mark_one_struct_component( inp_ATOM* at, int j, AT_NUMB *mark, AT_NUMB num_disconnected_components );
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int Free_INChI_Stereo( INChI_Stereo *pINChI_Stereo );
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INChI_Stereo *Alloc_INChI_Stereo(int num_at, int num_bonds);
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int RemoveInpAtBond( inp_ATOM *at, int iat, int k );
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int DisconnectInpAtBond( inp_ATOM *at, AT_NUMB *nOldCompNumber, int iat, int neigh_ord );
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int move_explicit_Hcation(inp_ATOM *at, int num_at, int iat, int iat_H, int bInAllComponents);
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int DisconnectOneLigand( inp_ATOM *at, AT_NUMB *nOldCompNumber, S_CHAR *bMetal, char *elnumber_Heteroat,
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int num_halogens, int num_atoms, int iMetal, int jLigand, INCHI_MODE *bTautFlagsDone );
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int bIsAmmoniumSalt( inp_ATOM *at, int i, int *piO, int *pk, S_CHAR *num_explicit_H );
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int DisconnectAmmoniumSalt ( inp_ATOM *at, int i, int iO, int k, S_CHAR *num_explicit_H );
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int bIsMetalSalt( inp_ATOM *at, int i );
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int DisconnectMetalSalt( inp_ATOM *at, int i );
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int bIsMetalToDisconnect(inp_ATOM *at, int i, int bCheckMetalValence);
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int get_iat_number( int el_number, const int el_num[], int el_num_len );
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int tot_unsat( int unsat[] );
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int max_unsat( int unsat[] );
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double dist3D( inp_ATOM *at1, inp_ATOM *at2 );
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double dist2D( inp_ATOM *at1, inp_ATOM *at2 );
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double dist_from_segm( double x, double y, double x1, double y1, double x2, double y2);
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int segments_intersect( double x11, double y11, double x12, double y12, /* segment #1 */
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double x21, double y21, double x22, double y22 );
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double GetMinDistDistribution( inp_ATOM *at, int num_at, int iat, int iat_H,
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int bInAllComponents, double min_dist[], int num_segm );
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int nFindOneOM(inp_ATOM *at, int at_no, int ord_OM[], int num_OM);
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int the_only_doublet_neigh(inp_ATOM *at, int i1, int *ineigh1, int *ineigh2);
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#ifndef NUMH
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#define NUM_ISO_H(AT,N) (AT[N].num_iso_H[0]+AT[N].num_iso_H[1]+AT[N].num_iso_H[2])
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#define NUMH(AT,N) (AT[N].num_H+NUM_ISO_H(AT,N))
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#endif
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/************************************************************************/
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int the_only_doublet_neigh(inp_ATOM *at, int i1, int *ineigh1, int *ineigh2)
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{
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int i, neigh1, num_rad1=0, num_rad2=0;
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inp_ATOM *a = at+i1, *b;
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if ( RADICAL_DOUBLET != a->radical )
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return -1;
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for ( i = 0; i < a->valence; i ++ ) {
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b = at + (neigh1 = (int)a->neighbor[i]);
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if ( RADICAL_DOUBLET == b->radical ) {
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num_rad1 ++;
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*ineigh1 = i;
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}
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}
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if ( 1 == num_rad1 ) {
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a = at + (neigh1 = (int)a->neighbor[*ineigh1]);
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for ( i = 0; i < a->valence; i ++ ) {
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b = at +(int)a->neighbor[i];
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if ( RADICAL_DOUBLET == b->radical ) {
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num_rad2 ++;
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*ineigh2 = i;
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}
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}
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if ( 1 == num_rad2 ) {
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return neigh1;
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}
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}
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return -1;
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}
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/************************************************************************/
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int fix_odd_things( int num_atoms, inp_ATOM *at )
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{ /* 0 1 2 3 4 5 6 7 8 9 */
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static const char el[] = "N;P;As;Sb;O;S;Se;Te;"; /* 8 elements + C, Si */
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static U_CHAR en[10]; /* same number: 8 elements */
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static int ne=0, ne2; /* will be 8 and 10 */
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static int el_number_P;
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static int el_number_H;
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static int el_number_C;
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static int el_number_O;
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static int el_number_Si;
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#define FIRST_NEIGHB2 4
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#define FIRST_CENTER2 5
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#define NUM_CENTERS_N 4
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int i1, i2, k1, k2, c, num_changes = 0;
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char elname[ATOM_EL_LEN];
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if ( !ne ) { /* one time initialization */
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const char *b, *e;
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int len;
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for ( b = el; e = strchr( b, ';'); b = e+1 ) {
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len = e-b;
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memcpy( elname, b, len );
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elname[len] = '\0';
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en[ne++] = get_periodic_table_number( elname );
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}
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ne2 = ne;
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el_number_P = get_periodic_table_number( "P" );
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el_number_H = get_periodic_table_number( "H" );
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el_number_O = get_periodic_table_number( "O" );
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en[ne2++] = el_number_C = get_periodic_table_number( "C" );
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en[ne2++] = el_number_Si = get_periodic_table_number( "Si" );
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}
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/* H(-)-X -> H-X(-); H(+)-X -> H-X(+) */
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for ( i1 = 0; i1 < num_atoms; i1 ++ ) {
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if ( 1 == at[i1].valence &&
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1 == abs(at[i1].charge) &&
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(0 == at[i1].radical || RADICAL_SINGLET == at[i1].radical) &&
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BOND_TYPE_SINGLE == at[i1].bond_type[0] &&
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el_number_H == at[i1].el_number &&
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el_number_H != at[i2=(int)at[i1].neighbor[0]].el_number &&
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!NUMH(at,i1) &&
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!NUMH(at,i2)
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) {
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at[i2].charge += at[i1].charge;
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at[i1].charge = 0;
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}
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}
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/* replace XHm(-)--Y==XHn(+) with XHm==Y--XHn, (n>=0 ,m>=0, X=N,P,As,Sb,O,S,Se,Te) */
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for ( i1 = 0; i1 < num_atoms; i1 ++ ) {
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if ( 1 != at[i1].charge ||
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at[i1].radical && RADICAL_SINGLET != at[i1].radical ||
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at[i1].chem_bonds_valence == at[i1].valence ||
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!memchr(en, at[i1].el_number, ne) ||
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get_el_valence( at[i1].el_number, at[i1].charge, 0 ) != at[i1].chem_bonds_valence+NUMH(at,i1) ) {
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continue;
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}
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/* found a candidate at[i1] for X in XHn(+) */
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159
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if ( 1 == at[i1].valence &&
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BOND_TYPE_DOUBLE == at[i1].bond_type[0] ) {
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c = (int)at[i1].neighbor[0];
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for ( k2 = 0; k2 < at[c].valence; k2 ++ ) {
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i2 = at[c].neighbor[k2];
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if ( 1 == at[i2].valence &&
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165
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-1 == at[i2].charge &&
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166
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at[i2].el_number == at[i1].el_number && /* exact match */
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167
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(0 == at[i2].radical || RADICAL_SINGLET == at[i2].radical) &&
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168
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BOND_TYPE_SINGLE == at[i2].bond_type[0] &&
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169
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/*memchr(en, at[i2].el_number, ne) &&*/
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get_el_valence( at[i2].el_number, at[i2].charge, 0 ) == at[i2].chem_bonds_valence+NUMH(at,i2) ) {
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171
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/* found both X(-) and X(+); change bonds and remove charges */
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for ( k1 = 0; k1 < at[c].valence && i1 != at[c].neighbor[k1]; k1 ++ )
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;
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174
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at[i1].charge = at[i2].charge = 0;
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at[i1].bond_type[0] = at[c].bond_type[k1] = BOND_TYPE_SINGLE;
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176
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at[i1].chem_bonds_valence --;
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at[i2].bond_type[0] = at[c].bond_type[k2] = BOND_TYPE_DOUBLE;
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178
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at[i2].chem_bonds_valence ++;
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179
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num_changes ++;
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180
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break;
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181
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}
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182
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}
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183
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}
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184
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else {
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185
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/* explicit H case: detect H-neighbors and Y */
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186
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int ineigh, neigh, i1_c, i2_c, num_H_i1, num_H_i2;
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187
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for ( ineigh = 0, num_H_i1 = 0, i1_c = -1; ineigh < at[i1].valence; ineigh ++ ) {
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188
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neigh = at[i1].neighbor[ineigh];
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189
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if ( at[neigh].el_number == el_number_H ) {
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190
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if ( at[neigh].chem_bonds_valence == 1 &&
|
191
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(0 == at[neigh].radical || RADICAL_SINGLET == at[neigh].radical)
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192
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) {
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193
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num_H_i1 ++; /* found H-neighbor */
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194
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} else {
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195
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break; /* wrong neighbor */
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196
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}
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197
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} else
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198
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if ( at[i1].bond_type[ineigh] == BOND_TYPE_DOUBLE ) {
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199
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/* found a candidate for Y; bond must bedouble */
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200
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i1_c = ineigh;
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201
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c = neigh;
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202
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}
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203
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}
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204
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if ( i1_c < 0 || num_H_i1 + 1 != at[i1].valence ) {
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205
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continue;
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206
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}
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207
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for ( k2 = 0; k2 < at[c].valence; k2 ++ ) {
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208
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i2 = at[c].neighbor[k2];
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209
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if (-1 == at[i2].charge &&
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210
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at[i2].el_number == at[i1].el_number && /* exact match */
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211
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(0 == at[i2].radical || RADICAL_SINGLET == at[i2].radical) &&
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212
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get_el_valence( at[i2].el_number, at[i2].charge, 0 ) == at[i2].chem_bonds_valence+NUMH(at,i2) ) {
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213
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for ( ineigh = 0, num_H_i2 = 0, i2_c = -1; ineigh < at[i2].valence; ineigh ++ ) {
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214
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neigh = at[i2].neighbor[ineigh];
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215
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if ( at[neigh].el_number == el_number_H ) {
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216
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if ( at[neigh].chem_bonds_valence == 1 &&
|
217
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(0 == at[neigh].radical || RADICAL_SINGLET == at[neigh].radical)
|
218
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) {
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219
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num_H_i2 ++; /* found H-neighbor */
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220
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} else {
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221
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break; /* wrong neighbor */
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222
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}
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223
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} else
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224
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if ( c == neigh && at[i2].bond_type[ineigh] == BOND_TYPE_SINGLE ) {
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225
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i2_c = ineigh; /* position of Y neighbor; bond must be single */
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226
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} else {
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227
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break;
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228
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}
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229
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}
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230
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if ( num_H_i2 + (i2_c >= 0) != at[i2].valence ) {
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231
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continue;
|
232
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}
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233
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/* found both X(-) and X(+); change bonds and remove charges */
|
234
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for ( k1 = 0; k1 < at[c].valence && i1 != at[c].neighbor[k1]; k1 ++ )
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235
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;
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236
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at[i1].charge = at[i2].charge = 0;
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237
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at[i1].bond_type[i1_c] = at[c].bond_type[k1] = BOND_TYPE_SINGLE;
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238
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at[i1].chem_bonds_valence --;
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239
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at[i2].bond_type[i2_c] = at[c].bond_type[k2] = BOND_TYPE_DOUBLE;
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240
|
+
at[i2].chem_bonds_valence ++;
|
241
|
+
num_changes ++;
|
242
|
+
break;
|
243
|
+
}
|
244
|
+
}
|
245
|
+
}
|
246
|
+
}
|
247
|
+
|
248
|
+
/* Replace
|
249
|
+
|
250
|
+
X- X X=O,S,Se,Te -- terminal atoms (NEIGHB2)
|
251
|
+
\ | \ ||
|
252
|
+
>Y++ with >Y Y=S,Se,Te -- central cation (CENTER2)
|
253
|
+
/ | / ||
|
254
|
+
X- X Y valence=4, original Y bond valence = 4
|
255
|
+
|
256
|
+
|
257
|
+
|
258
|
+
|
259
|
+
X- X X=O,S,Se,Te -- terminal atoms (NEIGHB2)
|
260
|
+
\ | \ ||
|
261
|
+
>P+ with >P
|
262
|
+
/ | / |
|
263
|
+
X- X- Y valence=4, original Y bond valence = 4
|
264
|
+
|
265
|
+
*/
|
266
|
+
|
267
|
+
for ( i1 = 0; i1 < num_atoms; i1 ++ ) {
|
268
|
+
if ( 1 == at[i1].valence &&
|
269
|
+
-1 == at[i1].charge &&
|
270
|
+
(0 == at[i1].radical || RADICAL_SINGLET == at[i1].radical) &&
|
271
|
+
!NUMH(at,i1) &&
|
272
|
+
BOND_TYPE_SINGLE == at[i1].bond_type[0] &&
|
273
|
+
memchr( en+FIRST_NEIGHB2, at[i1].el_number, ne-FIRST_NEIGHB2 )) {
|
274
|
+
int charge, i;
|
275
|
+
/* found a candidate for X */
|
276
|
+
c = (int)at[i1].neighbor[0]; /* candidate for Y */
|
277
|
+
if ( ((charge=2) == at[c].charge && memchr( en+FIRST_CENTER2, at[c].el_number, ne-FIRST_CENTER2) ||
|
278
|
+
(charge=1) == at[c].charge && el_number_P==at[c].el_number ) &&
|
279
|
+
4 == at[c].valence &&
|
280
|
+
(0 == at[c].radical || RADICAL_SINGLET == at[c].radical ) &&
|
281
|
+
at[c].valence == at[c].chem_bonds_valence &&
|
282
|
+
!NUMH(at,c) ) {
|
283
|
+
; /* accept */
|
284
|
+
} else {
|
285
|
+
continue; /* ignore at[i1] */
|
286
|
+
}
|
287
|
+
for ( k2 = 0; k2 < at[c].valence; k2 ++ ) {
|
288
|
+
i2 = at[c].neighbor[k2];
|
289
|
+
if ( i2 == i1 ) {
|
290
|
+
continue;
|
291
|
+
}
|
292
|
+
if ( 1 == at[i2].valence &&
|
293
|
+
-1 == at[i2].charge &&
|
294
|
+
memchr( en+FIRST_NEIGHB2, at[i2].el_number, ne-FIRST_NEIGHB2 ) &&
|
295
|
+
/*at[i2].el_number == at[i1].el_number &&*/ /* exact match */
|
296
|
+
(0 == at[i2].radical || RADICAL_SINGLET == at[i2].radical) &&
|
297
|
+
!NUMH(at,i2) &&
|
298
|
+
BOND_TYPE_SINGLE == at[i2].bond_type[0] ) {
|
299
|
+
/* found both X(-) and X(-); change bonds and remove charges */
|
300
|
+
for ( k1 = 0; k1 < at[c].valence && i1 != at[c].neighbor[k1]; k1 ++ )
|
301
|
+
;
|
302
|
+
for ( i = 0; i < charge; i ++ ) {
|
303
|
+
/* in case of P it does not matter which X atom is neutralized
|
304
|
+
because of tautomerism. However, neutral central atom is important
|
305
|
+
for the neutralization of the components */
|
306
|
+
switch( i ) {
|
307
|
+
case 0:
|
308
|
+
at[i1].charge = 0;
|
309
|
+
at[i1].bond_type[0] = at[c].bond_type[k1] = BOND_TYPE_DOUBLE;
|
310
|
+
at[i1].bond_stereo[0] = at[c].bond_stereo[k1] = 0;
|
311
|
+
at[i1].chem_bonds_valence ++;
|
312
|
+
at[c].chem_bonds_valence ++;
|
313
|
+
num_changes ++;
|
314
|
+
break;
|
315
|
+
case 1:
|
316
|
+
at[i2].charge = 0;
|
317
|
+
at[i2].bond_type[0] = at[c].bond_type[k2] = BOND_TYPE_DOUBLE;
|
318
|
+
at[i2].bond_stereo[0] = at[c].bond_stereo[k2] = 0;
|
319
|
+
at[i2].chem_bonds_valence ++;
|
320
|
+
at[c].chem_bonds_valence ++;
|
321
|
+
num_changes ++;
|
322
|
+
break;
|
323
|
+
}
|
324
|
+
}
|
325
|
+
break;
|
326
|
+
}
|
327
|
+
}
|
328
|
+
}
|
329
|
+
}
|
330
|
+
|
331
|
+
/* A(doublet)-B(doublet) -> A=B (A and B have no other doublet neighbors) */
|
332
|
+
/* A(doublet)=B(doublet) -> A#B (A and B have no other doublet neighbors) */
|
333
|
+
for( i1 = 0; i1 < num_atoms; i1 ++ ) {
|
334
|
+
if ( RADICAL_DOUBLET == at[i1].radical &&
|
335
|
+
0 <= (i2=the_only_doublet_neigh(at, i1, &k1, &k2)) ) {
|
336
|
+
if ( at[i1].bond_type[k1] <= BOND_TYPE_DOUBLE ) {
|
337
|
+
at[i1].bond_type[k1] ++;
|
338
|
+
at[i1].chem_bonds_valence ++;
|
339
|
+
at[i2].bond_type[k2] ++;
|
340
|
+
at[i2].chem_bonds_valence ++;
|
341
|
+
at[i1].radical = 0;
|
342
|
+
at[i2].radical = 0;
|
343
|
+
}
|
344
|
+
}
|
345
|
+
}
|
346
|
+
|
347
|
+
#if( REMOVE_ION_PAIRS_EARLY == 1 )
|
348
|
+
|
349
|
+
num_changes += remove_ion_pairs( num_atoms, at );
|
350
|
+
#endif
|
351
|
+
|
352
|
+
return num_changes;
|
353
|
+
}
|
354
|
+
/************************************************************************/
|
355
|
+
int post_fix_odd_things( int num_atoms, inp_ATOM *at )
|
356
|
+
{
|
357
|
+
int num_changes = 0;
|
358
|
+
/* currently does nothing */
|
359
|
+
return num_changes;
|
360
|
+
}
|
361
|
+
/************************************************************************/
|
362
|
+
int nFindOneOM(inp_ATOM *at, int at_no, int ord_OM[], int num_OM)
|
363
|
+
{
|
364
|
+
int i, n_OM, n_OM_best, best_value, cur_value, diff;
|
365
|
+
int num_best;
|
366
|
+
|
367
|
+
if ( 1 == num_OM ) {
|
368
|
+
return ord_OM[0];
|
369
|
+
}
|
370
|
+
if ( 1 > num_OM ) {
|
371
|
+
return -1;
|
372
|
+
}
|
373
|
+
|
374
|
+
/* select neighbors with min. number of bonds */
|
375
|
+
num_best = 1;
|
376
|
+
n_OM = (int)at[at_no].neighbor[ord_OM[0]];
|
377
|
+
best_value = (int)at[n_OM].valence;
|
378
|
+
/* compare number of bonds; move indexes of the best neighbors to the first elements of ord_OM[] */
|
379
|
+
for ( i = 1; i < num_OM; i ++ ) {
|
380
|
+
n_OM = at[at_no].neighbor[ord_OM[i]];
|
381
|
+
cur_value = (int)at[n_OM].valence;
|
382
|
+
diff = cur_value - best_value;
|
383
|
+
if ( diff < 0 ) {
|
384
|
+
n_OM_best = n_OM;
|
385
|
+
best_value = cur_value;
|
386
|
+
ord_OM[0] = ord_OM[i];
|
387
|
+
num_best = 1;
|
388
|
+
} else
|
389
|
+
if ( diff == 0 ) { /* was '=', pointed by WDI */
|
390
|
+
ord_OM[num_best ++] = ord_OM[i];
|
391
|
+
}
|
392
|
+
}
|
393
|
+
num_OM = num_best;
|
394
|
+
if ( 1 == num_OM ) {
|
395
|
+
return ord_OM[0];
|
396
|
+
}
|
397
|
+
/* select neighbors with min. periodic numbers */
|
398
|
+
num_best = 1;
|
399
|
+
n_OM = (int)at[at_no].neighbor[ord_OM[0]];
|
400
|
+
best_value = (int)at[n_OM].el_number;
|
401
|
+
/* compare periodic numbers; move indexes of the best neighbors to the first elements of ord_OM[] */
|
402
|
+
for ( i = 1; i < num_OM; i ++ ) {
|
403
|
+
n_OM = at[at_no].neighbor[ord_OM[i]];
|
404
|
+
cur_value = (int)at[n_OM].el_number;
|
405
|
+
diff = cur_value - best_value;
|
406
|
+
if ( diff < 0 ) {
|
407
|
+
n_OM_best = n_OM;
|
408
|
+
best_value = cur_value;
|
409
|
+
ord_OM[0] = ord_OM[i];
|
410
|
+
num_best = 1;
|
411
|
+
} else
|
412
|
+
if ( diff == 0 ) { /* was '=', pointed by WDI */
|
413
|
+
ord_OM[num_best ++] = ord_OM[i];
|
414
|
+
}
|
415
|
+
}
|
416
|
+
num_OM = num_best;
|
417
|
+
if ( 1 == num_OM ) {
|
418
|
+
return ord_OM[0];
|
419
|
+
}
|
420
|
+
/* if neighbors are not terminal atoms then reject */
|
421
|
+
if ( 1 < at[n_OM].valence ) {
|
422
|
+
return -1;
|
423
|
+
}
|
424
|
+
/* if neighbors are terminal atoms then the one without isotope or with lightest isotope */
|
425
|
+
num_best = 1;
|
426
|
+
n_OM = (int)at[at_no].neighbor[ord_OM[0]];
|
427
|
+
best_value = (int)at[n_OM].iso_atw_diff;
|
428
|
+
/* compare periodic numbers; move indexes of the best neighbors to the first elements of ord_OM[] */
|
429
|
+
for ( i = 1; i < num_OM; i ++ ) {
|
430
|
+
n_OM = at[at_no].neighbor[ord_OM[i]];
|
431
|
+
cur_value = (int)at[n_OM].el_number;
|
432
|
+
diff = cur_value - best_value;
|
433
|
+
if ( (!cur_value && best_value) || diff < 0 ) {
|
434
|
+
n_OM_best = n_OM;
|
435
|
+
best_value = cur_value;
|
436
|
+
ord_OM[0] = ord_OM[i];
|
437
|
+
num_best = 1;
|
438
|
+
} else
|
439
|
+
if ( diff == 0 ) { /* was '=', pointed by WDI */
|
440
|
+
ord_OM[num_best ++] = ord_OM[i];
|
441
|
+
}
|
442
|
+
}
|
443
|
+
num_OM = num_best;
|
444
|
+
if ( 1 == num_OM ) {
|
445
|
+
return ord_OM[0];
|
446
|
+
}
|
447
|
+
/* return any */
|
448
|
+
return ord_OM[0];
|
449
|
+
}
|
450
|
+
/************************************************************************/
|
451
|
+
/* the bonds are fixed in fix_special_bonds() */
|
452
|
+
int remove_ion_pairs( int num_atoms, inp_ATOM *at )
|
453
|
+
{
|
454
|
+
int num_changes = 0;
|
455
|
+
|
456
|
+
/* 0 1 2 3 4 5 6 7 8 9 8 9 */
|
457
|
+
static const char el[] = "N;P;As;Sb;O;S;Se;Te;C;Si"; /* 8 elements + C, Si */
|
458
|
+
static char en[12]; /* same number: 8 elements */
|
459
|
+
static int ne=0; /* will be 8 and 10 */
|
460
|
+
|
461
|
+
#define ELEM_N_FST 0
|
462
|
+
#define ELEM_N_LEN 4
|
463
|
+
#define ELEM_O_FST 4
|
464
|
+
#define ELEM_O_LEN 4
|
465
|
+
#define ELEM_C_FST 8
|
466
|
+
#define ELEM_C_LEN 2
|
467
|
+
|
468
|
+
#define MAX_NEIGH 6
|
469
|
+
|
470
|
+
int i, n, n2, i1, i2, i3, i4, type, chrg;
|
471
|
+
int num_C_II=0, num_C_plus=0, num_C_minus=0, num_N_plus=0, num_N_minus=0, num_O_plus=0, num_O_minus=0, num_All;
|
472
|
+
inp_ATOM *a;
|
473
|
+
char elname[ATOM_EL_LEN], *p;
|
474
|
+
if ( !ne ) { /* one time initialization */
|
475
|
+
const char *b, *e;
|
476
|
+
int len;
|
477
|
+
for ( b = el; e = strchr( b, ';'); b = e+1 ) {
|
478
|
+
len = e-b;
|
479
|
+
memcpy( elname, b, len );
|
480
|
+
elname[len] = '\0';
|
481
|
+
en[ne++] = get_periodic_table_number( elname );
|
482
|
+
}
|
483
|
+
en[ne] = '\0';
|
484
|
+
}
|
485
|
+
|
486
|
+
/****** count candidates ********/
|
487
|
+
for ( i = 0, a = at; i < num_atoms; i ++, a++ ) {
|
488
|
+
if ( 1 == (chrg=a->charge) || -1 == chrg ) {
|
489
|
+
if ( p = (char*)memchr( en, a->el_number, ne) ) {
|
490
|
+
n = p - en;
|
491
|
+
if ( n >= ELEM_C_FST ) {
|
492
|
+
if ( chrg > 0 )
|
493
|
+
num_C_plus ++;
|
494
|
+
else
|
495
|
+
num_C_minus ++;
|
496
|
+
} else
|
497
|
+
if ( n >= ELEM_O_FST ) {
|
498
|
+
if ( chrg > 0 )
|
499
|
+
num_O_plus ++;
|
500
|
+
else
|
501
|
+
num_O_minus ++;
|
502
|
+
} else {
|
503
|
+
if ( chrg > 0 )
|
504
|
+
num_N_plus ++;
|
505
|
+
else
|
506
|
+
num_N_minus ++;
|
507
|
+
}
|
508
|
+
}
|
509
|
+
} else
|
510
|
+
if ( !chrg && a->chem_bonds_valence + NUMH(a, 0) == 2 &&
|
511
|
+
get_el_valence( a->el_number, 0, 0 ) == 4 &&
|
512
|
+
NULL != memchr( en+ELEM_C_FST, a->el_number, ELEM_C_LEN) ) {
|
513
|
+
num_C_II ++;
|
514
|
+
}
|
515
|
+
}
|
516
|
+
num_All = num_C_II + num_C_plus + num_C_minus + num_N_plus + num_N_minus + num_O_plus + num_O_minus;
|
517
|
+
if ( !num_All ) {
|
518
|
+
return 0;
|
519
|
+
}
|
520
|
+
|
521
|
+
/**************************************************************************/
|
522
|
+
/*************************** Terminal ion pairs ***************************/
|
523
|
+
/**************************************************************************/
|
524
|
+
|
525
|
+
/*-------------------------------------------------------------------------
|
526
|
+
Pair type 1 N=N,P,As,Sb; O=O,S,Se,Te
|
527
|
+
===========
|
528
|
+
|
529
|
+
X X if X is another -O(-) then neutralize O(-)
|
530
|
+
| | that has a higher periodic table number
|
531
|
+
O=N(+)-O(-) => O=N=O
|
532
|
+
i n
|
533
|
+
--------------------------------------------------------------------------*/
|
534
|
+
for ( type = 1; type <= 18; type ++ ) {
|
535
|
+
if ( (!type || 1 == type) ) {
|
536
|
+
for ( i = 0; i < num_atoms && 0 < num_N_plus && 0 < num_O_minus; i ++ ) {
|
537
|
+
if ( 1 == at[i].charge && 3 == nNoMetalNumBonds(at, i) &&
|
538
|
+
4 == nNoMetalBondsValence(at, i) &&
|
539
|
+
NULL != memchr( en+ELEM_N_FST, at[i].el_number, ELEM_N_LEN) ) {
|
540
|
+
int num_OM = 0, ord_OM[3]; /* -O(-) */
|
541
|
+
int num_O = 0; /* =O */
|
542
|
+
int num_O_other = 0;
|
543
|
+
for ( i1 = 0; i1 < at[i].valence; i1 ++ ) {
|
544
|
+
n = at[i].neighbor[i1];
|
545
|
+
if ( 1 == nNoMetalNumBonds(at, n) && 0 == num_of_H( at, n ) &&
|
546
|
+
NULL != (p = (char*)memchr( en+ELEM_O_FST, at[n].el_number, ELEM_O_LEN)) ) {
|
547
|
+
if ( BOND_TYPE_SINGLE == at[i].bond_type[i1] &&
|
548
|
+
-1 == at[n].charge ) {
|
549
|
+
ord_OM[num_OM ++] = i1;
|
550
|
+
} else
|
551
|
+
if ( BOND_TYPE_DOUBLE == at[n].bond_type[0] &&
|
552
|
+
0 == at[n].charge ) {
|
553
|
+
num_O ++;
|
554
|
+
} else {
|
555
|
+
num_O_other ++;
|
556
|
+
}
|
557
|
+
}
|
558
|
+
}
|
559
|
+
if ( num_OM > 0 && num_O > 0 && !num_O_other &&
|
560
|
+
0 <= (i1=nFindOneOM(at, i, ord_OM, num_OM)) ) {
|
561
|
+
/* remove charges and increase bond order */
|
562
|
+
n = at[i].neighbor[i1];
|
563
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor;
|
564
|
+
at[i].bond_type[i1] ++;
|
565
|
+
at[n].bond_type[i2] ++;
|
566
|
+
at[i].chem_bonds_valence ++;
|
567
|
+
at[n].chem_bonds_valence ++;
|
568
|
+
at[i].charge --;
|
569
|
+
at[n].charge ++;
|
570
|
+
at[i].radical = 0;
|
571
|
+
at[n].radical = 0;
|
572
|
+
num_changes ++;
|
573
|
+
num_N_plus --;
|
574
|
+
num_O_minus --;
|
575
|
+
num_All -= 2;
|
576
|
+
}
|
577
|
+
}
|
578
|
+
}
|
579
|
+
}
|
580
|
+
/*-------------------------------------------------------------------------
|
581
|
+
Terminal pair types: 2,3,4,5,6,7,8,9 N=N,P,As,Sb; O=O,S,Se,Te; C=C,Si
|
582
|
+
====================================
|
583
|
+
type #
|
584
|
+
2 2: O=N-C(II)- => O=N#C- N=N,P,As,Sb; O=O,S,Se,Te; C=C,Si
|
585
|
+
3 9: O=O(+)-C(-)(III) => O=O=C(IV)
|
586
|
+
4 3: O(-)-N(+)(IV) => O=N(V) (input structure has at least 1 double bond)
|
587
|
+
5 4: O(-)-O(+)(III) => O=O(IV)
|
588
|
+
6 8: O(-)-O-C(+)(III) => O=O=C(IV)
|
589
|
+
7 5: N(-)=N(+)(IV) => N#N(V) allow terminal H on N(-)
|
590
|
+
8 6: N(-)=O(+)(III) => N#O-
|
591
|
+
9 7: N(-)=C(+)(III) => N#C-
|
592
|
+
--------------------------------------------------------------------------*/
|
593
|
+
if ( !type || 2 <= type && type <= 9 ) {
|
594
|
+
for ( i = 0; i < num_atoms && 0 < num_All; i ++ ) {
|
595
|
+
if ( 0 == at[i].charge && 1 == nNoMetalNumBonds(at, i) && 2 == nNoMetalBondsValence(at, i) &&
|
596
|
+
0 == num_of_H( at, i ) &&
|
597
|
+
NULL != memchr( en+ELEM_O_FST, at[i].el_number, ELEM_O_LEN) &&
|
598
|
+
0 <= ( i1 = nNoMetalNeighIndex(at, i)) &&
|
599
|
+
at[i].bond_type[i1] <= BOND_TYPE_TRIPLE ) {
|
600
|
+
/* terminal O= */
|
601
|
+
n = at[i].neighbor[i1];
|
602
|
+
if ( (!type || type == 2) && 0 < num_C_II ) { /* avoid alternating bonds */
|
603
|
+
if ( 0 == at[n].charge &&
|
604
|
+
2 == nNoMetalNumBonds(at, n) && 3 == nNoMetalBondsValence(at, n) &&
|
605
|
+
0 == num_of_H( at, n ) &&
|
606
|
+
NULL != memchr( en+ELEM_N_FST, at[n].el_number, ELEM_N_LEN) &&
|
607
|
+
0 <= (i2 = nNoMetalOtherNeighIndex( at, n, i ) ) &&
|
608
|
+
at[n].bond_type[i2] <= BOND_TYPE_TRIPLE ) {
|
609
|
+
/* i2 = index of opposite to at[i] neighbor of at[n] */
|
610
|
+
/*i2 = (at[n].neighbor[0] == i);*/
|
611
|
+
n2 = at[n].neighbor[i2];
|
612
|
+
if ( 0 == at[n2].charge &&
|
613
|
+
2 == at[n2].valence && 2 == at[n2].chem_bonds_valence &&
|
614
|
+
0 == num_of_H( at, n2 ) &&
|
615
|
+
NULL != memchr( en+ELEM_C_FST, at[n2].el_number, ELEM_C_LEN) ) {
|
616
|
+
/* i n n2 */
|
617
|
+
/* found O=N-C(II)- */
|
618
|
+
/* convert O=N-C(II)- => O=N#C- */
|
619
|
+
i3 = (at[n2].neighbor[0] != n); /* index of at[n] neighbor of n2 */
|
620
|
+
at[ n].chem_bonds_valence = 5; /* N */
|
621
|
+
at[n2].chem_bonds_valence = 4; /* C */
|
622
|
+
at[ n].bond_type[i2] = BOND_TYPE_TRIPLE;
|
623
|
+
at[n2].bond_type[i3] = BOND_TYPE_TRIPLE;
|
624
|
+
at[n2].radical = 0;
|
625
|
+
num_changes ++;
|
626
|
+
num_C_II --;
|
627
|
+
num_All --;
|
628
|
+
continue;
|
629
|
+
}
|
630
|
+
}
|
631
|
+
}
|
632
|
+
if ( (!type || type == 3) && 0 < num_O_plus && 0 < num_C_minus ) {
|
633
|
+
if ( 1 == at[n].charge && 2 == nNoMetalNumBonds(at, n) && 3 == nNoMetalBondsValence(at, n) &&
|
634
|
+
0 == num_of_H( at, n ) &&
|
635
|
+
NULL != memchr( en+ELEM_O_FST, at[n].el_number, ELEM_O_LEN) &&
|
636
|
+
0 <= (i2 = nNoMetalOtherNeighIndex( at, n, i ) ) &&
|
637
|
+
at[n].bond_type[i2] <= BOND_TYPE_TRIPLE ) {
|
638
|
+
/* found O=O(+)- */
|
639
|
+
/* i2 = index of opposite to at[i] neighbor of at[n] */
|
640
|
+
/*i2 = (at[n].neighbor[0] == i);*/
|
641
|
+
n2 = at[n].neighbor[i2];
|
642
|
+
if ( -1 == at[n2].charge && 3 >= nNoMetalNumBonds(at, n2) && 3 == nNoMetalBondsValence(at, n2)+NUMH(at,n2) &&
|
643
|
+
NULL != memchr( en+ELEM_C_FST, at[n2].el_number, ELEM_C_LEN) ) {
|
644
|
+
/* i n n2 */
|
645
|
+
/* found found O=O(+)-C(-)(III) */
|
646
|
+
/* convert O=O(+)-C(-)(III) => O=O=C(IV) */
|
647
|
+
i3 = (at[n2].neighbor[0] != n); /* index of at[n] neighbor of n2 */
|
648
|
+
at[ n].charge --;
|
649
|
+
at[n2].charge ++;
|
650
|
+
at[ n].chem_bonds_valence += 1; /* =O- => =O= */
|
651
|
+
at[n2].chem_bonds_valence += 1; /* -C => =C */
|
652
|
+
at[ n].bond_type[i2] = BOND_TYPE_DOUBLE;
|
653
|
+
at[n2].bond_type[i3] = BOND_TYPE_DOUBLE;
|
654
|
+
num_changes ++;
|
655
|
+
num_O_plus --;
|
656
|
+
num_C_minus --;
|
657
|
+
num_All -= 2;
|
658
|
+
continue;
|
659
|
+
}
|
660
|
+
}
|
661
|
+
}
|
662
|
+
} else
|
663
|
+
if ( -1 == at[i].charge &&
|
664
|
+
0 < num_O_minus + num_N_minus &&
|
665
|
+
0 < num_N_plus + num_O_plus + num_C_plus &&
|
666
|
+
1 == nNoMetalNumBonds(at, i) && 1 == nNoMetalBondsValence(at, i) &&
|
667
|
+
0 == num_of_H( at, i ) &&
|
668
|
+
NULL != memchr( en+ELEM_O_FST, at[i].el_number, ELEM_O_LEN) &&
|
669
|
+
0 <= (i1 = nNoMetalNeighIndex( at, i )) &&
|
670
|
+
at[i].bond_type[i1] <= BOND_TYPE_TRIPLE ) {
|
671
|
+
|
672
|
+
/* terminal O(-)- */
|
673
|
+
|
674
|
+
n = at[i].neighbor[i1];
|
675
|
+
|
676
|
+
if ( (!type || type == 4) && 0 < num_O_minus && 0 < num_N_plus && /* O(-)-N(+)(IV) */
|
677
|
+
1 == at[n].charge && 3 >= nNoMetalNumBonds(at, n) && 4 == nNoMetalBondsValence(at, n) &&
|
678
|
+
0 == num_of_H( at, n ) &&
|
679
|
+
NULL != memchr( en+ELEM_N_FST, at[n].el_number, ELEM_N_LEN) /* except >O(+)- */
|
680
|
+
) {
|
681
|
+
/* found O(-)-N(+)(IV) */
|
682
|
+
/* convert O(-)-N(+)(IV) => O=N(V) */
|
683
|
+
|
684
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor; /* index of at[i] neighbor of at[n] */
|
685
|
+
at[i].charge ++;
|
686
|
+
at[n].charge --;
|
687
|
+
at[i].chem_bonds_valence ++;
|
688
|
+
at[n].chem_bonds_valence ++;
|
689
|
+
at[i].bond_type[i1] ++;
|
690
|
+
at[n].bond_type[i2] ++;
|
691
|
+
num_changes ++;
|
692
|
+
num_O_minus --;
|
693
|
+
num_N_plus --;
|
694
|
+
num_All -= 2;
|
695
|
+
continue;
|
696
|
+
}
|
697
|
+
|
698
|
+
if ( (!type || type == 5) && 0 < num_O_minus && 0 < num_O_plus &&/* O(-)-O(+)(III) */
|
699
|
+
1 == at[n].charge && 3 >= nNoMetalNumBonds(at, n) && 3 == nNoMetalBondsValence(at, n) &&
|
700
|
+
0 == num_of_H( at, n ) &&
|
701
|
+
NULL != memchr( en+ELEM_O_FST, at[n].el_number, ELEM_O_LEN) /* except >O(+)- */
|
702
|
+
) {
|
703
|
+
/* found O(+)(III) */
|
704
|
+
/* convert O(-)-O(+)(III) => O=O(IV) */
|
705
|
+
|
706
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor; /* index of at[i] neighbor of at[n] */
|
707
|
+
at[i].charge ++;
|
708
|
+
at[n].charge --;
|
709
|
+
at[i].chem_bonds_valence ++;
|
710
|
+
at[n].chem_bonds_valence ++;
|
711
|
+
at[i].bond_type[i1] ++;
|
712
|
+
at[n].bond_type[i2] ++;
|
713
|
+
num_changes ++;
|
714
|
+
num_O_minus --;
|
715
|
+
num_O_plus --;
|
716
|
+
num_All -= 2;
|
717
|
+
continue;
|
718
|
+
}
|
719
|
+
/* i n n2 */
|
720
|
+
if ( (!type || type == 6) && /* O(-)-O-C(+)(III) */
|
721
|
+
0 < num_O_minus && 0 < num_C_plus &&
|
722
|
+
0 == at[n].charge && 2 == nNoMetalNumBonds(at, n) && 2 == nNoMetalBondsValence(at, n) &&
|
723
|
+
0 == num_of_H( at, n ) &&
|
724
|
+
NULL != memchr( en+ELEM_O_FST, at[n].el_number, ELEM_O_LEN) &&
|
725
|
+
0 <= (i2=nNoMetalOtherNeighIndex( at, n, i )) &&
|
726
|
+
at[n].bond_type[i2] <= BOND_TYPE_TRIPLE ) {
|
727
|
+
/* found O(-)-O- */
|
728
|
+
/* i2 = index of opposite to at[i] neighbor of at[n] */
|
729
|
+
/*i2 = (at[n].neighbor[0] == i);*/
|
730
|
+
n2 = at[n].neighbor[i2];
|
731
|
+
if ( 1 == at[n2].charge && 3 >= nNoMetalNumBonds(at, n2) &&
|
732
|
+
3 == nNoMetalBondsValence(at, n2)+NUMH(at,n2) &&
|
733
|
+
NULL != memchr( en+ELEM_C_FST, at[n2].el_number, ELEM_C_LEN) ) {
|
734
|
+
/* i n n2 */
|
735
|
+
/* found O(-)-O-C(+)(III) */
|
736
|
+
/* convert O(-)-O-C(+)(III) => O=O=C(IV) */
|
737
|
+
/*i3 = (at[n2].neighbor[0] != n);*/ /* i3 = index of at[n] neighbor of at[n2] */
|
738
|
+
i3 = is_in_the_list( at[n2].neighbor, (AT_NUMB)n, at[n2].valence ) - at[n2].neighbor;
|
739
|
+
/*i4 = index of at[i] in the adjacency list of at[n] */
|
740
|
+
i4 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor;
|
741
|
+
at[ i].charge ++;
|
742
|
+
at[n2].charge --;
|
743
|
+
at[ i].chem_bonds_valence += 1; /* O- => O= */
|
744
|
+
at[ n].chem_bonds_valence += 2; /* -O- => =O= */
|
745
|
+
at[n2].chem_bonds_valence += 1; /* -C => =C */
|
746
|
+
at[ i].bond_type[i1] = BOND_TYPE_DOUBLE;
|
747
|
+
at[ n].bond_type[i4] = BOND_TYPE_DOUBLE;
|
748
|
+
at[ n].bond_type[i2] = BOND_TYPE_DOUBLE;
|
749
|
+
at[n2].bond_type[i3] = BOND_TYPE_DOUBLE;
|
750
|
+
num_changes ++;
|
751
|
+
num_O_minus --;
|
752
|
+
num_C_plus --;
|
753
|
+
num_All -= 2;
|
754
|
+
continue;
|
755
|
+
}
|
756
|
+
}
|
757
|
+
} else
|
758
|
+
if ( -1 == at[i].charge && 0 < num_N_minus && 0 < num_N_plus+num_O_plus+num_C_plus &&
|
759
|
+
1 == nNoMetalNumBonds(at, i) && 2 == nNoMetalBondsValence(at, i)+NUMH(at, i) &&
|
760
|
+
/*0 == num_of_H( at, i ) &&*/
|
761
|
+
NULL != memchr( en+ELEM_N_FST, at[i].el_number, ELEM_N_LEN) &&
|
762
|
+
0 <= (i1 = nNoMetalNeighIndex( at, i )) &&
|
763
|
+
at[i].bond_type[i1] <= BOND_TYPE_TRIPLE ) {
|
764
|
+
/* terminal N(-)= */
|
765
|
+
n = at[i].neighbor[i1 = 0];
|
766
|
+
if ( (!type || type == 7) && 0 < num_N_plus && /* N(-)=N(+)(IV) */
|
767
|
+
1 == at[n].charge && 3 >= nNoMetalNumBonds(at, n) && 4 == nNoMetalBondsValence(at, n) &&
|
768
|
+
0 == num_of_H( at, n ) &&
|
769
|
+
NULL != memchr( en+ELEM_N_FST, at[n].el_number, ELEM_N_LEN)
|
770
|
+
) {
|
771
|
+
/* found N(-)-N(+)(IV) */
|
772
|
+
/* convert N(-)=N(+)(IV) => N#N(V) */
|
773
|
+
|
774
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor; /* index of at[i] neighbor of at[n] */
|
775
|
+
at[i].charge ++;
|
776
|
+
at[n].charge --;
|
777
|
+
at[i].chem_bonds_valence ++;
|
778
|
+
at[n].chem_bonds_valence ++;
|
779
|
+
at[i].bond_type[i1] ++;
|
780
|
+
at[n].bond_type[i2] ++;
|
781
|
+
num_changes ++;
|
782
|
+
num_N_minus --;
|
783
|
+
num_N_plus --;
|
784
|
+
num_All -= 2;
|
785
|
+
continue;
|
786
|
+
}
|
787
|
+
if ( (!type || type == 8) && 0 < num_O_plus && /* N(-)=O(+)(III) */
|
788
|
+
1 == at[n].charge && 2 == nNoMetalNumBonds(at, n) && 3 == nNoMetalBondsValence(at, n) &&
|
789
|
+
0 == num_of_H( at, n ) &&
|
790
|
+
NULL != memchr( en+ELEM_O_FST, at[n].el_number, ELEM_O_LEN)
|
791
|
+
) {
|
792
|
+
/* found N(-)-O(+)(III) */
|
793
|
+
/* convert N(-)=O(+)(III) => N#O(IV)- */
|
794
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor; /* index of at[i] neighbor of at[n] */
|
795
|
+
at[i].charge ++;
|
796
|
+
at[n].charge --;
|
797
|
+
at[i].chem_bonds_valence ++;
|
798
|
+
at[n].chem_bonds_valence ++;
|
799
|
+
at[i].bond_type[i1] ++;
|
800
|
+
at[n].bond_type[i2] ++;
|
801
|
+
num_changes ++;
|
802
|
+
num_N_minus --;
|
803
|
+
num_O_plus --;
|
804
|
+
num_All -= 2;
|
805
|
+
continue;
|
806
|
+
}
|
807
|
+
if ( (!type || type == 9) && 0 < num_C_plus && /* N(-)=C(+)(III) */
|
808
|
+
1 == at[n].charge && 2 == at[n].valence && 3 == at[n].chem_bonds_valence &&
|
809
|
+
0 == num_of_H( at, n ) &&
|
810
|
+
NULL != memchr( en+ELEM_C_FST, at[n].el_number, ELEM_C_LEN)
|
811
|
+
) {
|
812
|
+
/* found N(-)=C(+)(III) */
|
813
|
+
/* convert N(-)=C(+)(III) => N#C(IV)- */
|
814
|
+
|
815
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor; /* index of at[i] neighbor of at[n] */
|
816
|
+
at[i].charge ++;
|
817
|
+
at[n].charge --;
|
818
|
+
at[i].chem_bonds_valence ++;
|
819
|
+
at[n].chem_bonds_valence ++;
|
820
|
+
at[i].bond_type[i1] ++;
|
821
|
+
at[n].bond_type[i2] ++;
|
822
|
+
num_changes ++;
|
823
|
+
num_N_minus --;
|
824
|
+
num_C_plus --;
|
825
|
+
num_All -= 2;
|
826
|
+
continue;
|
827
|
+
}
|
828
|
+
}
|
829
|
+
}
|
830
|
+
}
|
831
|
+
|
832
|
+
/**************************************************************************/
|
833
|
+
/*********************** NON-Terminal ion pairs ***************************/
|
834
|
+
/**************************************************************************/
|
835
|
+
/*-------------------------------------------------------------------------
|
836
|
+
Non-Terminal pair types: 10,11,12,13,14 N=N,P,As,Sb; O=O,S,Se,Te; C=C,Si
|
837
|
+
========================================
|
838
|
+
|
839
|
+
10: N(+)(IV)-C(-)(III) => N(V)=C(IV) (N has 3 or 2 bonds)
|
840
|
+
11: N(+)(IV)=C(-)(III) => N(V)#C(IV) (N has 3 or 2 bonds)
|
841
|
+
12: N(+)(IV)-N(-)(II) => N(V)=N(III) (allow terminal H on N(-))
|
842
|
+
13: -O(+)-C(-)(III) => -O=C-
|
843
|
+
14: -O(+)=C(-)(III) => -O#C-
|
844
|
+
15: O(+)(III)-N(-)(II) => O(IV)=N(III) (allow terminal H on N(-))
|
845
|
+
--------------------------------------------------------------------------*/
|
846
|
+
if ( !type || 10 <= type && type <= 15 ) {
|
847
|
+
for ( i = 0; i < num_atoms && 0 < num_All; i ++ ) {
|
848
|
+
if ( 1 == at[i].charge &&
|
849
|
+
0 < num_N_plus + num_O_plus && 0 < num_C_minus + num_N_minus &&
|
850
|
+
4 >= nNoMetalNumBonds(at, i) && 4 == nNoMetalBondsValence(at, i) &&
|
851
|
+
0 == num_of_H( at, i ) &&
|
852
|
+
NULL != memchr( en+ELEM_N_FST, at[i].el_number, ELEM_N_LEN) ) {
|
853
|
+
/* found non-terminal N(+)(IV) */
|
854
|
+
if ( (!type || 10 == type) && 0 < num_N_plus && 0 < num_C_minus ) {
|
855
|
+
int num_neigh = 0, pos_neigh = -1;
|
856
|
+
for ( i1 = 0; i1 < at[i].valence; i1 ++ ) {
|
857
|
+
n = at[i].neighbor[i1];
|
858
|
+
if ( -1 == at[n].charge && 3 >= at[n].valence && 3 == at[n].chem_bonds_valence+NUMH(at,n) &&
|
859
|
+
/*0 == at[n].num_H &&*/
|
860
|
+
at[i].bond_type[i1] == BOND_TYPE_SINGLE &&
|
861
|
+
NULL != memchr( en+ELEM_C_FST, at[n].el_number, ELEM_C_LEN) ) {
|
862
|
+
/* found N(+)(IV)-C(-)(III); prepare conversion to N(V)=C(IV) */
|
863
|
+
num_neigh ++;
|
864
|
+
pos_neigh = i1;
|
865
|
+
}
|
866
|
+
}
|
867
|
+
i1=pos_neigh;
|
868
|
+
if ( 1 == num_neigh &&
|
869
|
+
at[i].bond_type[i1] <= BOND_TYPE_TRIPLE &&
|
870
|
+
!has_other_ion_neigh( at, i, n=at[i].neighbor[i1], en, ne ) &&
|
871
|
+
!has_other_ion_neigh( at, n, i, en, ne )) {
|
872
|
+
/*n = at[i].neighbor[i1=pos_neigh];*/
|
873
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor;
|
874
|
+
at[i].charge --;
|
875
|
+
at[n].charge ++;
|
876
|
+
at[i].chem_bonds_valence ++;
|
877
|
+
at[n].chem_bonds_valence ++;
|
878
|
+
at[i].bond_type[i1] ++;
|
879
|
+
at[n].bond_type[i2] ++;
|
880
|
+
num_changes ++;
|
881
|
+
num_C_minus --;
|
882
|
+
num_N_plus --;
|
883
|
+
num_All -= 2;
|
884
|
+
continue;
|
885
|
+
}
|
886
|
+
}
|
887
|
+
if ( (!type || 11 == type) && 0 < num_N_plus && 0 < num_C_minus ) {
|
888
|
+
int num_neigh = 0, pos_neigh = -1;
|
889
|
+
for ( i1 = 0; i1 < at[i].valence; i1 ++ ) {
|
890
|
+
n = at[i].neighbor[i1];
|
891
|
+
if ( -1 == at[n].charge && 3 >= at[n].valence && 3 == at[n].chem_bonds_valence+NUMH(at,n) &&
|
892
|
+
/*0 == at[n].num_H &&*/
|
893
|
+
at[i].bond_type[i1] == BOND_TYPE_DOUBLE &&
|
894
|
+
NULL != memchr( en+ELEM_C_FST, at[n].el_number, ELEM_C_LEN) ) {
|
895
|
+
/* found N(+)(IV)=C(-)(III); prepare conversion to N(V)#C(IV) */
|
896
|
+
num_neigh ++;
|
897
|
+
pos_neigh = i1;
|
898
|
+
}
|
899
|
+
}
|
900
|
+
if ( 1 == num_neigh &&
|
901
|
+
!has_other_ion_neigh( at, i, n=at[i].neighbor[i1=pos_neigh], en, ne ) &&
|
902
|
+
!has_other_ion_neigh( at, n, i, en, ne )) {
|
903
|
+
/*n = at[i].neighbor[i1=pos_neigh];*/
|
904
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor;
|
905
|
+
at[i].charge --;
|
906
|
+
at[n].charge ++;
|
907
|
+
at[i].chem_bonds_valence ++;
|
908
|
+
at[n].chem_bonds_valence ++;
|
909
|
+
at[i].bond_type[i1] ++;
|
910
|
+
at[n].bond_type[i2] ++;
|
911
|
+
num_changes ++;
|
912
|
+
num_C_minus --;
|
913
|
+
num_N_plus --;
|
914
|
+
num_All -= 2;
|
915
|
+
continue;
|
916
|
+
}
|
917
|
+
}
|
918
|
+
if ( !type || 12 == type && 0 < num_N_plus && 0 < num_N_minus ) {
|
919
|
+
int num_neigh = 0, pos_neigh = -1;
|
920
|
+
for ( i1 = 0; i1 < at[i].valence; i1 ++ ) {
|
921
|
+
n = at[i].neighbor[i1];
|
922
|
+
if ( -1 == at[n].charge && 2 >= nNoMetalNumBonds(at, n) &&
|
923
|
+
2 == nNoMetalBondsValence(at, n)+NUMH(at, n) &&
|
924
|
+
/*0 == num_of_H( at, n ) &&*/
|
925
|
+
at[i].bond_type[i1] == BOND_TYPE_SINGLE &&
|
926
|
+
NULL != memchr( en+ELEM_N_FST, at[n].el_number, ELEM_N_LEN) ) {
|
927
|
+
/* found N(+)(IV)=N(-)(II); prepare conversion to N(V)#N(III) */
|
928
|
+
num_neigh ++;
|
929
|
+
pos_neigh = i1;
|
930
|
+
}
|
931
|
+
}
|
932
|
+
if ( 1 == num_neigh &&
|
933
|
+
!has_other_ion_neigh( at, i, n=at[i].neighbor[i1=pos_neigh], en, ne ) &&
|
934
|
+
!has_other_ion_neigh( at, n, i, en, ne )) {
|
935
|
+
/*n = at[i].neighbor[i1=pos_neigh];*/
|
936
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor;
|
937
|
+
at[i].charge --;
|
938
|
+
at[n].charge ++;
|
939
|
+
at[i].chem_bonds_valence ++;
|
940
|
+
at[n].chem_bonds_valence ++;
|
941
|
+
at[i].bond_type[i1] ++;
|
942
|
+
at[n].bond_type[i2] ++;
|
943
|
+
num_changes ++;
|
944
|
+
num_N_minus --;
|
945
|
+
num_N_plus --;
|
946
|
+
num_All -= 2;
|
947
|
+
continue;
|
948
|
+
}
|
949
|
+
}
|
950
|
+
} else
|
951
|
+
if ( 1 == at[i].charge &&
|
952
|
+
0 < num_O_plus && 0 < num_C_minus + num_N_minus &&
|
953
|
+
3 >= nNoMetalNumBonds(at, i) && 3 == nNoMetalBondsValence(at, i) &&
|
954
|
+
0 == num_of_H( at, i ) &&
|
955
|
+
NULL != memchr( en+ELEM_O_FST, at[i].el_number, ELEM_O_LEN) ) {
|
956
|
+
/* found non-terminal O(+)(III) */
|
957
|
+
if ( (!type || 13 == type) && 0 < num_C_minus ) {
|
958
|
+
int num_neigh = 0, pos_neigh = -1;
|
959
|
+
for ( i1 = 0; i1 < at[i].valence; i1 ++ ) {
|
960
|
+
n = at[i].neighbor[i1];
|
961
|
+
if ( -1 == at[n].charge && 3 >= at[n].valence && 3 == at[n].chem_bonds_valence+NUMH(at,n) &&
|
962
|
+
/*0 == at[n].num_H &&*/
|
963
|
+
at[i].bond_type[i1] == BOND_TYPE_SINGLE &&
|
964
|
+
NULL != memchr( en+ELEM_C_FST, at[n].el_number, ELEM_C_LEN) ) {
|
965
|
+
/* found O(+)(III)-C(-)(II); prepare conversion to O(IV)=C(IV) */
|
966
|
+
num_neigh ++;
|
967
|
+
pos_neigh = i1;
|
968
|
+
}
|
969
|
+
}
|
970
|
+
if ( 1 == num_neigh &&
|
971
|
+
!has_other_ion_neigh( at, i, n=at[i].neighbor[i1=pos_neigh], en, ne ) &&
|
972
|
+
!has_other_ion_neigh( at, n, i, en, ne )) {
|
973
|
+
/*n = at[i].neighbor[i1=pos_neigh];*/
|
974
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor;
|
975
|
+
at[i].charge --;
|
976
|
+
at[n].charge ++;
|
977
|
+
at[i].chem_bonds_valence ++;
|
978
|
+
at[n].chem_bonds_valence ++;
|
979
|
+
at[i].bond_type[i1] ++;
|
980
|
+
at[n].bond_type[i2] ++;
|
981
|
+
num_changes ++;
|
982
|
+
num_C_minus --;
|
983
|
+
num_O_plus --;
|
984
|
+
num_All -= 2;
|
985
|
+
continue;
|
986
|
+
}
|
987
|
+
}
|
988
|
+
if ( (!type || 14 == type) && 0 < num_C_minus ) {
|
989
|
+
int num_neigh = 0, pos_neigh = -1;
|
990
|
+
for ( i1 = 0; i1 < at[i].valence; i1 ++ ) {
|
991
|
+
n = at[i].neighbor[i1];
|
992
|
+
if ( -1 == at[n].charge && 3 >= at[n].valence && 3 == at[n].chem_bonds_valence+NUMH(at,n) &&
|
993
|
+
/*0 == at[n].num_H &&*/
|
994
|
+
at[i].bond_type[i1] == BOND_TYPE_DOUBLE &&
|
995
|
+
NULL != memchr( en+ELEM_C_FST, at[n].el_number, ELEM_C_LEN) ) {
|
996
|
+
/* found O(+)(III)=C(-)(III); prepare conversion to O(IV)#C(IV) */
|
997
|
+
num_neigh ++;
|
998
|
+
pos_neigh = i1;
|
999
|
+
}
|
1000
|
+
}
|
1001
|
+
if ( 1 == num_neigh &&
|
1002
|
+
!has_other_ion_neigh( at, i, n=at[i].neighbor[i1=pos_neigh], en, ne ) &&
|
1003
|
+
!has_other_ion_neigh( at, n, i, en, ne )) {
|
1004
|
+
/*n = at[i].neighbor[i1=pos_neigh];*/
|
1005
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor;
|
1006
|
+
at[i].charge --;
|
1007
|
+
at[n].charge ++;
|
1008
|
+
at[i].chem_bonds_valence ++;
|
1009
|
+
at[n].chem_bonds_valence ++;
|
1010
|
+
at[i].bond_type[i1] ++;
|
1011
|
+
at[n].bond_type[i2] ++;
|
1012
|
+
num_changes ++;
|
1013
|
+
num_C_minus --;
|
1014
|
+
num_O_plus --;
|
1015
|
+
num_All -= 2;
|
1016
|
+
continue;
|
1017
|
+
}
|
1018
|
+
}
|
1019
|
+
if ( (!type || 15 == type) && 0 < num_N_minus ) {
|
1020
|
+
int num_neigh = 0, pos_neigh = -1;
|
1021
|
+
for ( i1 = 0; i1 < at[i].valence; i1 ++ ) {
|
1022
|
+
n = at[i].neighbor[i1];
|
1023
|
+
if ( -1 == at[n].charge && 2 >= nNoMetalNumBonds(at, n) &&
|
1024
|
+
2 == nNoMetalBondsValence(at, n)+NUMH(at, n) &&
|
1025
|
+
/*0 == num_of_H( at, n ) &&*/
|
1026
|
+
at[i].bond_type[i1] == BOND_TYPE_SINGLE &&
|
1027
|
+
NULL != memchr( en+ELEM_N_FST, at[n].el_number, ELEM_N_LEN) ) {
|
1028
|
+
/* found O(+)(III)=N(-)(II); prepare conversion to O(IV)#N(III) */
|
1029
|
+
num_neigh ++;
|
1030
|
+
pos_neigh = i1;
|
1031
|
+
}
|
1032
|
+
}
|
1033
|
+
if ( 1 == num_neigh &&
|
1034
|
+
!has_other_ion_neigh( at, i, n=at[i].neighbor[i1=pos_neigh], en, ne ) &&
|
1035
|
+
!has_other_ion_neigh( at, n, i, en, ne )) {
|
1036
|
+
/*n = at[i].neighbor[i1=pos_neigh];*/
|
1037
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor;
|
1038
|
+
at[i].charge --;
|
1039
|
+
at[n].charge ++;
|
1040
|
+
at[i].chem_bonds_valence ++;
|
1041
|
+
at[n].chem_bonds_valence ++;
|
1042
|
+
at[i].bond_type[i1] ++;
|
1043
|
+
at[n].bond_type[i2] ++;
|
1044
|
+
num_changes ++;
|
1045
|
+
num_N_minus --;
|
1046
|
+
num_O_plus --;
|
1047
|
+
num_All -= 2;
|
1048
|
+
continue;
|
1049
|
+
}
|
1050
|
+
}
|
1051
|
+
}
|
1052
|
+
}
|
1053
|
+
}
|
1054
|
+
/**************************************************************************/
|
1055
|
+
/*********************** NON-Terminal ion triples *************************/
|
1056
|
+
/**************************************************************************/
|
1057
|
+
/*-------------------------------------------------------------------------
|
1058
|
+
Non-Terminal triple types: 16, 17, 18 N=N,P,As,Sb; O=O,S,Se,Te; C=C,Si
|
1059
|
+
========================================
|
1060
|
+
16: C(+)(III)-O-N(-)(II) => C(IV)=O=N(III) (allow terminal H on N(-))
|
1061
|
+
|
1062
|
+
| |
|
1063
|
+
17: C(+)(III)-N-C(-)(III) => C(IV)=N=C(IV)
|
1064
|
+
|
1065
|
+
18: C(-)(III)-N=C(+)(III) => C(IV)=N#C(IV) (may have two or no charges)
|
1066
|
+
C(IV)=N-C(II) => C(IV)=N#C(IV)
|
1067
|
+
|
1068
|
+
*/
|
1069
|
+
if ( (!type || 16 == type) && 0 < num_C_plus && 0 < num_N_minus ) {
|
1070
|
+
int m[2], j[2], k;
|
1071
|
+
for ( i = 0; i < num_atoms; i ++ ) {
|
1072
|
+
if ( 0 == at[i].charge && 2 == nNoMetalNumBonds(at, i) && 2 == nNoMetalBondsValence(at, i) &&
|
1073
|
+
0 == num_of_H( at, i ) &&
|
1074
|
+
0 <= (j[0] = nNoMetalNeighIndex( at, i )) &&
|
1075
|
+
at[m[0]=at[i].neighbor[j[0]]].charge &&
|
1076
|
+
0 <= (j[1] = nNoMetalOtherNeighIndex( at, i, m[0] )) &&
|
1077
|
+
0 == at[m[0]].charge + at[m[1]=at[i].neighbor[j[1]]].charge &&
|
1078
|
+
5 >= nNoMetalBondsValence(at, m[0]) + nNoMetalBondsValence(at, m[1]) &&
|
1079
|
+
/*5 >= at[m[0]].chem_bonds_valence + at[m[1]].chem_bonds_valence &&*/
|
1080
|
+
NULL != memchr( en+ELEM_O_FST, at[i].el_number, ELEM_O_LEN) ) {
|
1081
|
+
/* found non-terminal A(+)-O-B(-); chem_bond_val of A+B <= 5 */
|
1082
|
+
int n_N=-1, n_C=-1, i_C=-1;
|
1083
|
+
for ( k = 0; k < 2; k ++ ) {
|
1084
|
+
n = m[k];
|
1085
|
+
if ( -1 == at[n].charge && 2 == nNoMetalNumBonds(at, n)+NUMH(at, n) &&
|
1086
|
+
/*0 == num_of_H( at, n ) &&*/
|
1087
|
+
NULL != memchr( en+ELEM_N_FST, at[n].el_number, ELEM_N_LEN) ) {
|
1088
|
+
n_N = n;
|
1089
|
+
} else
|
1090
|
+
if ( 1 == at[n].charge && 3 == at[n].chem_bonds_valence+NUMH(at,n) &&
|
1091
|
+
NULL != memchr( en+ELEM_C_FST, at[n].el_number, ELEM_C_LEN) ) {
|
1092
|
+
n_C = n;
|
1093
|
+
i_C = k;
|
1094
|
+
}
|
1095
|
+
}
|
1096
|
+
if ( n_C < 0 || n_N < 0 ||
|
1097
|
+
has_other_ion_in_sphere_2(at, n_C, n_N, en, ne ) ||
|
1098
|
+
has_other_ion_in_sphere_2(at, n_N, n_C, en, ne ) ) {
|
1099
|
+
continue;
|
1100
|
+
}
|
1101
|
+
/* C(+)(III)-O-N(-)(II) => C(IV)=O=N(III) */
|
1102
|
+
for ( k = 0; k < 2; k ++ ) {
|
1103
|
+
n = k? n_C : n_N;
|
1104
|
+
i1 = k? j[i_C] : j[1-i_C];
|
1105
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor;
|
1106
|
+
at[i].bond_type[i1] ++;
|
1107
|
+
at[n].bond_type[i2] ++;
|
1108
|
+
at[i].chem_bonds_valence ++;
|
1109
|
+
at[n].chem_bonds_valence ++;
|
1110
|
+
at[n].charge += (k? -1:1);
|
1111
|
+
}
|
1112
|
+
num_changes ++;
|
1113
|
+
num_N_minus --;
|
1114
|
+
num_C_plus --;
|
1115
|
+
num_All -= 2;
|
1116
|
+
}
|
1117
|
+
}
|
1118
|
+
}
|
1119
|
+
if ( (!type || 17 == type) && 0 < num_C_plus && 0 < num_C_minus ) {
|
1120
|
+
int m[3], c[3], j[3], k;
|
1121
|
+
for ( i = 0; i < num_atoms; i ++ ) {
|
1122
|
+
if ( 0 == at[i].charge && 3 == nNoMetalNumBonds(at, i) && 3 == nNoMetalBondsValence(at, i) &&
|
1123
|
+
0 == num_of_H( at, i ) &&
|
1124
|
+
0 <= ( j[0] = nNoMetalNeighIndex(at, i) ) &&
|
1125
|
+
0 <= ( j[1] = nNoMetalOtherNeighIndex( at, i, m[0] = at[i].neighbor[j[0]] ) ) &&
|
1126
|
+
0 <= ( j[2] = nNoMetalOtherNeighIndex2( at, i, m[0], m[1] = at[i].neighbor[j[1]] ) ) &&
|
1127
|
+
1 == !(c[0]=at[m[0]].charge)
|
1128
|
+
+ !(c[1]=at[m[1]].charge)
|
1129
|
+
+ !(c[2]=at[m[2]=at[i].neighbor[j[2]]].charge) &&
|
1130
|
+
0 == c[0] + c[1] + c[2] &&
|
1131
|
+
2 == (3== (c[0]? at[m[0]].chem_bonds_valence+NUMH(at,m[0]):0))
|
1132
|
+
+ (3== (c[1]? at[m[1]].chem_bonds_valence+NUMH(at,m[1]):0))
|
1133
|
+
+ (3== (c[2]? at[m[2]].chem_bonds_valence+NUMH(at,m[2]):0)) &&
|
1134
|
+
NULL != memchr( en+ELEM_N_FST, at[i].el_number, ELEM_N_LEN) ) {
|
1135
|
+
/* found non-terminal A(+)-O-B(-) */
|
1136
|
+
int n_Cp=-1, n_Cm=-1, i_Cp=-1, i_Cm=-1; /* p = positive, m = negatice ion C */
|
1137
|
+
for ( k = 0; k < 3; k ++ ) {
|
1138
|
+
if ( c[k] ) {
|
1139
|
+
n = m[k];
|
1140
|
+
if ( -1 == at[n].charge &&
|
1141
|
+
NULL != memchr( en+ELEM_C_FST, at[n].el_number, ELEM_C_LEN) ) {
|
1142
|
+
n_Cm = n;
|
1143
|
+
i_Cm = k;
|
1144
|
+
} else
|
1145
|
+
if ( 1 == at[n].charge &&
|
1146
|
+
NULL != memchr( en+ELEM_C_FST, at[n].el_number, ELEM_C_LEN) ) {
|
1147
|
+
n_Cp = n;
|
1148
|
+
i_Cp = k;
|
1149
|
+
}
|
1150
|
+
}
|
1151
|
+
}
|
1152
|
+
if ( n_Cp < 0 || n_Cm < 0 ||
|
1153
|
+
has_other_ion_in_sphere_2(at, n_Cp, n_Cm, en, ne ) ||
|
1154
|
+
has_other_ion_in_sphere_2(at, n_Cm, n_Cp, en, ne )) {
|
1155
|
+
continue;
|
1156
|
+
}
|
1157
|
+
/* | | */
|
1158
|
+
/* C(+)(III)-N-C(-)(III) => C(IV)=N=C(IV) */
|
1159
|
+
for ( k = 0; k < 2; k ++ ) {
|
1160
|
+
n = k? n_Cp : n_Cm;
|
1161
|
+
i1 = k? j[i_Cp] : j[i_Cm];
|
1162
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor;
|
1163
|
+
at[i].bond_type[i1] ++;
|
1164
|
+
at[n].bond_type[i2] ++;
|
1165
|
+
at[i].chem_bonds_valence ++;
|
1166
|
+
at[n].chem_bonds_valence ++;
|
1167
|
+
at[n].charge += (k? -1:1);
|
1168
|
+
}
|
1169
|
+
num_changes ++;
|
1170
|
+
num_C_minus --;
|
1171
|
+
num_C_plus --;
|
1172
|
+
num_All -= 2;
|
1173
|
+
}
|
1174
|
+
}
|
1175
|
+
}
|
1176
|
+
if ( (!type || 18 == type) && (0 < num_C_plus && 0 < num_C_minus || 0 < num_C_II) ) {
|
1177
|
+
int m[2], v[2], j[2], k;
|
1178
|
+
for ( i = 0; i < num_atoms; i ++ ) {
|
1179
|
+
if ( 0 == at[i].charge && 2 == nNoMetalNumBonds(at, i) && 3 == nNoMetalBondsValence(at, i) &&
|
1180
|
+
0 == num_of_H( at, i ) &&
|
1181
|
+
0 <= (j[0] = nNoMetalNeighIndex( at, i )) &&
|
1182
|
+
0 <= (j[1] = nNoMetalOtherNeighIndex( at, i, m[0] = at[i].neighbor[j[0]] )) &&
|
1183
|
+
0 == at[m[0]].charge
|
1184
|
+
+at[m[1]=at[i].neighbor[j[1]]].charge &&
|
1185
|
+
6 == (v[0]=at[m[0]].chem_bonds_valence+NUMH(at,m[0]))
|
1186
|
+
+(v[1]=at[m[1]].chem_bonds_valence+NUMH(at,m[1])) &&
|
1187
|
+
2 >= abs(v[0]-v[1]) &&
|
1188
|
+
NULL != memchr( en+ELEM_N_FST, at[i].el_number, ELEM_N_LEN) &&
|
1189
|
+
NULL != memchr( en+ELEM_C_FST, at[m[0]].el_number, ELEM_C_LEN) &&
|
1190
|
+
NULL != memchr( en+ELEM_C_FST, at[m[1]].el_number, ELEM_C_LEN)
|
1191
|
+
) {
|
1192
|
+
/* n_Cm i n_Cp */
|
1193
|
+
/* found non-terminal C(-)(III)-N=C(+)(III) or C(IV)=N-C(II): Cm-N-Cp */
|
1194
|
+
/* convert to C(IV)=N#C(IV) */
|
1195
|
+
int n_Cp=-1, n_Cm=-1, i_Cp=-1, i_Cm=-1; /* p = positive, m = negatice ion C */
|
1196
|
+
for ( k = 0; k < 2; k ++ ) {
|
1197
|
+
n = m[k];
|
1198
|
+
if ( v[k] == 4 || v[k] == 3 && at[i].bond_type[j[k]] == BOND_TYPE_SINGLE ) {
|
1199
|
+
n_Cm = n;
|
1200
|
+
i_Cm = k;
|
1201
|
+
} else
|
1202
|
+
if ( v[k] == 2 || v[k] == 3 && at[i].bond_type[j[k]] == BOND_TYPE_DOUBLE ) {
|
1203
|
+
n_Cp = n;
|
1204
|
+
i_Cp = k;
|
1205
|
+
}
|
1206
|
+
}
|
1207
|
+
if ( n_Cp < 0 || n_Cm < 0 || at[n_Cp].valence+NUMH(at,n_Cp) != 2 ) {
|
1208
|
+
continue; /* guarantees at[n_Cp].valence <= 2 */
|
1209
|
+
}
|
1210
|
+
if ( v[i_Cp] == 2 || !at[n_Cp].charge ) {
|
1211
|
+
if ( at[n_Cp].valence == 2 ) {
|
1212
|
+
/* neighbor of at[n_Cp] opposite to at[i] */
|
1213
|
+
k = at[n_Cp].neighbor[at[n_Cp].neighbor[0]==i];
|
1214
|
+
if ( NULL != memchr( en+ELEM_N_FST, at[k].el_number, ELEM_N_LEN) ) {
|
1215
|
+
continue;
|
1216
|
+
}
|
1217
|
+
}
|
1218
|
+
} else
|
1219
|
+
if ( at[n_Cp].charge ) {
|
1220
|
+
if ( has_other_ion_in_sphere_2(at, n_Cp, n_Cm, en, ne ) ||
|
1221
|
+
has_other_ion_in_sphere_2(at, n_Cm, n_Cp, en, ne )) {
|
1222
|
+
continue;
|
1223
|
+
}
|
1224
|
+
} else {
|
1225
|
+
continue; /* unknown case */
|
1226
|
+
}
|
1227
|
+
/* */
|
1228
|
+
/* C(-)(III)-N=C(+)(III) => C(IV)=N#C(IV) */
|
1229
|
+
/* C(IV)=N-C(II) => C(IV)=N#C(IV) */
|
1230
|
+
if ( at[n_Cp].charge ) {
|
1231
|
+
num_C_minus --;
|
1232
|
+
num_C_plus --;
|
1233
|
+
num_All -= 2;
|
1234
|
+
} else {
|
1235
|
+
num_C_II --;
|
1236
|
+
num_All --;
|
1237
|
+
}
|
1238
|
+
|
1239
|
+
for ( k = 0; k < 2; k ++ ) {
|
1240
|
+
n = k? n_Cp : n_Cm;
|
1241
|
+
i1 = k? j[i_Cp] : j[i_Cm];
|
1242
|
+
if ( v[i1] < 4 ) {
|
1243
|
+
int delta = 4 - v[i1];
|
1244
|
+
i2 = is_in_the_list( at[n].neighbor, (AT_NUMB)i, at[n].valence ) - at[n].neighbor;
|
1245
|
+
at[i].bond_type[i1] += delta;
|
1246
|
+
at[n].bond_type[i2] += delta;
|
1247
|
+
at[i].chem_bonds_valence += delta;
|
1248
|
+
at[n].chem_bonds_valence += delta;
|
1249
|
+
at[n].charge = 0;
|
1250
|
+
at[n].radical = 0;
|
1251
|
+
}
|
1252
|
+
}
|
1253
|
+
at[i].charge = 0;
|
1254
|
+
at[i].radical = 0;
|
1255
|
+
num_changes ++;
|
1256
|
+
}
|
1257
|
+
}
|
1258
|
+
}
|
1259
|
+
}
|
1260
|
+
|
1261
|
+
return num_changes;
|
1262
|
+
}
|
1263
|
+
|
1264
|
+
/*#if( DISCONNECT_SALTS == 1 )*/ /* { */
|
1265
|
+
/*************************************************************************************************/
|
1266
|
+
int RemoveInpAtBond( inp_ATOM *atom, int iat, int k )
|
1267
|
+
{
|
1268
|
+
int i, j, m, m2, k2;
|
1269
|
+
inp_ATOM *at = atom + iat;
|
1270
|
+
inp_ATOM *at2;
|
1271
|
+
int val = at->valence - 1;
|
1272
|
+
if ( val >= 0 ) {
|
1273
|
+
int bond = at->bond_type[k];
|
1274
|
+
if ( bond > BOND_TYPE_TRIPLE )
|
1275
|
+
bond = BOND_TYPE_SINGLE; /* added 08-06-2003 */
|
1276
|
+
|
1277
|
+
/* update CML tetrahedral atom parity. */
|
1278
|
+
if ( at->p_parity ) {
|
1279
|
+
for( m = 0; m < MAX_NUM_STEREO_ATOM_NEIGH; m ++ ) {
|
1280
|
+
if ( at->p_orig_at_num[m] == at->orig_at_number ) {
|
1281
|
+
at->p_parity = 0;
|
1282
|
+
break; /* only 3 bonds are present; removing one bond removes stereo */
|
1283
|
+
}
|
1284
|
+
}
|
1285
|
+
if ( at->p_parity /* at->valence == MAX_NUM_STEREO_ATOM_NEIGH*/ ) {
|
1286
|
+
for ( m = 0; m < at->valence; m ++ ) {
|
1287
|
+
if ( atom[(int)at->neighbor[k]].orig_at_number == at->p_orig_at_num[m] ) {
|
1288
|
+
break;
|
1289
|
+
}
|
1290
|
+
}
|
1291
|
+
if ( m < at->valence ) {
|
1292
|
+
at->p_orig_at_num[m] = at->orig_at_number;
|
1293
|
+
} else {
|
1294
|
+
at->p_parity = 0; /* wrong neighbors: at->neighbor[k] is not in the list of a stereo neighbors */
|
1295
|
+
}
|
1296
|
+
}
|
1297
|
+
}
|
1298
|
+
|
1299
|
+
/* update CML stereogenic bond parities; at this point no removed explicit H exist yet */
|
1300
|
+
if ( at->sb_parity[0] ) {
|
1301
|
+
for ( m = 0; m < MAX_NUM_STEREO_BONDS && at->sb_parity[m]; ) {
|
1302
|
+
if ( k == at->sb_ord[m] || k == at->sn_ord[m] && val < 2 && ATOM_PARITY_WELL_DEF(at->sb_parity[m]) ) {
|
1303
|
+
/* !!! FLAW: does take into account removed H !!! */
|
1304
|
+
/* stereogenic bond is being removed OR */
|
1305
|
+
/* remove stereogenic bond because its only neighbor is being removed */
|
1306
|
+
int pnxt_atom, pinxt2cur, pinxt_sb_parity_ord;
|
1307
|
+
int len= get_opposite_sb_atom( atom, iat, at->sb_ord[m], &pnxt_atom, &pinxt2cur, &pinxt_sb_parity_ord );
|
1308
|
+
if ( len ) {
|
1309
|
+
i = pinxt_sb_parity_ord;
|
1310
|
+
at2 = atom + pnxt_atom;
|
1311
|
+
k2 = pinxt2cur;
|
1312
|
+
} else {
|
1313
|
+
i = MAX_NUM_STEREO_BONDS;
|
1314
|
+
}
|
1315
|
+
/*
|
1316
|
+
at2 = atom + at->neighbor[ (int)at->sb_ord[m] ];
|
1317
|
+
for ( i = 0; i < MAX_NUM_STEREO_BONDS && at2->sb_parity[i]; i ++ ) {
|
1318
|
+
if ( iat == at2->neighbor[ (int)at2->sb_ord[i] ] )
|
1319
|
+
break;
|
1320
|
+
}
|
1321
|
+
*/
|
1322
|
+
if ( i < MAX_NUM_STEREO_BONDS && at2->sb_parity[i] ) {
|
1323
|
+
m2 = i;
|
1324
|
+
/* remove bond parity from at */
|
1325
|
+
if ( m < MAX_NUM_STEREO_BONDS-1 ) {
|
1326
|
+
memmove( at->sb_parity+m, at->sb_parity+m+1, (MAX_NUM_STEREO_BONDS-1 - m) * sizeof(at->sb_parity[0]));
|
1327
|
+
memmove( at->sb_ord+m, at->sb_ord+m+1, (MAX_NUM_STEREO_BONDS-1 - m) * sizeof(at->sb_ord[0]));
|
1328
|
+
memmove( at->sn_ord+m, at->sn_ord+m+1, (MAX_NUM_STEREO_BONDS-1 - m) * sizeof(at->sn_ord[0]));
|
1329
|
+
memmove( at->sn_orig_at_num+m, at->sn_orig_at_num+m+1, (MAX_NUM_STEREO_BONDS-1 - m) * sizeof(at->sn_orig_at_num[0]));
|
1330
|
+
}
|
1331
|
+
at->sb_parity[MAX_NUM_STEREO_BONDS-1] = 0;
|
1332
|
+
at->sb_ord[MAX_NUM_STEREO_BONDS-1] = 0;
|
1333
|
+
at->sn_ord[MAX_NUM_STEREO_BONDS-1] = 0;
|
1334
|
+
at->sn_orig_at_num[MAX_NUM_STEREO_BONDS-1] = 0;
|
1335
|
+
/* remove bond parity from at2 */
|
1336
|
+
if ( m2 < MAX_NUM_STEREO_BONDS-1 ) {
|
1337
|
+
memmove( at2->sb_parity+m2, at2->sb_parity+m2+1, (MAX_NUM_STEREO_BONDS-1 - m2) * sizeof(at2->sb_parity[0]));
|
1338
|
+
memmove( at2->sb_ord+m2, at2->sb_ord+m2+1, (MAX_NUM_STEREO_BONDS-1 - m2) * sizeof(at2->sb_ord[0]));
|
1339
|
+
memmove( at2->sn_ord+m2, at2->sn_ord+m2+1, (MAX_NUM_STEREO_BONDS-1 - m2) * sizeof(at2->sn_ord[0]));
|
1340
|
+
memmove( at2->sn_orig_at_num+m2, at2->sn_orig_at_num+m2+1, (MAX_NUM_STEREO_BONDS-1 - m2) * sizeof(at2->sn_orig_at_num[0]));
|
1341
|
+
}
|
1342
|
+
at2->sb_parity[MAX_NUM_STEREO_BONDS-1] = 0;
|
1343
|
+
at2->sb_ord[MAX_NUM_STEREO_BONDS-1] = 0;
|
1344
|
+
at2->sn_ord[MAX_NUM_STEREO_BONDS-1] = 0;
|
1345
|
+
at2->sn_orig_at_num[MAX_NUM_STEREO_BONDS-1] = 0;
|
1346
|
+
/* do not increment m here because the array elements have been shifted */
|
1347
|
+
} else {
|
1348
|
+
m ++; /* program error: inconsistent stereobond parity */
|
1349
|
+
}
|
1350
|
+
} else
|
1351
|
+
if ( k == at->sn_ord[m] ) {
|
1352
|
+
/* stereogenic bond neighbor is being removed; another neighbor remains */
|
1353
|
+
/* !!! FLAW: does take into account removed H !!! */
|
1354
|
+
for ( j = 0, i = -1; j < at->valence; j ++ ) {
|
1355
|
+
if ( j != k && j != at->sb_ord[m] ) {
|
1356
|
+
i = j;
|
1357
|
+
break;
|
1358
|
+
}
|
1359
|
+
}
|
1360
|
+
/* i is the position of the neighbor that will become a new neighbor */
|
1361
|
+
/***************************************************************************
|
1362
|
+
* at->sb_parity[m] is the direction (EVEN=clockwise, ODD=counterclockwise)
|
1363
|
+
* from stereobond to the neighbor. If the neighbor is removed then
|
1364
|
+
* the parity should invert, otherwise it should be unchanged.
|
1365
|
+
***************************************************************************/
|
1366
|
+
if ( i < 0 ) {
|
1367
|
+
/* no alternative neighbor is available */
|
1368
|
+
if ( ATOM_PARITY_WELL_DEF(at->sb_parity[m] ) ) {
|
1369
|
+
/* parity cannot be not well-defined anymore */
|
1370
|
+
int pnxt_atom, pinxt2cur, pinxt_sb_parity_ord;
|
1371
|
+
int len= get_opposite_sb_atom( atom, iat, at->sb_ord[m], &pnxt_atom, &pinxt2cur, &pinxt_sb_parity_ord );
|
1372
|
+
if ( len > 0 ) {
|
1373
|
+
atom[pnxt_atom].sb_parity[pinxt_sb_parity_ord] = at->sb_parity[m] = AB_PARITY_UNDF;
|
1374
|
+
}
|
1375
|
+
#ifdef _DEBUG
|
1376
|
+
else {
|
1377
|
+
int stop = 1; /* sb parities error */
|
1378
|
+
}
|
1379
|
+
#endif
|
1380
|
+
}
|
1381
|
+
at->sn_ord[m] = -99; /* sb neighbor has been disconnected */
|
1382
|
+
at->sb_ord[m] -= (at->sb_ord[m] > k); /* same as above */
|
1383
|
+
at->sn_orig_at_num[m] = 0;
|
1384
|
+
} else
|
1385
|
+
if ( i < at->valence ) {
|
1386
|
+
/* choose another stereogenic bond neighbor, its ord. number is i before bond removal */
|
1387
|
+
if ( ATOM_PARITY_WELL_DEF(at->sb_parity[m]) ) {
|
1388
|
+
/* ALL WRONG: 'move' previous stereo bond neighbor to the last position (pos. 2 out of 0,1,2) */
|
1389
|
+
/* the parity of the transpositions is (2 - at->sn_ord[m])%2 = at->sn_ord[m] % 2 */
|
1390
|
+
/* and replace the neighbor with another; the contribution to the parity is 1 */
|
1391
|
+
|
1392
|
+
/*at->sb_parity[m] = 2 - ( at->sb_parity[m] + at->sn_ord[m] + 1 ) % 2;*/
|
1393
|
+
|
1394
|
+
/*at->sb_parity[m] = 2 - ( at->sb_parity[m] + k + i +
|
1395
|
+
(i > k) + (i > at->sb_ord[m]) ) % 2;*/
|
1396
|
+
/*=== parity should be INVERTED ===*/
|
1397
|
+
at->sb_parity[m] = 3 - at->sb_parity[m];
|
1398
|
+
}
|
1399
|
+
at->sn_ord[m] = i - (i > k); /* ord. number shifted because preceding bond is removed */
|
1400
|
+
at->sb_ord[m] -= (at->sb_ord[m] > k); /* same as above */
|
1401
|
+
at->sn_orig_at_num[m] = atom[(int)at->neighbor[i]].orig_at_number;
|
1402
|
+
/*at->sb_parity[m] = 2 - ( at->sb_parity[m] + 1 ) % 2;*/
|
1403
|
+
} else {
|
1404
|
+
at->sb_parity[m] = 0; /* program error: inconsistent stereobond parity */
|
1405
|
+
}
|
1406
|
+
m ++;
|
1407
|
+
} else {
|
1408
|
+
/* removing another neighbor, k: first move it to the last position (pos. 2 out of 0,1,2) */
|
1409
|
+
if ( k < 2 && ATOM_PARITY_WELL_DEF(at->sb_parity[m]) ) {
|
1410
|
+
/*at->sb_parity[m] = 2 - ( at->sb_parity[m] + k ) % 2;*/
|
1411
|
+
/*at->sb_parity[m] = 2 - ( at->sb_parity[m] + (at->sn_ord[m] > k) + (at->sb_ord[m] > k) ) % 2;*/
|
1412
|
+
;/*==== Parity should remain UNCHANGED ===*/
|
1413
|
+
}
|
1414
|
+
if ( at->sb_ord[m] > k ) {
|
1415
|
+
at->sb_ord[m] --;
|
1416
|
+
}
|
1417
|
+
if ( at->sn_ord[m] > k ) {
|
1418
|
+
at->sn_ord[m] --;
|
1419
|
+
}
|
1420
|
+
m ++;
|
1421
|
+
}
|
1422
|
+
}
|
1423
|
+
}
|
1424
|
+
|
1425
|
+
if ( k < val ) {
|
1426
|
+
memmove( at->neighbor+k, at->neighbor+k+1, sizeof(at->neighbor[0])*(val-k) );
|
1427
|
+
memmove( at->bond_stereo+k, at->bond_stereo+k+1, sizeof(at->bond_stereo[0])*(val-k) );
|
1428
|
+
memmove( at->bond_type+k, at->bond_type+k+1, sizeof(at->bond_type[0])*(val-k) );
|
1429
|
+
}
|
1430
|
+
at->neighbor[val] = 0;
|
1431
|
+
at->bond_stereo[val] = 0;
|
1432
|
+
at->bond_type[val] = 0;
|
1433
|
+
at->valence = val;
|
1434
|
+
at->chem_bonds_valence -= bond;
|
1435
|
+
return 1;
|
1436
|
+
}
|
1437
|
+
return 0;
|
1438
|
+
}
|
1439
|
+
/*************************************************************************************************/
|
1440
|
+
int DisconnectInpAtBond( inp_ATOM *at, AT_NUMB *nOldCompNumber, int iat, int neigh_ord )
|
1441
|
+
{
|
1442
|
+
int neigh, i, ret = 0;
|
1443
|
+
int component;
|
1444
|
+
neigh = at[iat].neighbor[neigh_ord];
|
1445
|
+
for ( i = 0; i < at[neigh].valence; i ++ ) {
|
1446
|
+
if ( iat == (int)at[neigh].neighbor[i] )
|
1447
|
+
break;
|
1448
|
+
}
|
1449
|
+
if ( i < at[neigh].valence ) {
|
1450
|
+
ret += RemoveInpAtBond( at, iat, neigh_ord );
|
1451
|
+
ret += RemoveInpAtBond( at, neigh, i );
|
1452
|
+
if ( nOldCompNumber && ret ) {
|
1453
|
+
if ( component = at[iat].component ) {
|
1454
|
+
nOldCompNumber[component-1] = 0;
|
1455
|
+
}
|
1456
|
+
if ( component = at[neigh].component ) {
|
1457
|
+
nOldCompNumber[component-1] = 0;
|
1458
|
+
}
|
1459
|
+
}
|
1460
|
+
}
|
1461
|
+
return (ret == 2);
|
1462
|
+
}
|
1463
|
+
/*************************************************************************************************/
|
1464
|
+
int bIsAmmoniumSalt( inp_ATOM *at, int i, int *piO, int *pk, S_CHAR *num_explicit_H )
|
1465
|
+
{
|
1466
|
+
/* NH4(+charge)-O(-charge)-C -> NH3 + HO-C; any charge including 0, any C except charged or radical */
|
1467
|
+
/* F, Cl, Br, I */
|
1468
|
+
static U_CHAR el_number_C=0, el_number_O=0, el_number_H=0, el_number_N=0;
|
1469
|
+
static U_CHAR el_number_F=0, el_number_Cl=0, el_number_Br=0, el_number_I=0;
|
1470
|
+
int num_H, num_non_iso_H, num_impl_iso_H, bDisconnect = 1;
|
1471
|
+
int j, val, neigh, iO=-1, iC, k=-1;
|
1472
|
+
if ( 0 == el_number_C ) {
|
1473
|
+
/* one time initialization */
|
1474
|
+
el_number_C = get_periodic_table_number( "C" );
|
1475
|
+
el_number_O = get_periodic_table_number( "O" );
|
1476
|
+
el_number_H = get_periodic_table_number( "H" );
|
1477
|
+
el_number_N = get_periodic_table_number( "N" );
|
1478
|
+
el_number_F = get_periodic_table_number( "F" );
|
1479
|
+
el_number_Cl= get_periodic_table_number( "Cl" );
|
1480
|
+
el_number_Br= get_periodic_table_number( "Br" );
|
1481
|
+
el_number_I = get_periodic_table_number( "I" );
|
1482
|
+
}
|
1483
|
+
if ( at[i].el_number != el_number_N )
|
1484
|
+
return 0;
|
1485
|
+
|
1486
|
+
/* check for NH4-O-C... -> NH3 + HO-C... */
|
1487
|
+
val = at[i].valence;
|
1488
|
+
num_impl_iso_H = NUM_ISO_H(at,i);
|
1489
|
+
num_non_iso_H = at[i].num_H;
|
1490
|
+
num_H = num_non_iso_H + num_impl_iso_H;
|
1491
|
+
if ( val + num_H == 5 ) {
|
1492
|
+
int num_O = 0;
|
1493
|
+
memset( num_explicit_H, 0, (NUM_H_ISOTOPES+1)*sizeof(num_explicit_H[0]) );
|
1494
|
+
for ( j = 0; j < val; j ++ ) { /* looking for O: H4N-O-C... */
|
1495
|
+
neigh = at[i].neighbor[j];
|
1496
|
+
if ( at[neigh].num_H ||
|
1497
|
+
at[neigh].charge && (at[neigh].el_number != el_number_O || at[neigh].charge + at[i].charge) ||
|
1498
|
+
at[neigh].radical && at[neigh].radical != RADICAL_SINGLET ) {
|
1499
|
+
bDisconnect = 0;
|
1500
|
+
break; /* reject */
|
1501
|
+
}
|
1502
|
+
if ( at[neigh].el_number == el_number_H && at[neigh].valence == 1 &&
|
1503
|
+
!at[neigh].charge && !at[neigh].radical ) {
|
1504
|
+
num_H ++; /* at this point at[].num_H does not include explicit H count */
|
1505
|
+
num_non_iso_H += (0==at[neigh].iso_atw_diff);
|
1506
|
+
num_explicit_H[at[neigh].iso_atw_diff] ++; /* explicit H on N */
|
1507
|
+
} else
|
1508
|
+
if ( at[neigh].el_number == el_number_O && at[neigh].valence == 2 && !num_O ) {
|
1509
|
+
num_O ++; /* found O: N-O- */
|
1510
|
+
iO = neigh;
|
1511
|
+
k = j;
|
1512
|
+
iC = at[iO].neighbor[at[iO].neighbor[0] == i];
|
1513
|
+
if ( at[iC].el_number != el_number_C || /*
|
1514
|
+
at[iC].num_H ||
|
1515
|
+
at[iC].chem_bonds_valence != 4 || */
|
1516
|
+
at[iC].charge ||
|
1517
|
+
at[iC].radical && at[iC].radical != RADICAL_SINGLET /*||
|
1518
|
+
at[iC].valence == at[iC].chem_bonds_valence*/ ) {
|
1519
|
+
bDisconnect = 0;
|
1520
|
+
break; /* reject */
|
1521
|
+
}
|
1522
|
+
} else
|
1523
|
+
if ( (at[neigh].el_number == el_number_F ||
|
1524
|
+
at[neigh].el_number == el_number_Cl ||
|
1525
|
+
at[neigh].el_number == el_number_Br ||
|
1526
|
+
at[neigh].el_number == el_number_I ) &&
|
1527
|
+
at[neigh].valence == 1 && at[neigh].chem_bonds_valence == 1 &&
|
1528
|
+
!at[neigh].charge && !NUMH(at,neigh) && !num_O ) {
|
1529
|
+
num_O ++; /* found O: N-O- */
|
1530
|
+
iO = neigh;
|
1531
|
+
k = j;
|
1532
|
+
iC = -1;
|
1533
|
+
} else {
|
1534
|
+
bDisconnect = 0;
|
1535
|
+
break; /* reject */
|
1536
|
+
}
|
1537
|
+
}
|
1538
|
+
if ( bDisconnect && (num_O != 1 || num_H != 4) ) {
|
1539
|
+
bDisconnect = 0; /* reject */
|
1540
|
+
}
|
1541
|
+
} else {
|
1542
|
+
bDisconnect = 0;
|
1543
|
+
}
|
1544
|
+
if ( bDisconnect ) {
|
1545
|
+
*piO = iO;
|
1546
|
+
*pk = k;
|
1547
|
+
}
|
1548
|
+
return bDisconnect;
|
1549
|
+
}
|
1550
|
+
/*************************************************************************************************/
|
1551
|
+
int DisconnectAmmoniumSalt ( inp_ATOM *at, int iN, int iO, int k, S_CHAR *num_explicit_H )
|
1552
|
+
{
|
1553
|
+
/* disconnect NH4-O from O */
|
1554
|
+
/* Note: iO = at[iN].neighbor[k], at[iN] is N, at[iO].neighbor[0] is either N=at[iN] or C=at[iC] */
|
1555
|
+
int nMove_H_iso_diff = -1; /* do not move explicit H */
|
1556
|
+
int j, neigh, iso_diff, neigh_pos;
|
1557
|
+
static U_CHAR el_number_H = 0;
|
1558
|
+
int val = at[iN].valence;
|
1559
|
+
|
1560
|
+
if ( !el_number_H ) {
|
1561
|
+
el_number_H = get_periodic_table_number( "H" );
|
1562
|
+
}
|
1563
|
+
if ( at[iN].charge && !(at[iN].charge + at[iO].charge) ) {
|
1564
|
+
at[iN].charge = at[iO].charge = 0; /* remove charges */
|
1565
|
+
}
|
1566
|
+
neigh_pos = (at[iO].valence == 2)? (at[iO].neighbor[1] == iN) : 0; /* position of at[iN] in the neigh list of iO */
|
1567
|
+
/* disconnect bond O-N */
|
1568
|
+
RemoveInpAtBond( at, iO, neigh_pos );
|
1569
|
+
RemoveInpAtBond( at, iN, k );
|
1570
|
+
val --;
|
1571
|
+
|
1572
|
+
/* move 1 H from NH4 to O- or Cl */
|
1573
|
+
|
1574
|
+
/* find non-isotopic or the lightest isotopic H to move from N to O */
|
1575
|
+
for ( iso_diff = 0; iso_diff <= NUM_H_ISOTOPES; iso_diff ++ ) {
|
1576
|
+
if ( !iso_diff ) {
|
1577
|
+
/* find non-isotopic H */
|
1578
|
+
if ( at[iN].num_H ) {
|
1579
|
+
at[iN].num_H --; /* move non-isotopic implicit H */
|
1580
|
+
at[iO].num_H ++;
|
1581
|
+
break;
|
1582
|
+
} else
|
1583
|
+
if ( num_explicit_H[0] ) {
|
1584
|
+
nMove_H_iso_diff = 0; /* flag: move explicit non-isotopic H */
|
1585
|
+
break;
|
1586
|
+
}
|
1587
|
+
} else {
|
1588
|
+
/* find isotopic H */
|
1589
|
+
if ( at[iN].num_iso_H[iso_diff] ) {
|
1590
|
+
at[iN].num_iso_H[iso_diff] --; /* move implicit isotopic H, atw = 1 */
|
1591
|
+
at[iO].num_iso_H[iso_diff] ++;
|
1592
|
+
break;
|
1593
|
+
} else
|
1594
|
+
if ( num_explicit_H[iso_diff] ) {
|
1595
|
+
nMove_H_iso_diff = iso_diff; /* flag: move explicit isotopic H, atw = 1 */
|
1596
|
+
break;
|
1597
|
+
}
|
1598
|
+
}
|
1599
|
+
}
|
1600
|
+
if ( nMove_H_iso_diff >= 0 ) {
|
1601
|
+
/* move explicit H, it is isotopic if nMove_H_iso_diff > 0 */
|
1602
|
+
double dist2_H_O, min_dist2_H_O = -1.0;
|
1603
|
+
int jH = -1, iH = -1;
|
1604
|
+
for ( j = 0; j < val; j ++ ) { /* looking H in N-H such that H-O is shortest */
|
1605
|
+
neigh = at[iN].neighbor[j];
|
1606
|
+
if ( at[neigh].el_number == el_number_H &&
|
1607
|
+
at[neigh].iso_atw_diff == nMove_H_iso_diff ) {
|
1608
|
+
dist2_H_O = (at[neigh].x - at[iO].x) * (at[neigh].x - at[iO].x) +
|
1609
|
+
(at[neigh].y - at[iO].y) * (at[neigh].y - at[iO].y) +
|
1610
|
+
(at[neigh].z - at[iO].z) * (at[neigh].z - at[iO].z);
|
1611
|
+
if ( min_dist2_H_O < 0.0 || min_dist2_H_O > dist2_H_O ) {
|
1612
|
+
min_dist2_H_O = dist2_H_O;
|
1613
|
+
iH = neigh;
|
1614
|
+
jH = j;
|
1615
|
+
}
|
1616
|
+
}
|
1617
|
+
}
|
1618
|
+
/* reconnect; bonds do not need changes except stereo */
|
1619
|
+
neigh_pos = at[iO].valence;
|
1620
|
+
at[iO].neighbor[neigh_pos] = iH;
|
1621
|
+
at[iO].bond_stereo[neigh_pos] = 0;
|
1622
|
+
at[iO].bond_type[neigh_pos] = at[iH].bond_type[0];
|
1623
|
+
at[iO].chem_bonds_valence += at[iH].bond_type[0];
|
1624
|
+
at[iO].valence ++;
|
1625
|
+
at[iH].neighbor[0] = iO;
|
1626
|
+
at[iH].bond_stereo[0] = 0;
|
1627
|
+
/* disconnect H from N */
|
1628
|
+
RemoveInpAtBond( at, iN, jH );
|
1629
|
+
val --;
|
1630
|
+
if ( k > jH ) {
|
1631
|
+
k --;
|
1632
|
+
}
|
1633
|
+
}
|
1634
|
+
return 1;
|
1635
|
+
}
|
1636
|
+
/*************************************************************************************************/
|
1637
|
+
int bIsMetalSalt( inp_ATOM *at, int i )
|
1638
|
+
{
|
1639
|
+
int type, val, k, iO, iC, j, neigh;
|
1640
|
+
int bDisconnect = 1;
|
1641
|
+
static U_CHAR el_number_C=0, el_number_O=0, el_number_H=0;
|
1642
|
+
static U_CHAR el_number_F=0, el_number_Cl=0, el_number_Br=0, el_number_I=0;
|
1643
|
+
if ( 0 == el_number_C ) {
|
1644
|
+
/* one time initialization */
|
1645
|
+
el_number_C = get_periodic_table_number( "C" );
|
1646
|
+
el_number_O = get_periodic_table_number( "O" );
|
1647
|
+
el_number_H = get_periodic_table_number( "H" );
|
1648
|
+
el_number_F = get_periodic_table_number( "F" );
|
1649
|
+
el_number_Cl= get_periodic_table_number( "Cl" );
|
1650
|
+
el_number_Br= get_periodic_table_number( "Br" );
|
1651
|
+
el_number_I = get_periodic_table_number( "I" );
|
1652
|
+
}
|
1653
|
+
/* check for a metal atom:
|
1654
|
+
metal atom should be connected and be a metal */
|
1655
|
+
if ( !(val = at[i].valence) ||
|
1656
|
+
!(type = get_el_type( at[i].el_number )) ||
|
1657
|
+
!(type & IS_METAL) ) {
|
1658
|
+
bDisconnect = 0; /* reject */
|
1659
|
+
} else
|
1660
|
+
/* metal atom should not have adjacent H or multiple bonds or radical */
|
1661
|
+
if ( at[i].num_H ) {
|
1662
|
+
bDisconnect = 0; /* reject */
|
1663
|
+
} else
|
1664
|
+
/* check valence */
|
1665
|
+
if ( at[i].charge == 0 &&
|
1666
|
+
( (type & 1) && val == get_el_valence( at[i].el_number, 0, 0 ) ||
|
1667
|
+
(type & 2) && val == get_el_valence( at[i].el_number, 0, 1 ) ) ||
|
1668
|
+
at[i].charge > 0 &&
|
1669
|
+
(type & 1) && val == get_el_valence( at[i].el_number, at[i].charge, 0 ) ) {
|
1670
|
+
; /* accept */
|
1671
|
+
} else {
|
1672
|
+
bDisconnect = 0; /* reject */
|
1673
|
+
}
|
1674
|
+
if ( bDisconnect ) {
|
1675
|
+
/*************************************************************************
|
1676
|
+
* | *
|
1677
|
+
* check M neighbors. Disconnect if all neighbors are M-O-C# or M-O-C= *
|
1678
|
+
* | *
|
1679
|
+
*************************************************************************/
|
1680
|
+
for ( k = 0; k < at[i].valence; k ++ ) {
|
1681
|
+
iO = at[i].neighbor[k];
|
1682
|
+
/* halogenide 2004-07-08 */
|
1683
|
+
if ( (at[iO].el_number == el_number_F ||
|
1684
|
+
at[iO].el_number == el_number_Cl ||
|
1685
|
+
at[iO].el_number == el_number_Br ||
|
1686
|
+
at[iO].el_number == el_number_I ) &&
|
1687
|
+
at[iO].valence == 1 && at[iO].chem_bonds_valence == 1 &&
|
1688
|
+
!at[iO].charge && !(at[iO].radical && at[iO].radical != RADICAL_SINGLET) && !NUMH(at,iO) ) {
|
1689
|
+
; /* found */
|
1690
|
+
} else {
|
1691
|
+
/* -O-C= */
|
1692
|
+
if ( at[iO].el_number != el_number_O ||
|
1693
|
+
NUMH(at, iO) ||
|
1694
|
+
at[iO].valence != 2 ||
|
1695
|
+
at[iO].charge ||
|
1696
|
+
at[iO].radical && at[iO].radical != RADICAL_SINGLET ||
|
1697
|
+
at[iO].valence != at[iO].chem_bonds_valence ) {
|
1698
|
+
bDisconnect = 0; /* reject */
|
1699
|
+
break;
|
1700
|
+
}
|
1701
|
+
iC = at[iO].neighbor[at[iO].neighbor[0] == i];
|
1702
|
+
if ( at[iC].el_number != el_number_C ||
|
1703
|
+
at[iC].num_H ||
|
1704
|
+
at[iC].chem_bonds_valence != 4 ||
|
1705
|
+
at[iC].charge ||
|
1706
|
+
at[iC].radical && at[iC].radical != RADICAL_SINGLET ||
|
1707
|
+
at[iC].valence == at[iC].chem_bonds_valence ) {
|
1708
|
+
bDisconnect = 0; /* reject */
|
1709
|
+
break;
|
1710
|
+
}
|
1711
|
+
for ( j = 0; j < at[iC].valence; j ++ ) {
|
1712
|
+
neigh = at[iC].neighbor[j];
|
1713
|
+
if ( at[neigh].el_number == el_number_H ) {
|
1714
|
+
break;
|
1715
|
+
}
|
1716
|
+
}
|
1717
|
+
if ( j != at[iC].valence ) {
|
1718
|
+
bDisconnect = 0; /* reject */
|
1719
|
+
break;
|
1720
|
+
}
|
1721
|
+
}
|
1722
|
+
}
|
1723
|
+
}
|
1724
|
+
return bDisconnect;
|
1725
|
+
}
|
1726
|
+
/*************************************************************************************************/
|
1727
|
+
int DisconnectMetalSalt( inp_ATOM *at, int i )
|
1728
|
+
{
|
1729
|
+
int k, iO;
|
1730
|
+
/* disconnect metal atom or ion at[i] */
|
1731
|
+
for ( k = 0; k < at[i].valence; k ++ ) {
|
1732
|
+
iO = at[i].neighbor[k];
|
1733
|
+
if ( at[iO].valence == 2 ) {
|
1734
|
+
if ( at[iO].neighbor[0] == i ) { /* assuming atom O always has 2 bonds */
|
1735
|
+
/* copy the remaining neighbor to the 0 position */
|
1736
|
+
at[iO].neighbor[0] = at[iO].neighbor[1];
|
1737
|
+
at[iO].bond_stereo[0] = at[iO].bond_stereo[1];
|
1738
|
+
at[iO].bond_type[0] = at[iO].bond_type[1];
|
1739
|
+
}
|
1740
|
+
/* clear neighbor at position 1 */
|
1741
|
+
at[iO].neighbor[1] = 0;
|
1742
|
+
at[iO].bond_stereo[1] = 0;
|
1743
|
+
at[iO].bond_type[1] = 0;
|
1744
|
+
} else {
|
1745
|
+
/* clear neighbor at position 1 */
|
1746
|
+
at[iO].neighbor[0] = 0;
|
1747
|
+
at[iO].bond_stereo[0] = 0;
|
1748
|
+
at[iO].bond_type[0] = 0;
|
1749
|
+
}
|
1750
|
+
/* make O negatively charged */
|
1751
|
+
at[iO].charge = -1;
|
1752
|
+
/* reduce O valence to account for the removed single bond */
|
1753
|
+
at[iO].valence --;
|
1754
|
+
at[iO].chem_bonds_valence --;
|
1755
|
+
|
1756
|
+
/* clear metal neighbor (O) */
|
1757
|
+
at[i].neighbor[k] = 0;
|
1758
|
+
at[i].bond_stereo[k] = 0;
|
1759
|
+
at[i].bond_type[k] = 0;
|
1760
|
+
/* add a positive charge to the metal */
|
1761
|
+
at[i].charge ++;
|
1762
|
+
}
|
1763
|
+
/* set metal valence to zero because it has been disconnected */
|
1764
|
+
at[i].valence = 0;
|
1765
|
+
at[i].chem_bonds_valence = 0;
|
1766
|
+
return k;
|
1767
|
+
}
|
1768
|
+
|
1769
|
+
/*************************************************************************************************/
|
1770
|
+
int DisconnectSalts( ORIG_ATOM_DATA *orig_inp_data, int bDisconnect )
|
1771
|
+
{
|
1772
|
+
int i, k, iO, num_changes, val;
|
1773
|
+
S_CHAR num_explicit_H[NUM_H_ISOTOPES+1];
|
1774
|
+
inp_ATOM *at = orig_inp_data->at;
|
1775
|
+
int num_at = orig_inp_data->num_inp_atoms;
|
1776
|
+
|
1777
|
+
/* check each atom */
|
1778
|
+
for ( i = 0, num_changes = 0; i < num_at; i ++ ) {
|
1779
|
+
|
1780
|
+
if ( !(val = at[i].valence) || /* disconnected atom */
|
1781
|
+
val != at[i].chem_bonds_valence || /* a bond has higher multiplicity than 1 */
|
1782
|
+
at[i].radical && at[i].radical != RADICAL_SINGLET /* radical */ ) {
|
1783
|
+
continue; /* reject */
|
1784
|
+
}
|
1785
|
+
if ( bIsAmmoniumSalt( at, i, &iO, &k, num_explicit_H ) ) {
|
1786
|
+
if ( bDisconnect ) {
|
1787
|
+
DisconnectAmmoniumSalt ( at, i, iO, k, num_explicit_H );
|
1788
|
+
orig_inp_data->num_inp_bonds --;
|
1789
|
+
}
|
1790
|
+
/* count disconnected atoms */
|
1791
|
+
num_changes ++;
|
1792
|
+
} else
|
1793
|
+
if ( bIsMetalSalt( at, i ) ) {
|
1794
|
+
if ( bDisconnect ) {
|
1795
|
+
k = DisconnectMetalSalt( at, i );
|
1796
|
+
orig_inp_data->num_inp_bonds -= k;
|
1797
|
+
}
|
1798
|
+
num_changes ++;
|
1799
|
+
}
|
1800
|
+
}
|
1801
|
+
return num_changes;
|
1802
|
+
}
|
1803
|
+
/*****************************************************************************/
|
1804
|
+
/* Important: Salt disconnection is independent from coord. disconnection: */
|
1805
|
+
/* because different atoms are disconnected. */
|
1806
|
+
/* However, sal disconnection may need to be rerun after metal disconnection */
|
1807
|
+
/* because metal disconnection may make certain atoms be eligible for salt */
|
1808
|
+
/* disconnection */
|
1809
|
+
/*****************************************************************************/
|
1810
|
+
int bIsMetalToDisconnect(inp_ATOM *at, int i, int bCheckMetalValence)
|
1811
|
+
{
|
1812
|
+
int type, at_valence, num_H;
|
1813
|
+
/*
|
1814
|
+
if ( !at[i].valence )
|
1815
|
+
*/
|
1816
|
+
if ( !(type = get_el_type( at[i].el_number )) ||
|
1817
|
+
!(type & IS_METAL ) ) {
|
1818
|
+
return 0;
|
1819
|
+
}
|
1820
|
+
num_H = NUMH(at,i);
|
1821
|
+
at_valence = num_H + at[i].chem_bonds_valence;
|
1822
|
+
if ( !at_valence ) {
|
1823
|
+
return 0; /* nothing to disconnect */
|
1824
|
+
}
|
1825
|
+
if ( bCheckMetalValence ) {
|
1826
|
+
if ( abs(at[i].charge) > 1 ) {
|
1827
|
+
return 1; /* multiple charges */
|
1828
|
+
}
|
1829
|
+
for ( i = 0; i < 2 && (i & type); i ++ ) {
|
1830
|
+
if ( at_valence == get_el_valence( at[i].el_number, at[i].charge, i ) ) {
|
1831
|
+
return 2; /* atom has normal valence */
|
1832
|
+
}
|
1833
|
+
}
|
1834
|
+
}
|
1835
|
+
return 1;
|
1836
|
+
|
1837
|
+
}
|
1838
|
+
/*****************************************************************************/
|
1839
|
+
int bMayDisconnectMetals( ORIG_ATOM_DATA *orig_inp_data, int bCheckMetalValence, INCHI_MODE *bTautFlagsDone )
|
1840
|
+
{
|
1841
|
+
int i, j, k, iO, num_changes, val, bRadOrMultBonds, num_impl_H = 0;
|
1842
|
+
S_CHAR num_explicit_H[NUM_H_ISOTOPES+1];
|
1843
|
+
inp_ATOM *at = orig_inp_data->at;
|
1844
|
+
int num_at = orig_inp_data->num_inp_atoms;
|
1845
|
+
int *nNumImplH = &orig_inp_data->bDisconnectCoord;
|
1846
|
+
/* check each atom */
|
1847
|
+
for ( i = 0, num_changes = 0; i < num_at; i ++ ) {
|
1848
|
+
|
1849
|
+
if ( !(val = at[i].valence) && !NUMH(at,i) ) {
|
1850
|
+
continue; /* disconnected atom */
|
1851
|
+
}
|
1852
|
+
bRadOrMultBonds = (val == 0) ||
|
1853
|
+
(val != at[i].chem_bonds_valence) || /* a bond has higher multiplicity than 1 */
|
1854
|
+
(at[i].radical && at[i].radical != RADICAL_SINGLET); /* radical */
|
1855
|
+
|
1856
|
+
if ( !bRadOrMultBonds && bIsAmmoniumSalt( at, i, &iO, &k, num_explicit_H ) ) {
|
1857
|
+
;
|
1858
|
+
} else
|
1859
|
+
if ( !bRadOrMultBonds && bIsMetalSalt( at, i ) ) {
|
1860
|
+
;
|
1861
|
+
} else
|
1862
|
+
if ( 1 == (j = bIsMetalToDisconnect(at, i, bCheckMetalValence)) ) {
|
1863
|
+
num_impl_H += NUMH(at,i);
|
1864
|
+
num_changes ++;
|
1865
|
+
} else
|
1866
|
+
if ( 2 == j && bTautFlagsDone ) {
|
1867
|
+
*bTautFlagsDone |= TG_FLAG_CHECK_VALENCE_COORD_DONE;
|
1868
|
+
}
|
1869
|
+
}
|
1870
|
+
if ( nNumImplH )
|
1871
|
+
*nNumImplH = num_changes? num_impl_H+1 : 0;
|
1872
|
+
return num_changes;
|
1873
|
+
}
|
1874
|
+
/*****************************************************************************/
|
1875
|
+
#if( bRELEASE_VERSION == 0 && (EXTR_HAS_METAL_ATOM & (EXTR_MASK | EXTR_FLAG) ) )
|
1876
|
+
int bHasMetalAtom( ORIG_ATOM_DATA *orig_inp_data )
|
1877
|
+
{
|
1878
|
+
int i;
|
1879
|
+
inp_ATOM *at;
|
1880
|
+
if ( orig_inp_data && (at = orig_inp_data->at) ) {
|
1881
|
+
int num_at = orig_inp_data->num_inp_atoms;
|
1882
|
+
/* check each atom */
|
1883
|
+
for ( i = 0; i < num_at; i ++ ) {
|
1884
|
+
if ( IS_METAL & get_el_type( at[i].el_number ) ) {
|
1885
|
+
return 1;
|
1886
|
+
}
|
1887
|
+
}
|
1888
|
+
}
|
1889
|
+
return 0;
|
1890
|
+
}
|
1891
|
+
#endif
|
1892
|
+
/*****************************************************************************
|
1893
|
+
{ "F", 19, 19, 18.998403220, 0 , 0, {{0,}, {0,}, {1,}, {2,}, {3,5}, },},
|
1894
|
+
{ "Cl", 35, 35, 34.968852730, 0 , 0, {{0,}, {0,}, {1,3,5,7}, {2,4,6}, {3,5,}, },},
|
1895
|
+
{ "Br", 80, 79, 78.918336100, 0 , 0, {{0,}, {0,}, {1,3,5,7,}, {2,4,6,}, {3,5,}, },},
|
1896
|
+
{ "I", 127, 127, 126.904500000, 0 , 0, {{0,}, {0,}, {1,3,5,7,}, {2,4,6}, {3,5,}, },},
|
1897
|
+
{ "At", 210, 210, 209.987100000, 0 , 0, {{0,}, {0,}, {1,3,5,7,}, {2,4,6}, {3,5,}, },},
|
1898
|
+
{ "N", 14, 14, 14.003074000, 0 , 0, {{1,}, {2,}, {3,5}, {4,}, {3,}, },},
|
1899
|
+
{ "P", 31, 31, 30.973762000, 0 , 0, {{1,3,5,7,}, {2,4,6,}, {3,5,}, {4,}, {3,}, },},
|
1900
|
+
{ "As", 75, 75, 74.921594200, 0 , 0, {{0,}, {2,4,6,}, {3,5,}, {4,}, {3,}, },},
|
1901
|
+
{ "Sb", 122, 121, 120.903800000, 0 , 0, {{1,3,5,7,}, {2,4,6,}, {3,5,}, {2,4,}, {3,}, },},
|
1902
|
+
{ "O", 16, 16, 15.994914630, 0 , 0, {{0,}, {1,}, {2,}, {3,5,}, {4,}, },},
|
1903
|
+
{ "S", 32, 32, 31.972070700, 0 , 0, {{0,}, {1,3,5,7,}, {2,4,6}, {3,5,}, {4,}, },},
|
1904
|
+
{ "Se", 79, 80, 79.916519600, 0 , 0, {{0,}, {1,3,5,7,}, {2,4,6,}, {3,5,}, {4,}, },},
|
1905
|
+
{ "Te", 128, 130, 129.906200000, 0 , 0, {{0,}, {1,3,5,7,}, {2,4,6,}, {3,5,}, {2,4,}, },},
|
1906
|
+
{ "Po", 209, 209, 208.982400000, 0 , 0, {{0,}, {1,3,5,7,}, {2,4,6,}, {3,5,}, {2,4,}, },},
|
1907
|
+
{ "B", 11, 11, 11.009300000, 0 , 0, {{3,}, {4,}, {3,}, {2,}, {1,}, },},
|
1908
|
+
*****************************************************************************/
|
1909
|
+
int DisconnectMetals( ORIG_ATOM_DATA *orig_inp_data, int bCheckMetalValence, INCHI_MODE *bTautFlagsDone )
|
1910
|
+
/*inp_ATOM *atom, int num_atoms, int nNumExplH, int *new_num_atoms */
|
1911
|
+
{
|
1912
|
+
int i, j, k, n, iO, num_changes, val, bRadOrMultBonds;
|
1913
|
+
int num_impl_H, num_at, err, num_disconnected;
|
1914
|
+
S_CHAR num_explicit_H[NUM_H_ISOTOPES+1];
|
1915
|
+
static char elnumber_Heteroat[16] = {'\0', };
|
1916
|
+
static int num_halogens;
|
1917
|
+
inp_ATOM *at = NULL;
|
1918
|
+
S_CHAR *bMetal = NULL;
|
1919
|
+
inp_ATOM *atom = orig_inp_data->at;
|
1920
|
+
int num_atoms = orig_inp_data->num_inp_atoms;
|
1921
|
+
int nNumExplH = (orig_inp_data->bDisconnectCoord > 0)? orig_inp_data->bDisconnectCoord - 1 : 0;
|
1922
|
+
AT_NUMB *nOldCompNumber = orig_inp_data->nOldCompNumber;
|
1923
|
+
|
1924
|
+
err = 0;
|
1925
|
+
num_impl_H = 0;
|
1926
|
+
num_at = num_atoms;
|
1927
|
+
num_disconnected = 0;
|
1928
|
+
if ( !(at = (inp_ATOM *)inchi_calloc( num_at + nNumExplH, sizeof(at[0] ) )) ||
|
1929
|
+
!(bMetal = ( S_CHAR *)inchi_calloc( num_at + nNumExplH, sizeof(bMetal[0]) )) ) {
|
1930
|
+
err = 1;
|
1931
|
+
goto exit_function;
|
1932
|
+
}
|
1933
|
+
if (!elnumber_Heteroat[0] ) {
|
1934
|
+
i = 0;
|
1935
|
+
/* halogens */
|
1936
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "F" ); /* 0 */
|
1937
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "Cl" );
|
1938
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "Br" );
|
1939
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "I" );
|
1940
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "At" ); /* 4 */
|
1941
|
+
num_halogens = i;
|
1942
|
+
/* other non-metal */
|
1943
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "N" );
|
1944
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "P" );
|
1945
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "As" );
|
1946
|
+
/*elnumber_Heteroat[i++] = get_periodic_table_number( "Sb" );*/ /* metal 10-28-2003 */
|
1947
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "O" );
|
1948
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "S" );
|
1949
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "Se" );
|
1950
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "Te" );
|
1951
|
+
/*elnumber_Heteroat[i++] = get_periodic_table_number( "Po" );*/ /* metal 10-28-2003 */
|
1952
|
+
elnumber_Heteroat[i++] = (char)get_periodic_table_number( "B" );
|
1953
|
+
elnumber_Heteroat[i++] = 0;
|
1954
|
+
}
|
1955
|
+
|
1956
|
+
memcpy( at, atom, num_atoms * sizeof(at[0]) );
|
1957
|
+
|
1958
|
+
/* check each atom, mark metals */
|
1959
|
+
for ( i = 0, k = 0, num_changes = 0; i < num_atoms; i ++ ) {
|
1960
|
+
|
1961
|
+
if ( !(val = at[i].valence) && !NUMH(at,i) ) {
|
1962
|
+
continue; /* disconnected atom */
|
1963
|
+
}
|
1964
|
+
bRadOrMultBonds = (val == 0) ||
|
1965
|
+
(val != at[i].chem_bonds_valence) || /* a bond has higher multiplicity than 1 */
|
1966
|
+
(at[i].radical && at[i].radical != RADICAL_SINGLET); /* radical */
|
1967
|
+
|
1968
|
+
if ( !bRadOrMultBonds && bIsAmmoniumSalt( at, i, &iO, &k, num_explicit_H ) ) {
|
1969
|
+
;
|
1970
|
+
} else
|
1971
|
+
if ( !bRadOrMultBonds && bIsMetalSalt( at, i ) ) {
|
1972
|
+
;
|
1973
|
+
} else
|
1974
|
+
if ( 1 == (j = bIsMetalToDisconnect(at, i, bCheckMetalValence)) ) {
|
1975
|
+
num_impl_H += (k = NUMH(at,i));
|
1976
|
+
bMetal[i] = 1+k;
|
1977
|
+
num_changes ++;
|
1978
|
+
} else
|
1979
|
+
if ( 2 == j && bTautFlagsDone ) {
|
1980
|
+
*bTautFlagsDone |= TG_FLAG_CHECK_VALENCE_COORD_DONE;
|
1981
|
+
}
|
1982
|
+
}
|
1983
|
+
if ( num_impl_H != nNumExplH ) {
|
1984
|
+
err = 2;
|
1985
|
+
goto exit_function;
|
1986
|
+
}
|
1987
|
+
|
1988
|
+
|
1989
|
+
/* replace implicit H atoms with explicit H atoms */
|
1990
|
+
for ( i = 0; i < num_atoms && 0 < num_impl_H; i ++ ) {
|
1991
|
+
if ( bMetal[i] <= 1 ) {
|
1992
|
+
continue;
|
1993
|
+
}
|
1994
|
+
for ( k = 0; k < NUM_H_ISOTOPES+1; k ++ ) {
|
1995
|
+
n = k? at[i].num_iso_H[k-1] : at[i].num_H;
|
1996
|
+
for ( j = 0; j < n; j ++ ) {
|
1997
|
+
if ( num_at >= num_atoms + nNumExplH ) {
|
1998
|
+
err = 3;
|
1999
|
+
goto exit_function;
|
2000
|
+
}
|
2001
|
+
at[num_at].elname[0] = 'H';
|
2002
|
+
at[num_at].el_number = get_periodic_table_number(at[num_at].elname);
|
2003
|
+
at[num_at].iso_atw_diff = k;
|
2004
|
+
at[num_at].component = at[i].component;
|
2005
|
+
move_explicit_Hcation(at, num_at+1, i, num_at, 1);
|
2006
|
+
at[num_at].orig_at_number = num_at+1;
|
2007
|
+
num_at ++;
|
2008
|
+
num_impl_H --;
|
2009
|
+
bMetal[i] --;
|
2010
|
+
if ( k ) {
|
2011
|
+
at[i].num_iso_H[k-1] --;
|
2012
|
+
} else {
|
2013
|
+
at[i].num_H --;
|
2014
|
+
}
|
2015
|
+
}
|
2016
|
+
}
|
2017
|
+
if ( bMetal[i] != 1 ) {
|
2018
|
+
err = 4;
|
2019
|
+
goto exit_function;
|
2020
|
+
}
|
2021
|
+
}
|
2022
|
+
if ( num_at != num_atoms + nNumExplH ) {
|
2023
|
+
err = 5;
|
2024
|
+
goto exit_function;
|
2025
|
+
}
|
2026
|
+
|
2027
|
+
/* disconnect metal - ligand bonds */
|
2028
|
+
for ( i = 0; i < num_atoms; i ++ ) {
|
2029
|
+
if ( !bMetal[i] ) {
|
2030
|
+
continue;
|
2031
|
+
}
|
2032
|
+
/* disconnect metal atom M
|
2033
|
+
|
2034
|
+
Note: Defect in case of bridging ligands:
|
2035
|
+
|
2036
|
+
M M M M M M(+)
|
2037
|
+
\ / will be transformed to , not to
|
2038
|
+
N(+) N(+) N(-)
|
2039
|
+
/ \ / \ / \
|
2040
|
+
R R R R R R
|
2041
|
+
|
2042
|
+
Non-bridging are OK:
|
2043
|
+
|
2044
|
+
M R M(+) R
|
2045
|
+
\ / /
|
2046
|
+
N(+) ---> N
|
2047
|
+
/ \ / \
|
2048
|
+
R R R R
|
2049
|
+
|
2050
|
+
*/
|
2051
|
+
for ( j = at[i].valence-1; 0 <= j; j -- ) {
|
2052
|
+
if ( j < at[i].valence && !bMetal[ (int)at[i].neighbor[j] ] ) {
|
2053
|
+
/* do not break metal-metal bond here */
|
2054
|
+
num_disconnected += DisconnectOneLigand( at, nOldCompNumber, bMetal, elnumber_Heteroat,
|
2055
|
+
num_halogens, num_atoms, i, j, bTautFlagsDone );
|
2056
|
+
}
|
2057
|
+
}
|
2058
|
+
}
|
2059
|
+
/* disconnect metal-metal bonds */
|
2060
|
+
for ( i = 0; i < num_atoms; i ++ ) {
|
2061
|
+
if ( !bMetal[i] ) {
|
2062
|
+
continue;
|
2063
|
+
}
|
2064
|
+
for ( j = at[i].valence-1; 0 <= j; j -- ) {
|
2065
|
+
if ( j < at[i].valence && bMetal[ (int)at[i].neighbor[j] ] ) {
|
2066
|
+
/* break metal-metal bond here */
|
2067
|
+
num_disconnected += DisconnectOneLigand( at, nOldCompNumber, bMetal, elnumber_Heteroat,
|
2068
|
+
num_halogens, num_atoms, i, j, bTautFlagsDone );
|
2069
|
+
}
|
2070
|
+
}
|
2071
|
+
}
|
2072
|
+
|
2073
|
+
|
2074
|
+
exit_function:
|
2075
|
+
if ( !num_disconnected ) {
|
2076
|
+
err = 6;
|
2077
|
+
}
|
2078
|
+
if ( at && err ) {
|
2079
|
+
inchi_free( at );
|
2080
|
+
at = NULL;
|
2081
|
+
}
|
2082
|
+
if ( atom && at ) { /* changed if ( at ) to if ( atom && at ) 2004-04-03 */
|
2083
|
+
inchi_free( atom );
|
2084
|
+
atom = NULL;
|
2085
|
+
}
|
2086
|
+
if ( bMetal )
|
2087
|
+
inchi_free( bMetal );
|
2088
|
+
|
2089
|
+
if ( at ) {
|
2090
|
+
orig_inp_data->at = at;
|
2091
|
+
orig_inp_data->num_inp_atoms = num_at;
|
2092
|
+
}
|
2093
|
+
return err? -err : num_disconnected;
|
2094
|
+
}
|
2095
|
+
/*****************************************************************************/
|
2096
|
+
int DisconnectOneLigand( inp_ATOM *at, AT_NUMB *nOldCompNumber, S_CHAR *bMetal, char *elnumber_Heteroat,
|
2097
|
+
int num_halogens, int num_atoms, int iMetal, int jLigand, INCHI_MODE *bTautFlagsDone )
|
2098
|
+
{
|
2099
|
+
int i, j, iLigand, neigh, val;
|
2100
|
+
int metal_neigh_ord[MAXVAL], num_neigh_arom_bonds[MAXVAL];
|
2101
|
+
int num_metal_neigh, num_disconnections;
|
2102
|
+
int num_del_arom_bonds, num_tot_arom_bonds, new_charge;
|
2103
|
+
char *p;
|
2104
|
+
|
2105
|
+
iLigand = at[iMetal].neighbor[jLigand];
|
2106
|
+
num_metal_neigh = 0;
|
2107
|
+
num_disconnections = 0;
|
2108
|
+
num_del_arom_bonds = num_tot_arom_bonds = 0;
|
2109
|
+
|
2110
|
+
/* find bonds to disconnect */
|
2111
|
+
for ( i = 0; i < at[iLigand].valence; i ++ ) {
|
2112
|
+
num_neigh_arom_bonds[i] = 0;
|
2113
|
+
neigh = (int)at[iLigand].neighbor[i];
|
2114
|
+
if ( neigh < num_atoms && bMetal[ neigh ] ) {
|
2115
|
+
metal_neigh_ord[ num_metal_neigh ++ ] = i;
|
2116
|
+
if ( at[iLigand].bond_type[i] > BOND_TYPE_TRIPLE ) {
|
2117
|
+
/* aromatic bond */
|
2118
|
+
for ( j = 0; j < at[neigh].valence; j ++ ) {
|
2119
|
+
num_neigh_arom_bonds[i] += ( at[neigh].bond_type[j] > BOND_TYPE_TRIPLE );
|
2120
|
+
}
|
2121
|
+
num_del_arom_bonds ++;
|
2122
|
+
}
|
2123
|
+
}
|
2124
|
+
num_tot_arom_bonds += (at[iLigand].bond_type[i] > BOND_TYPE_TRIPLE);
|
2125
|
+
}
|
2126
|
+
/* Disconnect */
|
2127
|
+
if ( num_del_arom_bonds ) {
|
2128
|
+
/* fix chem_valence of the ligand and its neighbors in case of disconnecting arom. bonds */
|
2129
|
+
/* because in this case special care should be taken of updating at[].chem_bonds_valence */
|
2130
|
+
for ( i = 0; i < num_metal_neigh; i ++ ) {
|
2131
|
+
j = metal_neigh_ord[i];
|
2132
|
+
if ( num_neigh_arom_bonds[j] ) {
|
2133
|
+
neigh = at[iLigand].neighbor[j];
|
2134
|
+
at[neigh].chem_bonds_valence -= num_neigh_arom_bonds[j]/2 - (num_neigh_arom_bonds[j]-1)/2;
|
2135
|
+
}
|
2136
|
+
}
|
2137
|
+
at[iLigand].chem_bonds_valence -= num_tot_arom_bonds/2 - (num_tot_arom_bonds-num_del_arom_bonds)/2;
|
2138
|
+
}
|
2139
|
+
/* disconnect in reverse order, otherwise the metal_neigh_ord[i]
|
2140
|
+
becomes invalid after the first disconnection
|
2141
|
+
*/
|
2142
|
+
for ( i = num_metal_neigh-1; 0 <= i; i -- ) {
|
2143
|
+
num_disconnections += DisconnectInpAtBond( at, nOldCompNumber, iLigand, metal_neigh_ord[i] );
|
2144
|
+
}
|
2145
|
+
|
2146
|
+
/* attempt to change ligand charge to make its valence 'natural' */
|
2147
|
+
i = num_tot_arom_bonds - num_del_arom_bonds;
|
2148
|
+
if ( i && i != 2 && i != 3 ||
|
2149
|
+
at[iLigand].radical && at[iLigand].radical != RADICAL_SINGLET ||
|
2150
|
+
!(p = strchr( elnumber_Heteroat, at[iLigand].el_number ) ) ) {
|
2151
|
+
goto exit_function; /* non-standard atom */
|
2152
|
+
}
|
2153
|
+
val = at[iLigand].chem_bonds_valence + NUMH(at, iLigand);
|
2154
|
+
new_charge = MAX_ATOMS; /* impossible value */
|
2155
|
+
if ( !val ) {
|
2156
|
+
if ( p - elnumber_Heteroat < num_halogens ) {
|
2157
|
+
new_charge = -1;
|
2158
|
+
}
|
2159
|
+
} else {
|
2160
|
+
for ( i = -1; i <= 1; i ++ ) {
|
2161
|
+
if ( val == get_el_valence( at[iLigand].el_number, i, 0 ) ) {
|
2162
|
+
new_charge = i; /* found charge that fits chem. valence */
|
2163
|
+
break;
|
2164
|
+
}
|
2165
|
+
}
|
2166
|
+
}
|
2167
|
+
if ( new_charge != MAX_ATOMS ) {
|
2168
|
+
if ( (new_charge != at[iLigand].charge ||
|
2169
|
+
(at[iLigand].radical && at[iLigand].radical != RADICAL_SINGLET)) &&
|
2170
|
+
1 == num_metal_neigh ) {
|
2171
|
+
if ( 1 == new_charge && 4 == val && 2 == at[iLigand].valence &&
|
2172
|
+
4 == at[iLigand].chem_bonds_valence &&
|
2173
|
+
at[iLigand].bond_type[0] == at[iLigand].bond_type[1] ) {
|
2174
|
+
; /* do not add +1 charge to disconnected =N=, etc. 2004-10-27 */
|
2175
|
+
} else {
|
2176
|
+
if ( bTautFlagsDone && new_charge != at[iLigand].charge ) {
|
2177
|
+
*bTautFlagsDone |= TG_FLAG_MOVE_CHARGE_COORD_DONE;
|
2178
|
+
}
|
2179
|
+
at[iMetal].charge -= new_charge - at[iLigand].charge;
|
2180
|
+
at[iLigand].charge = new_charge;
|
2181
|
+
/*at[iLigand].radical = 0;*/
|
2182
|
+
}
|
2183
|
+
}
|
2184
|
+
}
|
2185
|
+
exit_function:
|
2186
|
+
return num_disconnections; /* ret;*/
|
2187
|
+
}
|
2188
|
+
|
2189
|
+
/****************************************************************************************/
|
2190
|
+
double dist3D( inp_ATOM *at1, inp_ATOM *at2 )
|
2191
|
+
{
|
2192
|
+
double dx = at1->x - at2->x;
|
2193
|
+
double dy = at1->y - at2->y;
|
2194
|
+
double dz = at1->z - at2->z;
|
2195
|
+
return sqrt( dx*dx+dy*dy+dz*dz );
|
2196
|
+
}
|
2197
|
+
/****************************************************************************************/
|
2198
|
+
#define MIN_BOND_LENGTH (1.0e-6)
|
2199
|
+
#define MIN_COS (1.0e-6)
|
2200
|
+
#define MIN_BOND_LENGTH2 (MIN_BOND_LENGTH*MIN_BOND_LENGTH)
|
2201
|
+
#define MAX_BOND_LENGTH (1.0e30)
|
2202
|
+
/****************************************************************************************/
|
2203
|
+
double GetMinDistDistribution( inp_ATOM *at, int num_at, int iat, int iat_H,
|
2204
|
+
int bInAllComponents, double min_dist[], int num_segm )
|
2205
|
+
{
|
2206
|
+
const double one_pi = 2.0*atan2(1.0 /* y */, 0.0 /* x */);
|
2207
|
+
const double two_pi = 2.0*one_pi;
|
2208
|
+
const double f_step = two_pi / num_segm;
|
2209
|
+
const double h_step = f_step/2.0;
|
2210
|
+
|
2211
|
+
int i, j, k, kk, ki, kn, n, num_bonds;
|
2212
|
+
double xi, yi, xn, yn, cross_prod_in, dot_prod_in, xni, yni, rni, tni, rmin;
|
2213
|
+
double fi, fk, fn, ft, rt, rk, ri, rn, c, ave_bond_len;
|
2214
|
+
|
2215
|
+
for ( i = 0; i < num_segm; i ++ ) {
|
2216
|
+
min_dist[i] = MAX_BOND_LENGTH; /* more than any distance */
|
2217
|
+
}
|
2218
|
+
num_bonds = 0;
|
2219
|
+
ave_bond_len = 0.0;
|
2220
|
+
for ( i = 0; i < num_at; i ++ ) {
|
2221
|
+
if ( i != iat && i != iat_H && (bInAllComponents || at[i].component == at[iat].component) ) {
|
2222
|
+
for ( j = 0; j < at[i].valence; j ++ ) {
|
2223
|
+
n = at[i].neighbor[j];
|
2224
|
+
if ( (n > i && n != iat) || n == iat_H )
|
2225
|
+
continue;
|
2226
|
+
#if( bRELEASE_VERSION != 1 && defined(_DEBUG) )
|
2227
|
+
if ( n == iat ) {
|
2228
|
+
int stop = 1; /* <BRKPT> */
|
2229
|
+
}
|
2230
|
+
#endif
|
2231
|
+
xi = at[i].x - at[iat].x; /* ri; i != iat */
|
2232
|
+
yi = at[i].y - at[iat].y;
|
2233
|
+
xn = at[n].x - at[iat].x; /* rn; possibly n == iat */
|
2234
|
+
yn = at[n].y - at[iat].y;
|
2235
|
+
cross_prod_in = xi*yn - xn*yi; /* ((r(i)-r(iat)) x (r(n)-r(iat)) */
|
2236
|
+
if ( cross_prod_in < -0.01*MIN_BOND_LENGTH2 ) {
|
2237
|
+
/* make sure the r(i)->r(n) vector is counterclockwise around at[iat] */
|
2238
|
+
swap( (char*)&xi, (char*)&xn, sizeof(xi) );
|
2239
|
+
swap( (char*)&yi, (char*)&yn, sizeof(yi) );
|
2240
|
+
cross_prod_in = -cross_prod_in;
|
2241
|
+
}
|
2242
|
+
xni = xn - xi; /* r(n)->r(i) */
|
2243
|
+
yni = yn - yi;
|
2244
|
+
rni = xni*xni + yni*yni;
|
2245
|
+
if ( rni > 0.01*MIN_BOND_LENGTH2 ) {
|
2246
|
+
/* vector length |ri->rn| is not too small */
|
2247
|
+
/* arrowhead of the vector r(t) = ri + (rn-ri)*t; 0 <= t <= 1 points to the bond ri->rn */
|
2248
|
+
/* r(tni) is perpendicular to the bond ri->rn so that min|r(t)| = r(tni) = |tni|*rni */
|
2249
|
+
tni = -(xni*xi + yni*yi)/rni;
|
2250
|
+
/* find min. distance from n-i bond to at[iat] */
|
2251
|
+
if ( tni < 0.0 ) {
|
2252
|
+
rmin = sqrt( xi*xi + yi*yi );
|
2253
|
+
} else
|
2254
|
+
if ( tni > 1.0 ) {
|
2255
|
+
rmin = sqrt( xn*xn + yn*yn );
|
2256
|
+
} else {
|
2257
|
+
rmin = sqrt(tni*tni*rni);
|
2258
|
+
}
|
2259
|
+
ave_bond_len += sqrt( rni );
|
2260
|
+
num_bonds ++;
|
2261
|
+
} else {
|
2262
|
+
/* zero length i-n bond */
|
2263
|
+
tni = 0.5; /* fake */
|
2264
|
+
rmin = sqrt( xi*xi + yi*yi ); /* arbitrarily choose one */
|
2265
|
+
}
|
2266
|
+
if ( rmin >= 0.1*MIN_BOND_LENGTH ) {
|
2267
|
+
/* at[iat] does not belong to at[i]-at[n] bond */
|
2268
|
+
int bCalc_rt = 1;
|
2269
|
+
fi = atan2( yi, xi );
|
2270
|
+
fn = (n == iat)? fi : atan2( yn, xn );
|
2271
|
+
if ( fi > fn ) {
|
2272
|
+
/* make sure fn - fi >= 0 */
|
2273
|
+
fn += two_pi;
|
2274
|
+
}
|
2275
|
+
if ( fi < 0.0 ) {
|
2276
|
+
fi += two_pi;
|
2277
|
+
fn += two_pi;
|
2278
|
+
}
|
2279
|
+
ki = (int)floor((fi+h_step)/f_step); /* cast does not match function type */
|
2280
|
+
kn = (int)floor((fn+h_step)/f_step);
|
2281
|
+
/* the bond may affect several segments */
|
2282
|
+
for ( k = ki; k <= kn; k ++ ) {
|
2283
|
+
kk = k % num_segm;
|
2284
|
+
if ( min_dist[kk] < rmin )
|
2285
|
+
continue;
|
2286
|
+
if ( bCalc_rt ) {
|
2287
|
+
if ( n == iat ) {
|
2288
|
+
ft = fi;
|
2289
|
+
rt = rmin;
|
2290
|
+
} else {
|
2291
|
+
double xt, yt;
|
2292
|
+
xt = xi + xni*tni;
|
2293
|
+
yt = yi + yni*tni;
|
2294
|
+
ft = atan2( yt, xt );
|
2295
|
+
rt = sqrt(xt*xt + yt*yt);
|
2296
|
+
}
|
2297
|
+
bCalc_rt = 0;
|
2298
|
+
}
|
2299
|
+
fk = f_step * kk;
|
2300
|
+
c = fabs(cos( fk - ft ));
|
2301
|
+
if ( c < MIN_COS )
|
2302
|
+
c = MIN_COS;
|
2303
|
+
rk = rt / c;
|
2304
|
+
if ( min_dist[kk] > rk ) {
|
2305
|
+
min_dist[kk] = rk;
|
2306
|
+
}
|
2307
|
+
}
|
2308
|
+
} else {
|
2309
|
+
/* rmin < 0.1*MIN_BOND_LENGTH */
|
2310
|
+
ri = xi*xi + yi*yi;
|
2311
|
+
rn = xn*xn + yn*yn;
|
2312
|
+
if ( ri > MIN_BOND_LENGTH2 && rn > MIN_BOND_LENGTH2 ) {
|
2313
|
+
dot_prod_in = xn*xi + yn*yi;
|
2314
|
+
/* a very short bond */
|
2315
|
+
if ( dot_prod_in > 0.01*MIN_BOND_LENGTH2 ) {
|
2316
|
+
/* bond does not cross at[iat] */
|
2317
|
+
double fyixi = atan2( yi, xi );
|
2318
|
+
if ( fyixi < 0.0 ) fyixi += two_pi;
|
2319
|
+
kk = (int)floor((fyixi+h_step)/f_step) % num_segm;
|
2320
|
+
if ( min_dist[kk] > rmin ) {
|
2321
|
+
min_dist[kk] = rmin;
|
2322
|
+
}
|
2323
|
+
} else
|
2324
|
+
if ( dot_prod_in < -0.01*MIN_BOND_LENGTH2 ) {
|
2325
|
+
/* bond does cross at[iat] */
|
2326
|
+
double fyixi = atan2( yi, xi );
|
2327
|
+
if ( fyixi < 0.0 ) fyixi += two_pi;
|
2328
|
+
kk = (int)floor((fyixi+h_step)/f_step) % num_segm;
|
2329
|
+
if ( min_dist[kk] > rmin ) {
|
2330
|
+
min_dist[kk] = rmin;
|
2331
|
+
}
|
2332
|
+
fyixi += one_pi;
|
2333
|
+
kk = (int)floor((fyixi+h_step)/f_step) % num_segm;
|
2334
|
+
if ( min_dist[kk] > rmin ) {
|
2335
|
+
min_dist[kk] = rmin;
|
2336
|
+
}
|
2337
|
+
} else {
|
2338
|
+
; /* error, should not happen */
|
2339
|
+
}
|
2340
|
+
} else
|
2341
|
+
if ( ri <= MIN_BOND_LENGTH2 && rn <= MIN_BOND_LENGTH2 ) {
|
2342
|
+
/* a very short bond coincides with at[iat]; ignore */
|
2343
|
+
;
|
2344
|
+
} else {
|
2345
|
+
/* one end of the bond coincides with at[iat] */
|
2346
|
+
fi = ri>rn? atan2( yi, xi) : atan2( yn, xn );
|
2347
|
+
if ( fi < 0.0 ) fi += two_pi;
|
2348
|
+
kk = (int)floor((fi+h_step)/f_step) % num_segm;
|
2349
|
+
if ( min_dist[kk] > rmin ) {
|
2350
|
+
min_dist[kk] = rmin;
|
2351
|
+
}
|
2352
|
+
}
|
2353
|
+
}
|
2354
|
+
}
|
2355
|
+
}
|
2356
|
+
}
|
2357
|
+
if ( num_bonds ) {
|
2358
|
+
return ave_bond_len / (double)num_bonds;
|
2359
|
+
} else {
|
2360
|
+
return 0.0;
|
2361
|
+
}
|
2362
|
+
}
|
2363
|
+
|
2364
|
+
/****************************************************************************************/
|
2365
|
+
int move_explicit_Hcation(inp_ATOM *at, int num_at, int iat, int iat_H, int bInAllComponents)
|
2366
|
+
{
|
2367
|
+
#define NUM_SEGM 20
|
2368
|
+
const double one_pi = 2.0*atan2(1.0 /* y */, 0.0 /* x */);
|
2369
|
+
const double two_pi = 2.0*one_pi;
|
2370
|
+
const double f_step = two_pi / NUM_SEGM;
|
2371
|
+
const double h_step = f_step/2.0;
|
2372
|
+
double min_dist[NUM_SEGM];
|
2373
|
+
int nB, i, k, kk, next, val;
|
2374
|
+
double r, r0, xd, yd, zd, xr, yr, zr, ave_bond_len;
|
2375
|
+
/*double step = 4.0*atan(1.0)/NUM_SEGM;*/
|
2376
|
+
/* find at[iat] neighbors coordinates */
|
2377
|
+
xd=yd=zd=0.0;
|
2378
|
+
if ( at[iat].valence ) {
|
2379
|
+
for ( i = 0, nB=0, r = 0.0; i < at[iat].valence; i ++ ) {
|
2380
|
+
next = at[iat].neighbor[i];
|
2381
|
+
xd += at[next].x;
|
2382
|
+
yd += at[next].y;
|
2383
|
+
zd += at[next].z;
|
2384
|
+
r += dist3D( at+iat, at+next );
|
2385
|
+
nB ++;
|
2386
|
+
}
|
2387
|
+
xd /= (double)nB;
|
2388
|
+
yd /= (double)nB;
|
2389
|
+
zd /= (double)nB;
|
2390
|
+
r /= (double)nB;
|
2391
|
+
r0 = sqrt((double)(xd-at[iat].x)*(xd-at[iat].x)
|
2392
|
+
+ (double)(yd-at[iat].y)*(yd-at[iat].y));
|
2393
|
+
} else {
|
2394
|
+
if ( at[iat_H].valence ) {
|
2395
|
+
r = dist3D( at+iat_H, at+ (int)at[iat_H].neighbor[0] );
|
2396
|
+
} else {
|
2397
|
+
r = 0.0;
|
2398
|
+
}
|
2399
|
+
r0 = 0.0;
|
2400
|
+
}
|
2401
|
+
ave_bond_len = GetMinDistDistribution( at, num_at, iat, iat_H, bInAllComponents, min_dist, NUM_SEGM );
|
2402
|
+
if ( r < MIN_BOND_LENGTH && ave_bond_len > MIN_BOND_LENGTH ) {
|
2403
|
+
r = ave_bond_len; /* ave_bond_len = 0.0 may mean that it is 0D structure */
|
2404
|
+
}
|
2405
|
+
if ( r > MIN_BOND_LENGTH ) {
|
2406
|
+
/* process non-zero bond lengths */
|
2407
|
+
double f;
|
2408
|
+
if ( 10.0*r0 < r ) {
|
2409
|
+
xr = -r; /* arbitrary */
|
2410
|
+
yr = 0.0;
|
2411
|
+
zr = 0.0;
|
2412
|
+
} else {
|
2413
|
+
/*
|
2414
|
+
if ( r0 < MIN_BOND_LENGTH ) {
|
2415
|
+
r0 = 1.0;
|
2416
|
+
}
|
2417
|
+
*/
|
2418
|
+
xr = r * ( at[iat].x - xd )/r0;
|
2419
|
+
yr = r * ( at[iat].y - yd )/r0; /* length = r */
|
2420
|
+
zr = r * ( at[iat].z - zd )/r0;
|
2421
|
+
|
2422
|
+
/* -- test: opposire direction --
|
2423
|
+
xr = -r * ( at[iat].x - xd )/r0;
|
2424
|
+
yr = -r * ( at[iat].y - yd )/r0;
|
2425
|
+
zr = -r * ( at[iat].z - zd )/r0;
|
2426
|
+
*/
|
2427
|
+
if ( xr*xr + yr*yr < 0.04*r*r ) {
|
2428
|
+
xr = -r;
|
2429
|
+
yr = 0.0;
|
2430
|
+
}
|
2431
|
+
}
|
2432
|
+
r = sqrt( xr*xr + yr*yr );
|
2433
|
+
f = atan2( yr, xr );
|
2434
|
+
|
2435
|
+
if ( f < 0.0 )
|
2436
|
+
f += two_pi;
|
2437
|
+
|
2438
|
+
|
2439
|
+
|
2440
|
+
kk = (int)floor((f+h_step)/f_step) % NUM_SEGM; /* cast does not match function type by design */
|
2441
|
+
if ( min_dist[kk] < 1.5* r ) {
|
2442
|
+
double dist = 1.5*r;
|
2443
|
+
int start=-1, len=0, start_max=-1, len_max=0;
|
2444
|
+
again:
|
2445
|
+
/* look for longest kk interval with min_dist[kk] >= dist */
|
2446
|
+
for ( k = 0, start = 0, len = 0, len_max = 0; k < 2*NUM_SEGM; k ++ ) {
|
2447
|
+
kk = k % NUM_SEGM;
|
2448
|
+
if ( min_dist[kk] >= dist ) {
|
2449
|
+
if ( !len ++) {
|
2450
|
+
start = k;
|
2451
|
+
}
|
2452
|
+
} else {
|
2453
|
+
if ( len > len_max ) {
|
2454
|
+
len_max = len;
|
2455
|
+
start_max = start;
|
2456
|
+
}
|
2457
|
+
len = 0;
|
2458
|
+
}
|
2459
|
+
}
|
2460
|
+
if ( !len_max ) {
|
2461
|
+
if ( dist > 0.1*r ) {
|
2462
|
+
dist *= 0.75;
|
2463
|
+
goto again;
|
2464
|
+
} else {
|
2465
|
+
goto done; /* do it anyway */
|
2466
|
+
}
|
2467
|
+
} else {
|
2468
|
+
/* found a good sector */
|
2469
|
+
f = f_step * (start_max + (double)(len_max - 1)/2.0);
|
2470
|
+
r0 = dist / 1.5;
|
2471
|
+
xr = r0 * cos(f);
|
2472
|
+
yr = r0 * sin(f);
|
2473
|
+
zr = zr/r*r0;
|
2474
|
+
}
|
2475
|
+
}
|
2476
|
+
} else {
|
2477
|
+
xr = yr = zr = 0;
|
2478
|
+
}
|
2479
|
+
|
2480
|
+
done:
|
2481
|
+
|
2482
|
+
if ( at[iat_H].valence ) {
|
2483
|
+
/* disconnect H */
|
2484
|
+
next = at[iat_H].neighbor[0];
|
2485
|
+
for ( i = 0; i < at[next].valence; i ++ ) {
|
2486
|
+
if ( at[next].neighbor[i] == iat_H ) {
|
2487
|
+
RemoveInpAtBond( at, next, i );
|
2488
|
+
i = 0; /* success */
|
2489
|
+
break;
|
2490
|
+
}
|
2491
|
+
}
|
2492
|
+
} else {
|
2493
|
+
/* isolated H+ cation */
|
2494
|
+
next = iat_H;
|
2495
|
+
i = 0;
|
2496
|
+
at[iat_H].valence = 1;
|
2497
|
+
at[iat_H].chem_bonds_valence = 1;
|
2498
|
+
at[iat_H].bond_type[0] = BOND_TYPE_SINGLE;
|
2499
|
+
}
|
2500
|
+
if ( 0 == i /*i < at[next].valence*/ ) {
|
2501
|
+
/* move charge */
|
2502
|
+
if ( at[next].charge > 0 && at[iat].charge < 0 ) {
|
2503
|
+
at[next].charge --;
|
2504
|
+
at[iat].charge ++;
|
2505
|
+
}
|
2506
|
+
/* connect H to at[iat] */
|
2507
|
+
val = at[iat].valence;
|
2508
|
+
at[iat].neighbor[val] = iat_H;
|
2509
|
+
at[iat].bond_type[val] = at[iat_H].bond_type[0];
|
2510
|
+
at[iat].bond_stereo[val] = 0;
|
2511
|
+
at[iat].chem_bonds_valence += at[iat_H].bond_type[0];
|
2512
|
+
at[iat].valence = val+1;
|
2513
|
+
|
2514
|
+
at[iat_H].component = at[iat].component;
|
2515
|
+
at[iat_H].neighbor[0] = iat;
|
2516
|
+
at[iat_H].bond_stereo[0] = 0; /* possible loss of stereo info */
|
2517
|
+
at[iat_H].x = at[iat].x + xr;
|
2518
|
+
at[iat_H].y = at[iat].y + yr;
|
2519
|
+
at[iat_H].z = at[iat].z + zr;
|
2520
|
+
return 1; /* success */
|
2521
|
+
}
|
2522
|
+
return 0; /* failed */
|
2523
|
+
}
|
2524
|
+
/****************************************************************************************/
|
2525
|
+
int get_iat_number( int el_number, const int el_num[], int el_num_len )
|
2526
|
+
{
|
2527
|
+
int i;
|
2528
|
+
for ( i = 0; i < el_num_len; i ++ ) {
|
2529
|
+
if ( el_num[i] == el_number )
|
2530
|
+
return i;
|
2531
|
+
}
|
2532
|
+
return -1;
|
2533
|
+
}
|
2534
|
+
|
2535
|
+
|
2536
|
+
/*#endif*/ /* } DISCONNECT_SALTS */
|
2537
|
+
typedef enum tagIonAtomType {
|
2538
|
+
IAT_H=0,
|
2539
|
+
IAT_C,
|
2540
|
+
IAT_N,
|
2541
|
+
IAT_P,
|
2542
|
+
IAT_O,
|
2543
|
+
IAT_S,
|
2544
|
+
IAT_Se,
|
2545
|
+
IAT_Te,
|
2546
|
+
IAT_F,
|
2547
|
+
IAT_Cl,
|
2548
|
+
IAT_Br,
|
2549
|
+
IAT_I,
|
2550
|
+
IAT_MAX
|
2551
|
+
} ION_ATOM_TYPE;
|
2552
|
+
|
2553
|
+
/****************************************************************************************/
|
2554
|
+
int bNumHeterAtomHasIsotopicH( inp_ATOM *atom, int num_atoms )
|
2555
|
+
{
|
2556
|
+
static int el_num[IAT_MAX];
|
2557
|
+
int i, j, val, is_O=0, is_Cl=0, is_N=0, is_H=0, num_H, iat_numb, bAccept, num_iso_H, cur_num_iso_H, num_iso_atoms;
|
2558
|
+
inp_ATOM *at, *at2;
|
2559
|
+
/* one time initialization */
|
2560
|
+
if ( !el_num[IAT_H]) {
|
2561
|
+
el_num[IAT_H ] = get_periodic_table_number( "H" );
|
2562
|
+
el_num[IAT_C ] = get_periodic_table_number( "C" );
|
2563
|
+
el_num[IAT_N ] = get_periodic_table_number( "N" );
|
2564
|
+
el_num[IAT_P ] = get_periodic_table_number( "P" );
|
2565
|
+
el_num[IAT_O ] = get_periodic_table_number( "O" );
|
2566
|
+
el_num[IAT_S ] = get_periodic_table_number( "S" );
|
2567
|
+
el_num[IAT_Se] = get_periodic_table_number( "Se");
|
2568
|
+
el_num[IAT_Te] = get_periodic_table_number( "Te");
|
2569
|
+
el_num[IAT_F ] = get_periodic_table_number( "F" );
|
2570
|
+
el_num[IAT_Cl] = get_periodic_table_number( "Cl");
|
2571
|
+
el_num[IAT_Br] = get_periodic_table_number( "Br");
|
2572
|
+
el_num[IAT_I ] = get_periodic_table_number( "I" );
|
2573
|
+
}
|
2574
|
+
num_iso_H = 0;
|
2575
|
+
num_iso_atoms = 0;
|
2576
|
+
for ( i = 0, at = atom; i < num_atoms; i ++, at ++ ) {
|
2577
|
+
|
2578
|
+
num_iso_atoms += ( at->iso_atw_diff != 0 || NUM_ISO_H(at,0) ); /* isotopic atoms and implicit isotopic H */
|
2579
|
+
|
2580
|
+
if ( 0 > (iat_numb = get_iat_number( at->el_number, el_num, IAT_MAX )) ) {
|
2581
|
+
continue;
|
2582
|
+
}
|
2583
|
+
|
2584
|
+
if ( abs(at->charge) > 1 || at->radical && RADICAL_SINGLET != at->radical ) {
|
2585
|
+
continue;
|
2586
|
+
}
|
2587
|
+
|
2588
|
+
val = -1;
|
2589
|
+
switch( iat_numb ) {
|
2590
|
+
case IAT_N:
|
2591
|
+
case IAT_P:
|
2592
|
+
is_N = 1;
|
2593
|
+
val = 3+at->charge;
|
2594
|
+
break;
|
2595
|
+
case IAT_O:
|
2596
|
+
case IAT_S:
|
2597
|
+
case IAT_Se:
|
2598
|
+
case IAT_Te:
|
2599
|
+
is_O = 1;
|
2600
|
+
val = 2+at->charge;
|
2601
|
+
break;
|
2602
|
+
case IAT_F:
|
2603
|
+
case IAT_Cl:
|
2604
|
+
case IAT_Br:
|
2605
|
+
case IAT_I:
|
2606
|
+
if ( at->charge == 0 ) {
|
2607
|
+
is_Cl = 1; /* isolated HCl */
|
2608
|
+
val = 1;
|
2609
|
+
}
|
2610
|
+
break;
|
2611
|
+
case IAT_H:
|
2612
|
+
if ( at->valence == 0 &&
|
2613
|
+
at->charge == 1 ) {
|
2614
|
+
is_H = 1; /* isolated proton */
|
2615
|
+
val = 0;
|
2616
|
+
}
|
2617
|
+
}
|
2618
|
+
if ( val < 0 ) {
|
2619
|
+
continue;
|
2620
|
+
}
|
2621
|
+
num_H = NUMH(at,0);
|
2622
|
+
if ( val != at->chem_bonds_valence + num_H ) {
|
2623
|
+
continue;
|
2624
|
+
}
|
2625
|
+
if ( is_H ) {
|
2626
|
+
bAccept = 1;
|
2627
|
+
cur_num_iso_H = (at->iso_atw_diff != 0);
|
2628
|
+
} else {
|
2629
|
+
cur_num_iso_H = 0;
|
2630
|
+
for ( j = 0, bAccept = 1; j < at->valence && bAccept; j ++ ) {
|
2631
|
+
at2 = atom + (int)at->neighbor[j];
|
2632
|
+
if ( at2->charge && at->charge || (at2->radical && RADICAL_SINGLET != at2->radical ) ) {
|
2633
|
+
bAccept = 0; /* adjacent charged/radical atoms: do not neutralizate */
|
2634
|
+
break;
|
2635
|
+
} else
|
2636
|
+
if ( at2->el_number == el_num[IAT_H ] && at2->valence == 1 && at2->iso_atw_diff ) {
|
2637
|
+
cur_num_iso_H ++; /* isotopic explicit H */
|
2638
|
+
}
|
2639
|
+
}
|
2640
|
+
if ( bAccept ) {
|
2641
|
+
num_iso_atoms -= cur_num_iso_H; /* avoid counting explicit H as isotopic atom */
|
2642
|
+
cur_num_iso_H += NUM_ISO_H(at,0);
|
2643
|
+
}
|
2644
|
+
|
2645
|
+
}
|
2646
|
+
num_iso_H += (bAccept && cur_num_iso_H); /* number of acceptable heteroatoms that have isotopic H */
|
2647
|
+
}
|
2648
|
+
return ((num_iso_H? 1:0) | (num_iso_atoms? 2:0));
|
2649
|
+
}
|
2650
|
+
|
2651
|
+
|
2652
|
+
/****************************************************/
|
2653
|
+
/* Mark and count disconnected structure components */
|
2654
|
+
/* by Depth-first searching each component */
|
2655
|
+
/****************************************************/
|
2656
|
+
int cmp_components( const void *a1, const void *a2 )
|
2657
|
+
{
|
2658
|
+
int ret;
|
2659
|
+
AT_NUMB n1;
|
2660
|
+
AT_NUMB n2;
|
2661
|
+
|
2662
|
+
n1 = ((const AT_NUMB *)a1)[0]; /* number of atoms in the component -- descending order */
|
2663
|
+
n2 = ((const AT_NUMB *)a2)[0];
|
2664
|
+
if ( ret = (int)n2 - (int)n1 ) {
|
2665
|
+
return ret;
|
2666
|
+
}
|
2667
|
+
/* stable sort */
|
2668
|
+
n1 = ((const AT_NUMB *)a1)[1]; /* component ordering number -- ascending order */
|
2669
|
+
n2 = ((const AT_NUMB *)a2)[1];
|
2670
|
+
ret = (int)n1 - (int)n2;
|
2671
|
+
|
2672
|
+
return ret;
|
2673
|
+
|
2674
|
+
}
|
2675
|
+
/*************************************************************************************************/
|
2676
|
+
int mark_one_struct_component( inp_ATOM* at, int j, AT_NUMB *mark, AT_NUMB num_disconnected_components )
|
2677
|
+
{
|
2678
|
+
if ( mark[j] ) {
|
2679
|
+
return 0;
|
2680
|
+
} else {
|
2681
|
+
int i;
|
2682
|
+
mark[j] = num_disconnected_components;
|
2683
|
+
for ( i = 0; i < at[j].valence; i++ ) {
|
2684
|
+
if ( !mark[(int)at[j].neighbor[i]] ) {
|
2685
|
+
mark_one_struct_component( at, (int)at[j].neighbor[i], mark, num_disconnected_components );
|
2686
|
+
}
|
2687
|
+
}
|
2688
|
+
}
|
2689
|
+
return 1;
|
2690
|
+
}
|
2691
|
+
/*************************************************************************************************/
|
2692
|
+
int MarkDisconnectedComponents( ORIG_ATOM_DATA *orig_at_data, int bProcessOldCompNumbers )
|
2693
|
+
{
|
2694
|
+
typedef AT_NUMB AT_TRIPLE[3];
|
2695
|
+
|
2696
|
+
inp_ATOM *at = orig_at_data->at;
|
2697
|
+
int num_at = orig_at_data->num_inp_atoms;
|
2698
|
+
AT_NUMB *nCurAtLen = NULL;
|
2699
|
+
AT_NUMB *nNewCompNumber = NULL;
|
2700
|
+
AT_NUMB *nOldCompNumber = NULL;
|
2701
|
+
int i, j, num_components, ret;
|
2702
|
+
int new_comp_no;
|
2703
|
+
AT_NUMB old_comp_no, another_comp_no, no_component;
|
2704
|
+
|
2705
|
+
/* component_nbr[i][0] = number of atoms in the component i-1
|
2706
|
+
* component_nbr[i][1] = original component number (id-1) = i
|
2707
|
+
* after sorting:
|
2708
|
+
* component_nbr[j][2] = new number of component #(component_nbr[i][1]+1)
|
2709
|
+
*/
|
2710
|
+
AT_TRIPLE *component_nbr = NULL;
|
2711
|
+
|
2712
|
+
/* initialize */
|
2713
|
+
if ( bProcessOldCompNumbers && !orig_at_data->nOldCompNumber ) {
|
2714
|
+
bProcessOldCompNumbers = 0;
|
2715
|
+
}
|
2716
|
+
/*
|
2717
|
+
for ( j = 0; j < num_at; j ++ ) {
|
2718
|
+
at[j].component = 0;
|
2719
|
+
}
|
2720
|
+
*/
|
2721
|
+
ret = -1;
|
2722
|
+
if ( !num_at ) {
|
2723
|
+
return 0;
|
2724
|
+
}
|
2725
|
+
if ( !( nNewCompNumber = (AT_NUMB *) inchi_calloc( num_at, sizeof(nNewCompNumber[0]) ) ) ) {
|
2726
|
+
goto exit_function;
|
2727
|
+
}
|
2728
|
+
/* mark and count */
|
2729
|
+
for ( j = 0, num_components = 0; j < num_at; j++ ) {
|
2730
|
+
if ( !nNewCompNumber[j] ) {
|
2731
|
+
/* nNewCompNumber[i] will contain new component number for atom at[i], i=0..num_at-1 */
|
2732
|
+
mark_one_struct_component( at, j, nNewCompNumber, (AT_NUMB)(num_components+1) );
|
2733
|
+
num_components ++;
|
2734
|
+
}
|
2735
|
+
}
|
2736
|
+
/* Allocate more memory */
|
2737
|
+
i = inchi_max( num_components, orig_at_data->num_components );
|
2738
|
+
if ( !(nCurAtLen = (AT_NUMB *) inchi_calloc( num_components+1, sizeof(nCurAtLen[0]) ) ) ||
|
2739
|
+
!(nOldCompNumber = (AT_NUMB *) inchi_calloc( i +1, sizeof(nOldCompNumber[0]) ) ) ||
|
2740
|
+
!(component_nbr = (AT_TRIPLE *) inchi_calloc( num_components+1, sizeof(component_nbr[0]) ) ) ) {
|
2741
|
+
goto exit_function;
|
2742
|
+
}
|
2743
|
+
|
2744
|
+
/* count atoms per component and renumber the components */
|
2745
|
+
for ( i = 0; i < num_components; i ++ ) {
|
2746
|
+
component_nbr[i][0] = 0; /* number of atoms in the component */
|
2747
|
+
component_nbr[i][1] = i; /* component ordering number */
|
2748
|
+
}
|
2749
|
+
for ( j = 0; j < num_at; j ++ ) {
|
2750
|
+
component_nbr[(int)nNewCompNumber[j]-1][0] ++; /* count atoms in each component */
|
2751
|
+
}
|
2752
|
+
/* sort key: number of atoms; order: descending */
|
2753
|
+
qsort( (void*)component_nbr[0], num_components,
|
2754
|
+
sizeof(component_nbr[0]), cmp_components);
|
2755
|
+
/* invert the transposition */
|
2756
|
+
for ( i = 0; i < num_components; i ++ ) {
|
2757
|
+
nCurAtLen[i] = component_nbr[i][0];
|
2758
|
+
component_nbr[ component_nbr[i][1] ][2] = i+1;
|
2759
|
+
}
|
2760
|
+
/* renumber the components so that the component with the greatest number of atoms is the first */
|
2761
|
+
no_component = num_at+1;
|
2762
|
+
for ( j = 0; j < num_at; j ++ ) {
|
2763
|
+
/* new component number for at[j] */
|
2764
|
+
new_comp_no = component_nbr[(int)nNewCompNumber[j]-1][2]-1; /* starts from 0 */
|
2765
|
+
if ( bProcessOldCompNumbers ) {
|
2766
|
+
/* old component number for at[j] */
|
2767
|
+
old_comp_no = at[j].component;
|
2768
|
+
/* fill out nOldCompNumber[]; initially it contains zeroes */
|
2769
|
+
if ( !old_comp_no ) {
|
2770
|
+
nOldCompNumber[new_comp_no] = no_component; /* atom did not have component number */
|
2771
|
+
} else
|
2772
|
+
if ( nOldCompNumber[new_comp_no] != old_comp_no ) {
|
2773
|
+
if ( !nOldCompNumber[new_comp_no] ) {
|
2774
|
+
nOldCompNumber[new_comp_no] = old_comp_no;
|
2775
|
+
} else {
|
2776
|
+
/* at[j] moved from old comp #old_comp_no to old comp #nOldCompNumber[new_comp_no]
|
2777
|
+
Both components cannot be equal to any current component */
|
2778
|
+
another_comp_no = nOldCompNumber[new_comp_no];
|
2779
|
+
for ( i = 0; i < num_components; i ++ ) {
|
2780
|
+
if ( nOldCompNumber[i] == old_comp_no ||
|
2781
|
+
nOldCompNumber[i] == another_comp_no ) {
|
2782
|
+
nOldCompNumber[i] = no_component;
|
2783
|
+
}
|
2784
|
+
}
|
2785
|
+
/* nOldCompNumber[new_comp_no] = num_at+1; */
|
2786
|
+
}
|
2787
|
+
}
|
2788
|
+
}
|
2789
|
+
/* orig_at_data->nOldCompNumber */
|
2790
|
+
at[j].component = new_comp_no+1; /* starts from 1 */
|
2791
|
+
}
|
2792
|
+
if ( bProcessOldCompNumbers ) {
|
2793
|
+
for ( j = 0; j < num_components; j ++ ) {
|
2794
|
+
if ( nOldCompNumber[j] == no_component ) {
|
2795
|
+
/* the component has atom from another component */
|
2796
|
+
nOldCompNumber[j] = 0;
|
2797
|
+
} else
|
2798
|
+
if ( nOldCompNumber[j] &&
|
2799
|
+
!orig_at_data->nOldCompNumber[nOldCompNumber[j]-1] ) {
|
2800
|
+
/* the component has changed in the previous processing */
|
2801
|
+
nOldCompNumber[j] = 0;
|
2802
|
+
}
|
2803
|
+
}
|
2804
|
+
} else {
|
2805
|
+
for ( j = 0; j < num_components; j ++ ) {
|
2806
|
+
nOldCompNumber[j] = j + 1;
|
2807
|
+
}
|
2808
|
+
}
|
2809
|
+
ret = num_components;
|
2810
|
+
exit_function:
|
2811
|
+
if ( nNewCompNumber )
|
2812
|
+
inchi_free( nNewCompNumber );
|
2813
|
+
if ( component_nbr )
|
2814
|
+
inchi_free( component_nbr );
|
2815
|
+
|
2816
|
+
if ( ret < 0 ) {
|
2817
|
+
if ( nCurAtLen ) {
|
2818
|
+
inchi_free( nCurAtLen );
|
2819
|
+
nCurAtLen = NULL;
|
2820
|
+
}
|
2821
|
+
if ( nOldCompNumber ) {
|
2822
|
+
inchi_free( nOldCompNumber );
|
2823
|
+
nOldCompNumber = NULL;
|
2824
|
+
}
|
2825
|
+
num_components = ret;
|
2826
|
+
}
|
2827
|
+
/* avoid memory leaks */
|
2828
|
+
if ( orig_at_data->nCurAtLen )
|
2829
|
+
inchi_free ( orig_at_data->nCurAtLen );
|
2830
|
+
if ( orig_at_data->nOldCompNumber )
|
2831
|
+
inchi_free ( orig_at_data->nOldCompNumber );
|
2832
|
+
|
2833
|
+
orig_at_data->nCurAtLen = nCurAtLen;
|
2834
|
+
orig_at_data->nOldCompNumber = nOldCompNumber;
|
2835
|
+
|
2836
|
+
orig_at_data->num_components = num_components;
|
2837
|
+
|
2838
|
+
return num_components; /* number of disconnected components; 1=>single connected structure*/
|
2839
|
+
}
|
2840
|
+
/******************************************************************************/
|
2841
|
+
/* Extract one (connected) component */
|
2842
|
+
/******************************************************************************/
|
2843
|
+
int ExtractConnectedComponent( inp_ATOM *at, int num_at, int component_number, inp_ATOM *component_at )
|
2844
|
+
{
|
2845
|
+
int i, j, num_component_at;
|
2846
|
+
AT_NUMB *number;
|
2847
|
+
if ( NULL == (number = (AT_NUMB*)inchi_calloc(num_at, sizeof(AT_NUMB)))){
|
2848
|
+
return CT_OUT_OF_RAM; /* out of memory */ /* <BRKPT> */
|
2849
|
+
}
|
2850
|
+
/* copy atoms */
|
2851
|
+
for ( i = 0, num_component_at = 0; i < num_at; i ++ ) {
|
2852
|
+
if ( at[i].component == component_number ) {
|
2853
|
+
number[i] = num_component_at;
|
2854
|
+
component_at[num_component_at ++] = at[i];
|
2855
|
+
}
|
2856
|
+
}
|
2857
|
+
/* renumber neighbors */
|
2858
|
+
for ( i = 0; i < num_component_at; i ++ ) {
|
2859
|
+
component_at[i].orig_compt_at_numb = (AT_NUMB)(i + 1);
|
2860
|
+
for ( j = 0; j < component_at[i].valence; j ++ ) {
|
2861
|
+
component_at[i].neighbor[j] = number[(int)component_at[i].neighbor[j]];
|
2862
|
+
}
|
2863
|
+
}
|
2864
|
+
inchi_free( number );
|
2865
|
+
return num_component_at;
|
2866
|
+
}
|
2867
|
+
/****************************************************************/
|
2868
|
+
int SetConnectedComponentNumber( inp_ATOM *at, int num_at, int component_number )
|
2869
|
+
{
|
2870
|
+
int i;
|
2871
|
+
for ( i = 0; i < num_at; i ++ ) {
|
2872
|
+
at[i].component = (AT_NUMB)component_number;
|
2873
|
+
}
|
2874
|
+
return 0;
|
2875
|
+
}
|
2876
|
+
/****************************************************************/
|
2877
|
+
|
2878
|
+
int Free_INChI_Stereo( INChI_Stereo *pINChI_Stereo )
|
2879
|
+
{
|
2880
|
+
if ( pINChI_Stereo ) {
|
2881
|
+
qzfree( pINChI_Stereo->nNumber );
|
2882
|
+
qzfree( pINChI_Stereo->t_parity );
|
2883
|
+
qzfree( pINChI_Stereo->nNumberInv );
|
2884
|
+
qzfree( pINChI_Stereo->t_parityInv );
|
2885
|
+
qzfree( pINChI_Stereo->nBondAtom1 );
|
2886
|
+
qzfree( pINChI_Stereo->nBondAtom2 );
|
2887
|
+
qzfree( pINChI_Stereo->b_parity );
|
2888
|
+
}
|
2889
|
+
return 0;
|
2890
|
+
}
|
2891
|
+
|
2892
|
+
/****************************************************************/
|
2893
|
+
INChI_Stereo *Alloc_INChI_Stereo(int num_at, int num_bonds)
|
2894
|
+
{
|
2895
|
+
INChI_Stereo *pINChI_Stereo = (INChI_Stereo *)inchi_calloc(1, sizeof(INChI_Stereo));
|
2896
|
+
if ( pINChI_Stereo ) {
|
2897
|
+
if ( num_at &&
|
2898
|
+
(pINChI_Stereo->nNumber = (AT_NUMB *)inchi_calloc(num_at, sizeof(pINChI_Stereo->nNumber[0]))) &&
|
2899
|
+
(pINChI_Stereo->t_parity = (S_CHAR *)inchi_calloc(num_at, sizeof(pINChI_Stereo->t_parity[0])))
|
2900
|
+
&& (pINChI_Stereo->nNumberInv = (AT_NUMB *)inchi_calloc(num_at, sizeof(pINChI_Stereo->nNumberInv[0])))
|
2901
|
+
&& (pINChI_Stereo->t_parityInv = (S_CHAR *)inchi_calloc(num_at, sizeof(pINChI_Stereo->t_parityInv[0])))
|
2902
|
+
) {
|
2903
|
+
;
|
2904
|
+
} else
|
2905
|
+
if ( num_at ) {
|
2906
|
+
goto out_of_RAM;
|
2907
|
+
}
|
2908
|
+
if ( num_bonds &&
|
2909
|
+
(pINChI_Stereo->nBondAtom1 =(AT_NUMB *)inchi_calloc(num_bonds, sizeof(pINChI_Stereo->nBondAtom1[0]))) &&
|
2910
|
+
(pINChI_Stereo->nBondAtom2 =(AT_NUMB *)inchi_calloc(num_bonds, sizeof(pINChI_Stereo->nBondAtom2[0]))) &&
|
2911
|
+
(pINChI_Stereo->b_parity =(S_CHAR *)inchi_calloc(num_bonds, sizeof(pINChI_Stereo->b_parity[0]))) ) {
|
2912
|
+
;
|
2913
|
+
} else
|
2914
|
+
if ( num_bonds ) {
|
2915
|
+
goto out_of_RAM;
|
2916
|
+
}
|
2917
|
+
return pINChI_Stereo;
|
2918
|
+
|
2919
|
+
out_of_RAM:
|
2920
|
+
Free_INChI_Stereo( pINChI_Stereo );
|
2921
|
+
qzfree( pINChI_Stereo );
|
2922
|
+
}
|
2923
|
+
return NULL;
|
2924
|
+
}
|
2925
|
+
/****************************************************************/
|
2926
|
+
int Free_INChI(INChI **ppINChI)
|
2927
|
+
{
|
2928
|
+
INChI *pINChI;
|
2929
|
+
|
2930
|
+
if ( pINChI = *ppINChI ) {
|
2931
|
+
#if( bREUSE_INCHI == 1 )
|
2932
|
+
if ( pINChI->nRefCount -- > 0 )
|
2933
|
+
return 1;
|
2934
|
+
#endif
|
2935
|
+
|
2936
|
+
Free_INChI_Stereo(pINChI->Stereo );
|
2937
|
+
Free_INChI_Stereo(pINChI->StereoIsotopic );
|
2938
|
+
/*
|
2939
|
+
Free_INChI_Stereo(pINChI->StereoInv );
|
2940
|
+
Free_INChI_Stereo(pINChI->StereoIsotopicInv);
|
2941
|
+
*/
|
2942
|
+
qzfree(pINChI->nAtom );
|
2943
|
+
qzfree(pINChI->nConnTable );
|
2944
|
+
qzfree(pINChI->nTautomer );
|
2945
|
+
qzfree(pINChI->nNum_H );
|
2946
|
+
qzfree(pINChI->nNum_H_fixed );
|
2947
|
+
qzfree(pINChI->IsotopicAtom );
|
2948
|
+
qzfree(pINChI->IsotopicTGroup );
|
2949
|
+
qzfree(pINChI->nPossibleLocationsOfIsotopicH);
|
2950
|
+
qzfree(pINChI->Stereo );
|
2951
|
+
qzfree(pINChI->StereoIsotopic );
|
2952
|
+
/*
|
2953
|
+
qzfree(pINChI->StereoInv );
|
2954
|
+
qzfree(pINChI->StereoIsotopicInv);
|
2955
|
+
*/
|
2956
|
+
qzfree(pINChI->szHillFormula );
|
2957
|
+
/*
|
2958
|
+
pINChI->nAtom = NULL;
|
2959
|
+
pINChI->nConnTable = NULL;
|
2960
|
+
pINChI->nTautomer = NULL;
|
2961
|
+
pINChI->nNum_H = NULL;
|
2962
|
+
pINChI->IsotopicAtom = NULL;
|
2963
|
+
pINChI->IsotopicTGroup = NULL;
|
2964
|
+
pINChI->Stereo = NULL;
|
2965
|
+
pINChI->StereoIsotopic = NULL;
|
2966
|
+
pINChI->szHillFormula = NULL;
|
2967
|
+
*/
|
2968
|
+
qzfree( pINChI );
|
2969
|
+
*ppINChI = NULL;
|
2970
|
+
|
2971
|
+
}
|
2972
|
+
return 0;
|
2973
|
+
}
|
2974
|
+
|
2975
|
+
/****************************************************************/
|
2976
|
+
INChI *Alloc_INChI( inp_ATOM *at, int num_at, int *found_num_bonds, int *found_num_isotopic, int nAllocMode )
|
2977
|
+
{
|
2978
|
+
int i, num_bonds, num_isotopic_atoms;
|
2979
|
+
INChI *pINChI;
|
2980
|
+
int bIsotopic = (nAllocMode & REQ_MODE_ISO);
|
2981
|
+
/* int bTautomeric = (nAllocMode & REQ_MODE_TAUT); */
|
2982
|
+
|
2983
|
+
if ( num_at <= 0 || NULL == (pINChI = (INChI *)inchi_calloc( 1, sizeof(INChI)))) {
|
2984
|
+
return NULL;
|
2985
|
+
}
|
2986
|
+
|
2987
|
+
for ( i = 0, num_bonds = 0, num_isotopic_atoms = 0; i < num_at; i ++ ) {
|
2988
|
+
num_bonds += at[i].valence;
|
2989
|
+
/* if ( bIsotopic ) { */
|
2990
|
+
num_isotopic_atoms += (0 != at[i].iso_atw_diff ||
|
2991
|
+
!strcmp(at[i].elname, "D") ||
|
2992
|
+
!strcmp(at[i].elname, "T") ||
|
2993
|
+
at[i].num_iso_H[0] ||
|
2994
|
+
at[i].num_iso_H[1] ||
|
2995
|
+
at[i].num_iso_H[2]);
|
2996
|
+
/* } */
|
2997
|
+
|
2998
|
+
}
|
2999
|
+
num_bonds /= 2;
|
3000
|
+
|
3001
|
+
*found_num_bonds = num_bonds;
|
3002
|
+
*found_num_isotopic = num_isotopic_atoms;
|
3003
|
+
|
3004
|
+
|
3005
|
+
if ( (pINChI->nAtom = (U_CHAR*) inchi_calloc( num_at, sizeof(pINChI->nAtom[0]))) &&
|
3006
|
+
(pINChI->nConnTable = (AT_NUMB*)inchi_calloc( num_at+num_bonds, sizeof(pINChI->nConnTable[0]))) &&
|
3007
|
+
(pINChI->nTautomer = (AT_NUMB*)inchi_calloc( ((3+INCHI_T_NUM_MOVABLE)*num_at)/2+1, sizeof(pINChI->nTautomer[0]))) &&
|
3008
|
+
(pINChI->nNum_H = (S_CHAR*) inchi_calloc( num_at, sizeof(pINChI->nNum_H[0]))) &&
|
3009
|
+
(pINChI->nNum_H_fixed= (S_CHAR*) inchi_calloc( num_at, sizeof(pINChI->nNum_H_fixed[0])))
|
3010
|
+
) {
|
3011
|
+
; /* nTautomer length: max. number of tautomeric groups is num_at/2
|
3012
|
+
|
3013
|
+
1 word -> number of t-groups
|
3014
|
+
|
3015
|
+
each group has:
|
3016
|
+
|
3017
|
+
1 word -> number of endpoints+INCHI_T_NUM_MOVABLE
|
3018
|
+
INCHI_T_NUM_MOVABLE words -> number(s) of moveable attachments
|
3019
|
+
numbers of endpoints words -> canon. numbers
|
3020
|
+
|
3021
|
+
max. occurs if each t-group has 2 atoms (num_at/2 t-groups) and all atoms
|
3022
|
+
belong to t-groups (num_at endpoints)
|
3023
|
+
|
3024
|
+
Total: 1 + (number of t-groups)*(1+INCHI_T_NUM_MOVABLE) + (number of endpoints) <=
|
3025
|
+
1 + (num_at/2) * (1+INCHI_T_NUM_MOVABLE) + num_at <=
|
3026
|
+
1 + (3+INCHI_T_NUM_MOVABLE)*num_at/2 words.
|
3027
|
+
*/
|
3028
|
+
|
3029
|
+
} else {
|
3030
|
+
goto out_of_RAM;
|
3031
|
+
}
|
3032
|
+
pINChI->szHillFormula = NULL; /* the length is unknown */
|
3033
|
+
if ( bIsotopic ) {
|
3034
|
+
if ( num_isotopic_atoms &&
|
3035
|
+
(pINChI->IsotopicAtom = (INChI_IsotopicAtom *)inchi_calloc(num_isotopic_atoms, sizeof(INChI_IsotopicAtom) )) &&
|
3036
|
+
(pINChI->IsotopicTGroup = (INChI_IsotopicTGroup *)inchi_calloc(num_isotopic_atoms, sizeof(INChI_IsotopicTGroup) ))
|
3037
|
+
) {
|
3038
|
+
;
|
3039
|
+
} else
|
3040
|
+
if ( num_isotopic_atoms ) {
|
3041
|
+
goto out_of_RAM;
|
3042
|
+
}
|
3043
|
+
if ( !(pINChI->nPossibleLocationsOfIsotopicH = (AT_NUMB *)inchi_calloc( num_at+1, sizeof(pINChI->nPossibleLocationsOfIsotopicH[0]) ) ) ) {
|
3044
|
+
goto out_of_RAM;
|
3045
|
+
}
|
3046
|
+
}
|
3047
|
+
|
3048
|
+
if ((pINChI->Stereo = Alloc_INChI_Stereo(num_at, num_bonds))
|
3049
|
+
) {
|
3050
|
+
;
|
3051
|
+
} else {
|
3052
|
+
goto out_of_RAM;
|
3053
|
+
}
|
3054
|
+
if ( bIsotopic ) {
|
3055
|
+
if ((pINChI->StereoIsotopic = Alloc_INChI_Stereo(num_at, num_bonds))
|
3056
|
+
) {
|
3057
|
+
;
|
3058
|
+
} else {
|
3059
|
+
goto out_of_RAM;
|
3060
|
+
}
|
3061
|
+
}
|
3062
|
+
return pINChI;
|
3063
|
+
|
3064
|
+
out_of_RAM:
|
3065
|
+
if ( pINChI ) {
|
3066
|
+
Free_INChI(&pINChI);
|
3067
|
+
/*
|
3068
|
+
inchi_free(pINChI);
|
3069
|
+
*/
|
3070
|
+
}
|
3071
|
+
return NULL;
|
3072
|
+
}
|
3073
|
+
/****************************************************************/
|
3074
|
+
int Free_INChI_Aux( INChI_Aux **ppINChI_Aux )
|
3075
|
+
{
|
3076
|
+
INChI_Aux *pINChI_Aux = *ppINChI_Aux;
|
3077
|
+
if ( pINChI_Aux ) {
|
3078
|
+
#if( bREUSE_INCHI == 1 )
|
3079
|
+
if ( pINChI_Aux->nRefCount -- > 0 )
|
3080
|
+
return 1;
|
3081
|
+
#endif
|
3082
|
+
|
3083
|
+
qzfree( pINChI_Aux->nOrigAtNosInCanonOrd );
|
3084
|
+
qzfree( pINChI_Aux->nIsotopicOrigAtNosInCanonOrd );
|
3085
|
+
qzfree( pINChI_Aux->nOrigAtNosInCanonOrdInv );
|
3086
|
+
qzfree( pINChI_Aux->nIsotopicOrigAtNosInCanonOrdInv );
|
3087
|
+
qzfree( pINChI_Aux->szOrigCoord );
|
3088
|
+
qzfree( pINChI_Aux->OrigInfo );
|
3089
|
+
/*
|
3090
|
+
qzfree( pINChI_Aux->nOriginalAtomNumber );
|
3091
|
+
qzfree( pINChI_Aux->nCanonicalTGroupNumbers );
|
3092
|
+
qzfree( pINChI_Aux->nIsotopicCanonicalTGroupNumbers);
|
3093
|
+
qzfree( pINChI_Aux->nTautomer );
|
3094
|
+
qzfree( pINChI_Aux->nNontautomericCanonicalNumbers );
|
3095
|
+
qzfree( pINChI_Aux->nIsotopicCanonicalNumbers );
|
3096
|
+
qzfree( pINChI_Aux->nNontautomericIsotopicCanonicalNumbers );
|
3097
|
+
qzfree( pINChI_Aux->nNontautomericEquNumbers );
|
3098
|
+
qzfree( pINChI_Aux->nNontautomericIsotopicEquNumbers );
|
3099
|
+
*/
|
3100
|
+
qzfree( pINChI_Aux->nConstitEquNumbers );
|
3101
|
+
qzfree( pINChI_Aux->nConstitEquTGroupNumbers );
|
3102
|
+
qzfree( pINChI_Aux->nConstitEquIsotopicNumbers );
|
3103
|
+
qzfree( pINChI_Aux->nConstitEquIsotopicTGroupNumbers );
|
3104
|
+
qzfree( pINChI_Aux );
|
3105
|
+
*ppINChI_Aux = NULL;
|
3106
|
+
}
|
3107
|
+
return 0;
|
3108
|
+
}
|
3109
|
+
/****************************************************************/
|
3110
|
+
INChI_Aux *Alloc_INChI_Aux( int num_at, int num_isotopic_atoms, int nAllocMode, int bOrigCoord )
|
3111
|
+
{
|
3112
|
+
INChI_Aux *pINChI_Aux;
|
3113
|
+
int bIsotopic = (nAllocMode & REQ_MODE_ISO);
|
3114
|
+
int num_at_tg = num_at + num_at/2;
|
3115
|
+
/* int bTautomeric = (nAllocMode & REQ_MODE_TAUT); */
|
3116
|
+
|
3117
|
+
if ( num_at <= 0 || NULL == (pINChI_Aux = (INChI_Aux *)inchi_calloc(sizeof(INChI_Aux), 1))) {
|
3118
|
+
return NULL;
|
3119
|
+
}
|
3120
|
+
if ( (pINChI_Aux->nOrigAtNosInCanonOrd = (AT_NUMB*)inchi_calloc(sizeof(pINChI_Aux->nOrigAtNosInCanonOrd[0]), num_at_tg)) &&
|
3121
|
+
(pINChI_Aux->nOrigAtNosInCanonOrdInv = (AT_NUMB*)inchi_calloc(sizeof(pINChI_Aux->nOrigAtNosInCanonOrd[0]), num_at_tg)) &&
|
3122
|
+
(pINChI_Aux->nConstitEquNumbers = (AT_NUMB*)inchi_calloc(sizeof(pINChI_Aux->nConstitEquNumbers[0]), num_at_tg)) ) {
|
3123
|
+
;
|
3124
|
+
} else {
|
3125
|
+
goto out_of_RAM;
|
3126
|
+
}
|
3127
|
+
|
3128
|
+
if ( num_at > 1 &&
|
3129
|
+
(pINChI_Aux->nConstitEquTGroupNumbers = (AT_NUMB*)inchi_calloc(sizeof(pINChI_Aux->nConstitEquTGroupNumbers[0]), num_at/2)) ) {
|
3130
|
+
;
|
3131
|
+
} else
|
3132
|
+
if ( num_at > 1 ) {
|
3133
|
+
goto out_of_RAM;
|
3134
|
+
}
|
3135
|
+
|
3136
|
+
if ( num_at > 0 ) {
|
3137
|
+
pINChI_Aux->OrigInfo = (ORIG_INFO *)inchi_calloc(sizeof(pINChI_Aux->OrigInfo[0]), num_at);
|
3138
|
+
if ( !pINChI_Aux->OrigInfo )
|
3139
|
+
goto out_of_RAM;
|
3140
|
+
}
|
3141
|
+
if ( bOrigCoord && num_at > 0 ) {
|
3142
|
+
pINChI_Aux->szOrigCoord = (MOL_COORD *)inchi_calloc(sizeof(pINChI_Aux->szOrigCoord[0]), num_at);
|
3143
|
+
if ( !pINChI_Aux->szOrigCoord )
|
3144
|
+
goto out_of_RAM;
|
3145
|
+
}
|
3146
|
+
if ( bIsotopic ) {
|
3147
|
+
if ( /*num_isotopic_atoms &&*/
|
3148
|
+
(pINChI_Aux->nIsotopicOrigAtNosInCanonOrd = (AT_NUMB*)inchi_calloc(sizeof(pINChI_Aux->nIsotopicOrigAtNosInCanonOrd[0]), num_at_tg)) &&
|
3149
|
+
(pINChI_Aux->nIsotopicOrigAtNosInCanonOrdInv = (AT_NUMB*)inchi_calloc(sizeof(pINChI_Aux->nIsotopicOrigAtNosInCanonOrd[0]), num_at_tg)) &&
|
3150
|
+
(pINChI_Aux->nConstitEquIsotopicNumbers = (AT_NUMB*)inchi_calloc(sizeof(pINChI_Aux->nConstitEquIsotopicNumbers[0]), num_at_tg)) ) {
|
3151
|
+
;
|
3152
|
+
} else
|
3153
|
+
if ( num_isotopic_atoms ) {
|
3154
|
+
goto out_of_RAM;
|
3155
|
+
}
|
3156
|
+
if ( /*num_isotopic_atoms && num_at > 1 &&*/
|
3157
|
+
(pINChI_Aux->nConstitEquIsotopicTGroupNumbers = (AT_NUMB*)inchi_calloc(sizeof(pINChI_Aux->nConstitEquIsotopicTGroupNumbers[0]), num_at/2)) ) {
|
3158
|
+
;
|
3159
|
+
} else
|
3160
|
+
if ( num_isotopic_atoms && num_at > 1 ) {
|
3161
|
+
goto out_of_RAM;
|
3162
|
+
}
|
3163
|
+
}
|
3164
|
+
return pINChI_Aux;
|
3165
|
+
|
3166
|
+
|
3167
|
+
out_of_RAM:
|
3168
|
+
if ( pINChI_Aux ) {
|
3169
|
+
Free_INChI_Aux(&pINChI_Aux);
|
3170
|
+
/*
|
3171
|
+
inchi_free(pINChI_Aux);
|
3172
|
+
*/
|
3173
|
+
}
|
3174
|
+
return NULL;
|
3175
|
+
}
|
3176
|
+
/***********************************************************************************/
|
3177
|
+
#define ABNORMAL_AT(i) ( at[i].charge && at[i].radical || abs(at[i].charge) > 3 || \
|
3178
|
+
( at[i].radical && at[i].radical != RADICAL_DOUBLET) || \
|
3179
|
+
at[i].iso_atw_diff && (at[i].iso_atw_diff == 1 || at[i].iso_atw_diff < -3 || at[i].iso_atw_diff > 6 ))
|
3180
|
+
#define ALIASED_AT(i) (0 < NUM_ISO_H(at, i))
|
3181
|
+
/***********************************************************************************/
|
3182
|
+
#if( TEST_RENUMB_ATOMS_SAVE_LONGEST == 1 )
|
3183
|
+
int WriteToSDfile( const INP_ATOM_DATA *inp_at_data, INCHI_FILE* fcb, const char* name, const char* comment,
|
3184
|
+
const char *szLabel, const char *szValue)
|
3185
|
+
{
|
3186
|
+
int i, j, k, num_bonds=0, ret=0;
|
3187
|
+
int bAtomNeedsAlias;
|
3188
|
+
int flag_bad_charge=0, nNumAddLines=0, nNumIso=0, nNumChargeLines=0, nNumRadicalLines=0, nNumAliasLines=0;
|
3189
|
+
/*sp_ATOM *at; */
|
3190
|
+
float fzero=0.0F;
|
3191
|
+
double x, y;
|
3192
|
+
int bNext /*, s*/;
|
3193
|
+
const inp_ATOM *at = inp_at_data->at_fixed_bonds? inp_at_data->at_fixed_bonds : inp_at_data->at;
|
3194
|
+
int num_atoms = inp_at_data->num_at;
|
3195
|
+
/*at = species->atom;*/
|
3196
|
+
|
3197
|
+
/*my_fprintf(fcb,"%ld.MOL\n",species->casno);*/
|
3198
|
+
{ /* block start */
|
3199
|
+
char strLocName[82];
|
3200
|
+
memset(strLocName, 0, sizeof(strLocName) );
|
3201
|
+
if ( name && *name ) {
|
3202
|
+
strncpy( strLocName, name, 80 );
|
3203
|
+
}
|
3204
|
+
inchi_print_nodisplay( fcb,"%s\n", strLocName );
|
3205
|
+
} /* block end */
|
3206
|
+
/**********************************************************************/
|
3207
|
+
/** **/
|
3208
|
+
/** Important: Atoms with alias cannot have charge, radical, or **/
|
3209
|
+
/** isotope differences. **/
|
3210
|
+
/** **/
|
3211
|
+
/** Atoms with alias cannot be abnormal. **/
|
3212
|
+
/** **/
|
3213
|
+
/** Abnormal atoms are atoms which need M CHG, M RAD, M ISO **/
|
3214
|
+
/** **/
|
3215
|
+
/**********************************************************************/
|
3216
|
+
|
3217
|
+
/* F10.5 F12.5 I6
|
3218
|
+
IIPPPPPPPPMMDDYYHHmmddSSssssssssssEEEEEEEEEEEERRRRRR
|
3219
|
+
my_fprintf( fcb,"NISTTRANHP09089809272D 1 1.0 0.0 %6ld\n", lEpa);*/
|
3220
|
+
inchi_print_nodisplay( fcb," -%s v%s SDfile Output \n", INCHI_NAME, INCHI_VERSION);
|
3221
|
+
/*y_fprintf(fcb, " -CPSS- 1213981200n\n");*/
|
3222
|
+
|
3223
|
+
{ /*block start*/
|
3224
|
+
char strLocName[82];
|
3225
|
+
|
3226
|
+
memset(strLocName, 0, sizeof(strLocName) );
|
3227
|
+
if ( comment && *comment ) {
|
3228
|
+
strncpy( strLocName, comment, 80 );
|
3229
|
+
}
|
3230
|
+
inchi_print_nodisplay( fcb,"%s\n", strLocName );
|
3231
|
+
} /*block end*/
|
3232
|
+
for (i=0; i< num_atoms; i++)
|
3233
|
+
num_bonds += at[i].valence;
|
3234
|
+
num_bonds /= 2;
|
3235
|
+
|
3236
|
+
/*find if we need "M CHG" and "M RAD"*/
|
3237
|
+
for (i=0, nNumAddLines = 0, nNumIso=0; i < num_atoms; i++) {
|
3238
|
+
bAtomNeedsAlias = ALIASED_AT(i); /* 5-3-99 DCh */
|
3239
|
+
nNumAddLines += !bAtomNeedsAlias && ABNORMAL_AT(i);
|
3240
|
+
nNumAliasLines += 2 * bAtomNeedsAlias;
|
3241
|
+
nNumIso += ( 0 == strcmp( at[i].elname, "D" ) || ( 0 == strcmp( at[i].elname, "T" ) ) );
|
3242
|
+
}
|
3243
|
+
|
3244
|
+
/* count additional M lines*/
|
3245
|
+
if ( nNumAddLines || nNumAliasLines ) {
|
3246
|
+
for (i=0, nNumChargeLines=0, nNumRadicalLines=0; i < num_atoms; i++) {
|
3247
|
+
nNumChargeLines += (0 != at[i].charge) && !ALIASED_AT(i);
|
3248
|
+
nNumRadicalLines += (0 != at[i].radical) && !ALIASED_AT(i);
|
3249
|
+
}
|
3250
|
+
}
|
3251
|
+
nNumChargeLines = ( nNumChargeLines + 7 ) / 8;
|
3252
|
+
nNumRadicalLines = ( nNumRadicalLines + 7 ) / 8;
|
3253
|
+
nNumIso = ( nNumIso + 7 ) / 8;
|
3254
|
+
|
3255
|
+
nNumAddLines = nNumChargeLines + nNumRadicalLines + nNumAliasLines; /* 1 for M END*/
|
3256
|
+
|
3257
|
+
if ( nNumAddLines == 0 ) {
|
3258
|
+
nNumIso = 0; /* keep isotopes description in CTable only*/
|
3259
|
+
} else {
|
3260
|
+
nNumAddLines += nNumIso+1; /* add 1 for "M END" line*/
|
3261
|
+
}
|
3262
|
+
|
3263
|
+
/* aaa bbblllfffcccsssxxxrrrpppiiimmmvvvvvv*/
|
3264
|
+
inchi_print_nodisplay(fcb,"%3d%3d 0 0 0 0 0 0 0 0%3d%s\n",num_atoms, num_bonds, nNumAddLines,nNumAddLines?" V2000":"");
|
3265
|
+
/* atoms block*/
|
3266
|
+
for (i=0; i < num_atoms; i++) {
|
3267
|
+
char elname[ATOM_EL_LEN] = "\0\0\0\0\0";
|
3268
|
+
int iso = 0;
|
3269
|
+
int charge = 0;
|
3270
|
+
int valence = 0;
|
3271
|
+
bAtomNeedsAlias = ALIASED_AT(i);
|
3272
|
+
/* isotope*/
|
3273
|
+
iso = !strcmp( at[i].elname, "D" )? 1:
|
3274
|
+
!strcmp( at[i].elname, "T" )? 2: 0;
|
3275
|
+
|
3276
|
+
if ( iso ) {
|
3277
|
+
/* deuterium or tritium*/
|
3278
|
+
strcpy ( elname, "H" );
|
3279
|
+
} else
|
3280
|
+
if ( bAtomNeedsAlias ) {
|
3281
|
+
strcpy ( elname, "C" );
|
3282
|
+
} else {
|
3283
|
+
strncpy ( elname, at[i].elname, sizeof(elname)-1 );
|
3284
|
+
}
|
3285
|
+
/*
|
3286
|
+
if ( !iso ) {
|
3287
|
+
strncpy ( elname, at[i].elname, sizeof(elname)-1 );
|
3288
|
+
} else
|
3289
|
+
if ( ALIASED_AT(i) ) {
|
3290
|
+
strcpy ( elname, "C" );
|
3291
|
+
} else {
|
3292
|
+
-- deuterium or tritium --
|
3293
|
+
strcpy ( elname, "H" );
|
3294
|
+
}
|
3295
|
+
*/
|
3296
|
+
if ( !ABNORMAL_AT(i) && !bAtomNeedsAlias ) {
|
3297
|
+
|
3298
|
+
/* Only normal atoms without alias can be here*/
|
3299
|
+
|
3300
|
+
/* charge*/
|
3301
|
+
switch ( at[i].charge ) {
|
3302
|
+
case 3: charge = 1; break;
|
3303
|
+
case 2: charge = 2; break;
|
3304
|
+
case 1: charge = 3; break;
|
3305
|
+
case -1: charge = 5; break;
|
3306
|
+
case -2: charge = 6; break;
|
3307
|
+
case -3: charge = 7; break;
|
3308
|
+
case 0: charge = 0; break;
|
3309
|
+
default: flag_bad_charge = 1; break;
|
3310
|
+
};
|
3311
|
+
/* radical*/
|
3312
|
+
if ( at[i].radical ) {
|
3313
|
+
if ( at[i].radical == RADICAL_DOUBLET ) {
|
3314
|
+
flag_bad_charge |= (charge != 0);
|
3315
|
+
charge = 4;
|
3316
|
+
} else {
|
3317
|
+
flag_bad_charge |= 2;
|
3318
|
+
}
|
3319
|
+
}
|
3320
|
+
if ( flag_bad_charge ) {
|
3321
|
+
charge = 0;
|
3322
|
+
}
|
3323
|
+
}
|
3324
|
+
|
3325
|
+
x = at[i].x;
|
3326
|
+
y = at[i].y;
|
3327
|
+
/* --- just removed --
|
3328
|
+
if ( c && c->xCoeff != 0.0 && c->yCoeff != 0.0 ) {
|
3329
|
+
x = (x - c->xShift)/c->xCoeff;
|
3330
|
+
y = (y - c->yShift)/c->yCoeff;
|
3331
|
+
} else {
|
3332
|
+
y = -y;
|
3333
|
+
}
|
3334
|
+
----------------------*/
|
3335
|
+
if( at[i].num_H > 0 ) {
|
3336
|
+
for ( j = 0, valence = 0; j < at[i].valence; j++ ) {
|
3337
|
+
switch( k = at[i].bond_type[j] ) { /* fixed valence calculation 12-23-99 DCh.*/
|
3338
|
+
case 2:
|
3339
|
+
case 3:
|
3340
|
+
valence += 2*k;
|
3341
|
+
break;
|
3342
|
+
case 4:
|
3343
|
+
valence += 3;
|
3344
|
+
break;
|
3345
|
+
default:
|
3346
|
+
valence += 2;
|
3347
|
+
}
|
3348
|
+
}
|
3349
|
+
valence = valence/2 + at[i].num_H;
|
3350
|
+
} else
|
3351
|
+
/* Added 07-09-2003 DCh*/
|
3352
|
+
if ( at[i].chem_bonds_valence > 0 && at[i].chem_bonds_valence < 15 ) {
|
3353
|
+
valence = at[i].chem_bonds_valence;
|
3354
|
+
} else
|
3355
|
+
/* Added 07-09-2003 DCh*/
|
3356
|
+
if ( !at[i].valence && !at[i].num_H && !at[i].chem_bonds_valence ) {
|
3357
|
+
valence = 15;
|
3358
|
+
}
|
3359
|
+
/*my_fprintf(fcb,"%10.4f%10.4f%10.4f %-3.3s%2d%3d 0 0 0 0 0 0 0\n",*/
|
3360
|
+
/* (float)at[i].x, (float)(-at[i].y), fzero, at[i].elname, iso, charge);*/
|
3361
|
+
/* xxxxxxyyyyyyzzzzzz aaa____ddcccsssnnnbbbvvvrrriiimmmeee */
|
3362
|
+
inchi_print_nodisplay(fcb,"%10.4f%10.4f%10.4f %-3.3s%2d%3d 0 0%3d 0 0 0 0\n",
|
3363
|
+
x, y, (double)fzero, elname, (int)iso, (int)charge, valence /* at[i].special*/);
|
3364
|
+
/* reflect image against x-axis;
|
3365
|
+
when transforming MOLfile back to STDATA in mol_to_stdata(...),
|
3366
|
+
make one more reflection to restore original orientation.
|
3367
|
+
Reason: in MS Search y-axis is directed from top to bottom,
|
3368
|
+
while in MOLfile y-axis goes from bottom to top.
|
3369
|
+
*/
|
3370
|
+
}
|
3371
|
+
bNext = 0; /* debug only*/
|
3372
|
+
|
3373
|
+
/* bonds*/
|
3374
|
+
for (i=0; i< num_atoms; i++) {
|
3375
|
+
for (j=0; j<at[i].valence; j++) {
|
3376
|
+
if (i < at[i].neighbor[j]) {
|
3377
|
+
if ( k=at[i].bond_stereo[j] ) {
|
3378
|
+
/* bond stereo */
|
3379
|
+
if ( k < 0 ) {
|
3380
|
+
/* transposition */
|
3381
|
+
inchi_print_nodisplay(fcb,"%3u%3u%3u%3u 0 0 0\n",
|
3382
|
+
(unsigned)(at[i].neighbor[j]+1), (unsigned)(i+1), (unsigned)(at[i].bond_type[j]), (unsigned)abs(k));
|
3383
|
+
} else {
|
3384
|
+
/* no transposition*/
|
3385
|
+
inchi_print_nodisplay(fcb,"%3u%3u%3u%3u 0 0 0\n",
|
3386
|
+
(unsigned)(i+1), (unsigned)(at[i].neighbor[j]+1), (unsigned)(at[i].bond_type[j]), (unsigned)abs(k));
|
3387
|
+
}
|
3388
|
+
} else {
|
3389
|
+
inchi_print_nodisplay(fcb,"%3u%3u%3u 0 0 0 0\n",
|
3390
|
+
(unsigned)(i+1), (unsigned)(at[i].neighbor[j]+1), (unsigned)(at[i].bond_type[j]));
|
3391
|
+
}
|
3392
|
+
}
|
3393
|
+
}
|
3394
|
+
}
|
3395
|
+
if ( nNumAddLines ) {
|
3396
|
+
char str_m[66], entry[10];
|
3397
|
+
int num_m;
|
3398
|
+
|
3399
|
+
/* Aliases. 5-3-99 DCh.*/
|
3400
|
+
if ( nNumAliasLines ) {
|
3401
|
+
num_m = 0;
|
3402
|
+
for (i=0; i < num_atoms; i++) {
|
3403
|
+
if ( ALIASED_AT(i) ) {
|
3404
|
+
inchi_print_nodisplay( fcb, "A %d\n", i+1 );
|
3405
|
+
num_m ++;
|
3406
|
+
strcpy( str_m, at[i].elname );
|
3407
|
+
/* Add charge to the Alias */
|
3408
|
+
if ( at[i].charge){
|
3409
|
+
strcat(str_m, at[i].charge>0? "+" : "-");
|
3410
|
+
if ( 1 < (j=abs(at[i].charge)) )
|
3411
|
+
sprintf( str_m+strlen(str_m), "%d", j );
|
3412
|
+
}
|
3413
|
+
/* Add radical to the Alias */
|
3414
|
+
for ( j = inchi_min(2,at[i].radical); 0 < j; j-- ) {
|
3415
|
+
strcat( str_m, "^" );
|
3416
|
+
}
|
3417
|
+
inchi_print_nodisplay( fcb, "%s\n", str_m );
|
3418
|
+
num_m ++;
|
3419
|
+
}
|
3420
|
+
}
|
3421
|
+
if ( num_m != nNumAliasLines ) {
|
3422
|
+
/* error in lines counting*/
|
3423
|
+
ret ++;
|
3424
|
+
}
|
3425
|
+
}
|
3426
|
+
/* charges*/
|
3427
|
+
str_m[0] = 0;
|
3428
|
+
num_m = 0;
|
3429
|
+
if ( nNumChargeLines ) {
|
3430
|
+
for (i=0; i < num_atoms; i++) {
|
3431
|
+
if ( at[i].charge && !ALIASED_AT(i) ) {
|
3432
|
+
sprintf( entry, " %3d %3d", i+1, (int)at[i].charge );
|
3433
|
+
strcat( str_m, entry );
|
3434
|
+
num_m ++;
|
3435
|
+
}
|
3436
|
+
if ( i == num_atoms-1 && num_m || num_m == 8 ) {
|
3437
|
+
inchi_print_nodisplay( fcb, "M CHG%3d%s\n", num_m, str_m );
|
3438
|
+
str_m[0] = 0;
|
3439
|
+
num_m = 0;
|
3440
|
+
}
|
3441
|
+
}
|
3442
|
+
}
|
3443
|
+
/* radicals*/
|
3444
|
+
str_m[0] = 0;
|
3445
|
+
num_m = 0;
|
3446
|
+
if ( nNumRadicalLines ) {
|
3447
|
+
for (i=0; i < num_atoms; i++) {
|
3448
|
+
if ( at[i].radical && !ALIASED_AT(i) ) {
|
3449
|
+
int radical = (at[i].radical==RADICAL_SINGLET ||
|
3450
|
+
at[i].radical==RADICAL_DOUBLET ||
|
3451
|
+
at[i].radical==RADICAL_TRIPLET)? at[i].radical : 0;
|
3452
|
+
if ( radical ) {
|
3453
|
+
sprintf( entry, " %3d %3d", i+1, radical );
|
3454
|
+
strcat( str_m, entry );
|
3455
|
+
num_m ++;
|
3456
|
+
}
|
3457
|
+
}
|
3458
|
+
if ( i == num_atoms-1 && num_m || num_m == 8 ) {
|
3459
|
+
inchi_print_nodisplay( fcb, "M RAD%3d%s\n", num_m, str_m );
|
3460
|
+
str_m[0] = 0;
|
3461
|
+
num_m = 0;
|
3462
|
+
}
|
3463
|
+
}
|
3464
|
+
}
|
3465
|
+
/* isotopes*/
|
3466
|
+
str_m[0] = 0;
|
3467
|
+
num_m = 0;
|
3468
|
+
if ( nNumIso ) {
|
3469
|
+
for (i=0; i < num_atoms; i++) {
|
3470
|
+
if ( 0 == strcmp( at[i].elname, "D" ) ) {
|
3471
|
+
sprintf( entry, " %3d %3d", i+1, 2 );
|
3472
|
+
strcat( str_m, entry );
|
3473
|
+
num_m ++;
|
3474
|
+
} else
|
3475
|
+
if ( 0 == strcmp( at[i].elname, "T" ) ) {
|
3476
|
+
sprintf( entry, " %3d %3d", i+1, 3 );
|
3477
|
+
strcat( str_m, entry );
|
3478
|
+
num_m ++;
|
3479
|
+
}
|
3480
|
+
if ( i == num_atoms-1 && num_m || num_m == 8 ) {
|
3481
|
+
inchi_print_nodisplay( fcb, "M ISO%3d%s\n", num_m, str_m );
|
3482
|
+
str_m[0] = 0;
|
3483
|
+
num_m = 0;
|
3484
|
+
}
|
3485
|
+
}
|
3486
|
+
}
|
3487
|
+
inchi_print_nodisplay( fcb, "M END\n" );
|
3488
|
+
}
|
3489
|
+
if ( szValue && szValue[0] ) {
|
3490
|
+
if ( szLabel && szLabel[0] ) {
|
3491
|
+
inchi_print_nodisplay( fcb, "> <%s>\n", szLabel );
|
3492
|
+
} else {
|
3493
|
+
inchi_print_nodisplay( fcb, "> <ID>\n" );
|
3494
|
+
}
|
3495
|
+
inchi_print_nodisplay( fcb, " %s\n\n", szValue );
|
3496
|
+
}
|
3497
|
+
inchi_print_nodisplay(fcb, "$$$$\n");
|
3498
|
+
|
3499
|
+
|
3500
|
+
return ret;
|
3501
|
+
|
3502
|
+
}
|
3503
|
+
#endif
|
3504
|
+
/***************************************************************************************************/
|
3505
|
+
int WriteOrigAtomDataToSDfile( const ORIG_ATOM_DATA *inp_at_data, INCHI_FILE* fcb, const char* name, const char* comment,
|
3506
|
+
int bChiralFlag, const char *szLabel, const char *szValue)
|
3507
|
+
{
|
3508
|
+
int i, j, k, num_bonds=0, ret=0;
|
3509
|
+
int bAtomNeedsAlias;
|
3510
|
+
int flag_bad_charge=0, nNumAddLines=0, nNumIso=0, nNumAddIso=0, nNumChargeLines=0, nNumRadicalLines=0, nNumAliasLines=0;
|
3511
|
+
/*sp_ATOM *at; */
|
3512
|
+
/* float fzero=0.0F; */
|
3513
|
+
double x, y, z;
|
3514
|
+
int bNext /*, s*/;
|
3515
|
+
const inp_ATOM *at = inp_at_data->at;
|
3516
|
+
int num_atoms = inp_at_data->num_inp_atoms;
|
3517
|
+
/*at = species->atom;*/
|
3518
|
+
|
3519
|
+
/*my_fprintf(fcb,"%ld.MOL\n",species->casno);*/
|
3520
|
+
{ /* block start */
|
3521
|
+
char strLocName[82];
|
3522
|
+
memset(strLocName, 0, sizeof(strLocName) );
|
3523
|
+
if ( name && *name ) {
|
3524
|
+
strncpy( strLocName, name, 80 );
|
3525
|
+
/* --- debug only ---
|
3526
|
+
if ( strstr( name, "#3959" ) ) {
|
3527
|
+
int stop = 1;
|
3528
|
+
}
|
3529
|
+
*/
|
3530
|
+
}
|
3531
|
+
inchi_print_nodisplay( fcb,"%s\n", strLocName );
|
3532
|
+
} /* block end */
|
3533
|
+
/**********************************************************************/
|
3534
|
+
/** **/
|
3535
|
+
/** Important: Atoms with alias cannot have charge, radical **/
|
3536
|
+
/** isotope differences are allowed **/
|
3537
|
+
/** **/
|
3538
|
+
/** Atoms with alias cannot be abnormal. **/
|
3539
|
+
/** **/
|
3540
|
+
/** Abnormal atoms are atoms which need M CHG, M RAD, M ISO **/
|
3541
|
+
/** **/
|
3542
|
+
/** Output aliased atoms if they have implicit D or T **/
|
3543
|
+
/** **/
|
3544
|
+
/**********************************************************************/
|
3545
|
+
|
3546
|
+
/* F10.5 F12.5 I6
|
3547
|
+
IIPPPPPPPPMMDDYYHHmmddSSssssssssssEEEEEEEEEEEERRRRRR
|
3548
|
+
my_fprintf( fcb,"NISTTRANHP09089809272D 1 1.0 0.0 %6ld\n", lEpa);*/
|
3549
|
+
inchi_print_nodisplay( fcb," %s v%s SDfile Output \n", INCHI_NAME, INCHI_VERSION);
|
3550
|
+
/*y_fprintf(fcb, " -CPSS- 1213981200n\n");*/
|
3551
|
+
|
3552
|
+
{ /*block start*/
|
3553
|
+
char strLocName[82];
|
3554
|
+
|
3555
|
+
memset(strLocName, 0, sizeof(strLocName) );
|
3556
|
+
if ( comment && *comment ) {
|
3557
|
+
strncpy( strLocName, comment, 80 );
|
3558
|
+
}
|
3559
|
+
inchi_print_nodisplay( fcb,"%s\n", strLocName );
|
3560
|
+
} /*block end*/
|
3561
|
+
for (i=0; i< num_atoms; i++)
|
3562
|
+
num_bonds += at[i].valence;
|
3563
|
+
num_bonds /= 2;
|
3564
|
+
|
3565
|
+
/*find if we need "M CHG" and "M RAD"*/
|
3566
|
+
for (i=0, nNumAddLines = 0, nNumIso=0; i < num_atoms; i++) {
|
3567
|
+
bAtomNeedsAlias = ALIASED_AT(i); /* has isotopic implicit D or T; ignoring pure 1H */
|
3568
|
+
nNumAddLines += !bAtomNeedsAlias && ABNORMAL_AT(i); /* abnormal means atom needs CHG, RAD, or ISO entry */
|
3569
|
+
nNumAliasLines += 2 * bAtomNeedsAlias;
|
3570
|
+
nNumIso += ( 0 == strcmp( at[i].elname, "D" ) || ( 0 == strcmp( at[i].elname, "T" ) || at[i].iso_atw_diff ) );
|
3571
|
+
nNumAddIso += at[i].iso_atw_diff && (at[i].iso_atw_diff == 1 || at[i].iso_atw_diff < -3 || at[i].iso_atw_diff > 6 );
|
3572
|
+
}
|
3573
|
+
|
3574
|
+
/* count additional M lines*/
|
3575
|
+
if ( nNumAddLines || nNumAliasLines ) {
|
3576
|
+
for (i=0, nNumChargeLines=0, nNumRadicalLines=0; i < num_atoms; i++) {
|
3577
|
+
nNumChargeLines += (0 != at[i].charge) && !ALIASED_AT(i);
|
3578
|
+
nNumRadicalLines += (0 != at[i].radical) && !ALIASED_AT(i);
|
3579
|
+
}
|
3580
|
+
}
|
3581
|
+
nNumChargeLines = ( nNumChargeLines + 7 ) / 8;
|
3582
|
+
nNumRadicalLines = ( nNumRadicalLines + 7 ) / 8;
|
3583
|
+
nNumIso = ( nNumIso + 7 ) / 8;
|
3584
|
+
/* recalculate number of added lines */
|
3585
|
+
nNumAddLines = nNumChargeLines + nNumRadicalLines + nNumAliasLines; /* 1 for M END*/
|
3586
|
+
|
3587
|
+
if ( nNumAddLines == 0 && nNumAddIso == 0 ) {
|
3588
|
+
nNumIso = 0; /* keep isotopes description in CTable only*/
|
3589
|
+
} else {
|
3590
|
+
nNumAddLines += nNumIso+1; /* add 1 for "M END" line*/
|
3591
|
+
}
|
3592
|
+
if ( !nNumAddLines )
|
3593
|
+
nNumAddLines = 1; /* always add V2000 and M END */
|
3594
|
+
|
3595
|
+
/* aaabbblllfffcccsssxxxrrrpppiiimmmvvvvvv*/
|
3596
|
+
inchi_print_nodisplay(fcb,"%3d%3d 0 0%3d 0 0 0 0 0%3d%s\n",
|
3597
|
+
num_atoms, num_bonds, bChiralFlag?1:0, nNumAddLines,nNumAddLines?" V2000":"");
|
3598
|
+
/* atoms block*/
|
3599
|
+
for (i=0; i < num_atoms; i++) {
|
3600
|
+
char elname[ATOM_EL_LEN] = "\0\0\0\0\0";
|
3601
|
+
int iso = 0;
|
3602
|
+
int charge = 0;
|
3603
|
+
int valence = 0;
|
3604
|
+
bAtomNeedsAlias = ALIASED_AT(i);
|
3605
|
+
/* isotope*/
|
3606
|
+
iso = !strcmp( at[i].elname, "D" )? 1:
|
3607
|
+
!strcmp( at[i].elname, "T" )? 2: 0;
|
3608
|
+
|
3609
|
+
if ( iso ) {
|
3610
|
+
/* deuterium or tritium*/
|
3611
|
+
strcpy ( elname, "H" );
|
3612
|
+
} else
|
3613
|
+
if ( bAtomNeedsAlias ) {
|
3614
|
+
strcpy ( elname, "C" );
|
3615
|
+
} else {
|
3616
|
+
strncpy ( elname, at[i].elname, sizeof(elname)-1 );
|
3617
|
+
}
|
3618
|
+
if ( !iso && at[i].iso_atw_diff && at[i].iso_atw_diff != 1 && -3 <= at[i].iso_atw_diff && at[i].iso_atw_diff <= 5 ) {
|
3619
|
+
iso = (at[i].iso_atw_diff > 0)? at[i].iso_atw_diff-1 : at[i].iso_atw_diff;
|
3620
|
+
}
|
3621
|
+
|
3622
|
+
/*
|
3623
|
+
if ( !iso ) {
|
3624
|
+
strncpy ( elname, at[i].elname, sizeof(elname)-1 );
|
3625
|
+
} else
|
3626
|
+
if ( ALIASED_AT(i) ) {
|
3627
|
+
strcpy ( elname, "C" );
|
3628
|
+
} else {
|
3629
|
+
-- deuterium or tritium --
|
3630
|
+
strcpy ( elname, "H" );
|
3631
|
+
}
|
3632
|
+
*/
|
3633
|
+
if ( !ABNORMAL_AT(i) && !bAtomNeedsAlias ) {
|
3634
|
+
|
3635
|
+
/* Only normal atoms without alias can be here*/
|
3636
|
+
|
3637
|
+
/* charge*/
|
3638
|
+
switch ( at[i].charge ) {
|
3639
|
+
case 3: charge = 1; break;
|
3640
|
+
case 2: charge = 2; break;
|
3641
|
+
case 1: charge = 3; break;
|
3642
|
+
case -1: charge = 5; break;
|
3643
|
+
case -2: charge = 6; break;
|
3644
|
+
case -3: charge = 7; break;
|
3645
|
+
case 0: charge = 0; break;
|
3646
|
+
default: flag_bad_charge = 1; break;
|
3647
|
+
};
|
3648
|
+
/* radical*/
|
3649
|
+
if ( at[i].radical ) {
|
3650
|
+
if ( at[i].radical == RADICAL_DOUBLET ) {
|
3651
|
+
flag_bad_charge |= (charge != 0);
|
3652
|
+
charge = 4;
|
3653
|
+
} else {
|
3654
|
+
flag_bad_charge |= 2;
|
3655
|
+
}
|
3656
|
+
}
|
3657
|
+
if ( flag_bad_charge ) {
|
3658
|
+
charge = 0;
|
3659
|
+
}
|
3660
|
+
}
|
3661
|
+
|
3662
|
+
x = at[i].x;
|
3663
|
+
y = at[i].y;
|
3664
|
+
z = at[i].z;
|
3665
|
+
/* --- just removed --
|
3666
|
+
if ( c && c->xCoeff != 0.0 && c->yCoeff != 0.0 ) {
|
3667
|
+
x = (x - c->xShift)/c->xCoeff;
|
3668
|
+
y = (y - c->yShift)/c->yCoeff;
|
3669
|
+
} else {
|
3670
|
+
y = -y;
|
3671
|
+
}
|
3672
|
+
----------------------*/
|
3673
|
+
/* valence -- set only if needed */
|
3674
|
+
valence=needed_unusual_el_valence( at[i].el_number, at[i].charge, at[i].radical,
|
3675
|
+
at[i].chem_bonds_valence, at[i].num_H, at[i].valence );
|
3676
|
+
if ( valence < 0 ) {
|
3677
|
+
valence = 15; /* means no bonds nor H */
|
3678
|
+
}
|
3679
|
+
|
3680
|
+
/*my_fprintf(fcb,"%10.4f%10.4f%10.4f %-3.3s%2d%3d 0 0 0 0 0 0 0\n",*/
|
3681
|
+
/* (float)at[i].x, (float)(-at[i].y), fzero, at[i].elname, iso, charge);*/
|
3682
|
+
/* xxxxxxyyyyyyzzzzzz aaa____ddcccsssnnnbbbvvvrrriiimmmeee */
|
3683
|
+
inchi_print_nodisplay(fcb,"%10.4f%10.4f%10.4f %-3.3s%2d%3d 0 0%3d 0 0 0 0\n",
|
3684
|
+
x, y, z, elname, (int)iso, (int)charge, valence /* at[i].special*/);
|
3685
|
+
/* reflect image against x-axis;
|
3686
|
+
when transforming MOLfile back to STDATA in mol_to_stdata(...),
|
3687
|
+
make one more reflection to restore original orientation.
|
3688
|
+
Reason: in MS Search y-axis is directed from top to bottom,
|
3689
|
+
while in MOLfile y-axis goes from bottom to top.
|
3690
|
+
*/
|
3691
|
+
}
|
3692
|
+
bNext = 0; /* debug only*/
|
3693
|
+
|
3694
|
+
/* bonds*/
|
3695
|
+
for (i=0; i< num_atoms; i++) {
|
3696
|
+
for (j=0; j<at[i].valence; j++) {
|
3697
|
+
if (i < at[i].neighbor[j]) {
|
3698
|
+
if ( k=at[i].bond_stereo[j] ) {
|
3699
|
+
/* bond stereo */
|
3700
|
+
if ( k < 0 ) {
|
3701
|
+
/* transposition */
|
3702
|
+
inchi_print_nodisplay(fcb,"%3u%3u%3u%3u 0 0 0\n",
|
3703
|
+
(unsigned)(at[i].neighbor[j]+1), (unsigned)(i+1), (unsigned)(at[i].bond_type[j]), (unsigned)abs(k));
|
3704
|
+
} else {
|
3705
|
+
/* no transposition*/
|
3706
|
+
inchi_print_nodisplay(fcb,"%3u%3u%3u%3u 0 0 0\n",
|
3707
|
+
(unsigned)(i+1), (unsigned)(at[i].neighbor[j]+1), (unsigned)(at[i].bond_type[j]), (unsigned)abs(k));
|
3708
|
+
}
|
3709
|
+
} else {
|
3710
|
+
inchi_print_nodisplay(fcb,"%3u%3u%3u 0 0 0 0\n",
|
3711
|
+
(unsigned)(i+1), (unsigned)(at[i].neighbor[j]+1), (unsigned)(at[i].bond_type[j]));
|
3712
|
+
}
|
3713
|
+
}
|
3714
|
+
}
|
3715
|
+
}
|
3716
|
+
if ( nNumAddLines ) {
|
3717
|
+
char str_m[66], entry[10];
|
3718
|
+
int num_m;
|
3719
|
+
|
3720
|
+
/* Aliases. 5-3-99 DCh.*/
|
3721
|
+
if ( nNumAliasLines ) {
|
3722
|
+
num_m = 0;
|
3723
|
+
for (i=0; i < num_atoms; i++) {
|
3724
|
+
if ( ALIASED_AT(i) ) {
|
3725
|
+
int len;
|
3726
|
+
inchi_print_nodisplay( fcb, "A %d\n", i+1 );
|
3727
|
+
num_m ++;
|
3728
|
+
len = sprintf( str_m, "%s", at[i].elname );
|
3729
|
+
/* add isotopic H to the alias */
|
3730
|
+
for ( k = 1; k < NUM_H_ISOTOPES; k ++ ) {
|
3731
|
+
if ( at[i].num_iso_H[k] ) {
|
3732
|
+
len += sprintf( str_m+len, "%s", k==1? "D" : k==2? "T" : "?" );
|
3733
|
+
if ( at[i].num_iso_H[k] != 1 ) {
|
3734
|
+
len += sprintf( str_m+len, "%d", (int)at[i].num_iso_H[k] );
|
3735
|
+
}
|
3736
|
+
}
|
3737
|
+
}
|
3738
|
+
/* Add charge to the Alias */
|
3739
|
+
if ( at[i].charge){
|
3740
|
+
len += sprintf(str_m+len, "%s", at[i].charge>0? "+" : "-");
|
3741
|
+
if ( 1 < (j=abs(at[i].charge)) ) {
|
3742
|
+
len += sprintf( str_m+len, "%d", j );
|
3743
|
+
}
|
3744
|
+
}
|
3745
|
+
/* Add radical to the Alias */
|
3746
|
+
if ( at[i].radical == RADICAL_SINGLET ) {
|
3747
|
+
len += sprintf( str_m+len, "%s", ":" );
|
3748
|
+
} else
|
3749
|
+
if ( at[i].radical == RADICAL_DOUBLET ) {
|
3750
|
+
len += sprintf( str_m+len, "%s", "^" );
|
3751
|
+
} else
|
3752
|
+
if ( at[i].radical == RADICAL_TRIPLET ) {
|
3753
|
+
len += sprintf( str_m+len, "%s", "^^" );
|
3754
|
+
}
|
3755
|
+
inchi_print_nodisplay( fcb, "%s\n", str_m );
|
3756
|
+
num_m ++;
|
3757
|
+
}
|
3758
|
+
}
|
3759
|
+
if ( num_m != nNumAliasLines ) {
|
3760
|
+
/* error in lines counting*/
|
3761
|
+
ret ++;
|
3762
|
+
}
|
3763
|
+
}
|
3764
|
+
/* charges*/
|
3765
|
+
str_m[0] = 0;
|
3766
|
+
num_m = 0;
|
3767
|
+
if ( nNumChargeLines ) {
|
3768
|
+
for (i=0; i < num_atoms; i++) {
|
3769
|
+
if ( at[i].charge && !ALIASED_AT(i) ) {
|
3770
|
+
sprintf( entry, " %3d %3d", i+1, (int)at[i].charge );
|
3771
|
+
strcat( str_m, entry );
|
3772
|
+
num_m ++;
|
3773
|
+
}
|
3774
|
+
if ( i == num_atoms-1 && num_m || num_m == 8 ) {
|
3775
|
+
inchi_print_nodisplay( fcb, "M CHG%3d%s\n", num_m, str_m );
|
3776
|
+
str_m[0] = 0;
|
3777
|
+
num_m = 0;
|
3778
|
+
}
|
3779
|
+
}
|
3780
|
+
}
|
3781
|
+
/* radicals*/
|
3782
|
+
str_m[0] = 0;
|
3783
|
+
num_m = 0;
|
3784
|
+
if ( nNumRadicalLines ) {
|
3785
|
+
for (i=0; i < num_atoms; i++) {
|
3786
|
+
if ( at[i].radical && !ALIASED_AT(i) ) {
|
3787
|
+
int radical = (at[i].radical==RADICAL_SINGLET ||
|
3788
|
+
at[i].radical==RADICAL_DOUBLET ||
|
3789
|
+
at[i].radical==RADICAL_TRIPLET)? at[i].radical : 0;
|
3790
|
+
if ( radical ) {
|
3791
|
+
sprintf( entry, " %3d %3d", i+1, radical );
|
3792
|
+
strcat( str_m, entry );
|
3793
|
+
num_m ++;
|
3794
|
+
}
|
3795
|
+
}
|
3796
|
+
if ( i == num_atoms-1 && num_m || num_m == 8 ) {
|
3797
|
+
inchi_print_nodisplay( fcb, "M RAD%3d%s\n", num_m, str_m );
|
3798
|
+
str_m[0] = 0;
|
3799
|
+
num_m = 0;
|
3800
|
+
}
|
3801
|
+
}
|
3802
|
+
}
|
3803
|
+
/* isotopes*/
|
3804
|
+
str_m[0] = 0;
|
3805
|
+
num_m = 0;
|
3806
|
+
if ( nNumIso ) {
|
3807
|
+
for (i=0; i < num_atoms; i++) {
|
3808
|
+
if ( 0 == strcmp( at[i].elname, "D" ) ) {
|
3809
|
+
sprintf( entry, " %3d %3d", i+1, 2 );
|
3810
|
+
strcat( str_m, entry );
|
3811
|
+
num_m ++;
|
3812
|
+
} else
|
3813
|
+
if ( 0 == strcmp( at[i].elname, "T" ) ) {
|
3814
|
+
sprintf( entry, " %3d %3d", i+1, 3 );
|
3815
|
+
strcat( str_m, entry );
|
3816
|
+
num_m ++;
|
3817
|
+
} else
|
3818
|
+
if ( k = at[i].iso_atw_diff ) {
|
3819
|
+
int mw = get_atw_from_elnum( at[i].el_number );
|
3820
|
+
mw += (k > 0)? k-1 : k;
|
3821
|
+
sprintf( entry, " %3d %3d", i+1, mw );
|
3822
|
+
strcat( str_m, entry );
|
3823
|
+
num_m ++;
|
3824
|
+
}
|
3825
|
+
if ( i == num_atoms-1 && num_m || num_m == 8 ) {
|
3826
|
+
inchi_print_nodisplay( fcb, "M ISO%3d%s\n", num_m, str_m );
|
3827
|
+
str_m[0] = 0;
|
3828
|
+
num_m = 0;
|
3829
|
+
}
|
3830
|
+
}
|
3831
|
+
}
|
3832
|
+
inchi_print_nodisplay( fcb, "M END\n" );
|
3833
|
+
}
|
3834
|
+
if ( szValue && szValue[0] ) {
|
3835
|
+
if ( szLabel && szLabel[0] ) {
|
3836
|
+
inchi_print_nodisplay( fcb, "> <%s>\n", szLabel );
|
3837
|
+
} else {
|
3838
|
+
inchi_print_nodisplay( fcb, "> <ID>\n" );
|
3839
|
+
}
|
3840
|
+
inchi_print_nodisplay( fcb, " %s\n\n", szValue );
|
3841
|
+
}
|
3842
|
+
inchi_print_nodisplay(fcb, "$$$$\n");
|
3843
|
+
|
3844
|
+
|
3845
|
+
return ret;
|
3846
|
+
|
3847
|
+
}
|
3848
|
+
|
3849
|
+
#ifdef INCHI_ANSI_ONLY
|
3850
|
+
#ifndef INCHI_LIBRARY
|
3851
|
+
/*
|
3852
|
+
#include <stdio.h>
|
3853
|
+
#include "inpdef.h"
|
3854
|
+
*/
|
3855
|
+
void PrintFileName( const char *fmt, INCHI_FILE *output_file, const char *szFname )
|
3856
|
+
{
|
3857
|
+
inchi_print_nodisplay( output_file, fmt, szFname );
|
3858
|
+
}
|
3859
|
+
#endif
|
3860
|
+
#endif
|
3861
|
+
|